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We present detailed calculations of the magnetic ground state properties of Cs$_2$CuCl$_4$ in an applied magnetic field, and compare our results with recent experiments. The material is described by a spin Hamiltonian, determined with…

Strongly Correlated Electrons · Physics 2007-05-23 M. Y. Veillette , J. T. Chalker , R. Coldea

We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field…

Strongly Correlated Electrons · Physics 2013-06-25 Y. Tokiwa , T. Radu , R. Coldea , H. Wilhelm , Z. Tylczynski , F. Steglich

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

Strongly Correlated Electrons · Physics 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

Although magnetically ordered at low temperatures, the spin-1/2 triangular antiferromagnet Cs_2CuCl_4 exhibits remarkable spin dynamics that strongly suggest proximity to a spin liquid phase. Here we address the question of whether a…

Strongly Correlated Electrons · Physics 2013-05-29 Jason Alicea , Matthew P. A. Fisher

A field-induced quantum spin liquid (QSL) state is an extraordinary phenomenon, hitherto unobserved in metallic frustrated compounds. Recent bulk measurements have revealed intriguing field-induced magnetic states in metallic frustrated…

Strongly Correlated Electrons · Physics 2026-01-12 I. Ishant , Z. Guguchia , V. Fritsch , O. Stockert , M. Majumder

Quantum triangular-lattice antiferromagnets are important prototype systems to investigate phenomena of the geometrical frustration in condensed matter. Apart from highly unusual magnetic properties, they possess a rich phase diagram…

Strongly Correlated Electrons · Physics 2019-03-13 S. A. Zvyagin , D. Graf , T. Sakurai , S. Kimura , H. Nojiri , J. Wosnitza , H. Ohta , T. Ono , H. Tanaka

Unlike conventional magnets where the magnetic moments are partially or completely static in the ground state, in a quantum spin liquid they remain in collective motion down to the lowest temperatures. The importance of this state is that…

We report a thorough theoretical study of the low temperature phase diagram of Cs_2CuCl_4, a spatially anisotropic spin S=1/2 triangular lattice antiferromagnet, in a magnetic field. Our results, obtained in a quasi-one-dimensional limit in…

Strongly Correlated Electrons · Physics 2015-03-17 Oleg A. Starykh , Hosho Katsura , Leon Balents

We report positive muon spin relaxation measurements on the triangular lattice magnetic system FeGa2S4. A magnetic transition not previously detected by specific heat and magnetic susceptibility measurements is found in zero field at T^*…

Strongly Correlated Electrons · Physics 2012-04-25 P. Dalmas de Reotier , A. Yaouanc , D. E. MacLaughlin , Songrui Zhao , T. Higo , S. Nakatsuji , Y. Nambu , C. Marin , G. Lapertot , A. Amato , C. Baines

We study spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single crystal neutron scattering in zero and applied magnetic field. The magnetically ordered phase appearing below TN=8 K remains nonconventional…

Using ac susceptibility, dc magnetization and heat capacity measurements, we have investigated the magnetic properties of $Cd_{0.5}Cu_{0.5}Cr_2O_4$. $Cd_{0.5}Cu_{0.5}Cr_2O_4$ has an extraordinary magnetic phase including a metastable…

Materials Science · Physics 2015-05-13 Li-qin Yan , Wen Yin , Ferran Maciá , Jun-rong Zhang , Lun-hua He , Fang-wei Wang

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…

KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…

Strongly Correlated Electrons · Physics 2009-11-13 K. Goto , T. Osakabe , K. Kakurai , Y. Uwatoko , A. Oosawa , J. Kawakami , H. Tanaka

The study of magnetic frustration in classical spin systems was motivated by the prediction and discovery of classical spin liquid states. These uncommon magnetic phases are characterized by a massive degeneracy of their ground state…

Realisation of the tetragonal phase of $Cs_2CuCl_4$ is possible using specific crystal growth conditions at a temperature below $281K$. This work deals with the comparison of the magnetic susceptibility and the magnetization of this new…

Cs2CoBr4 is a triangular-lattice antiferromagnet which can be viewed as weakly interacting spin chains due to spatially anisotropic frustrating exchange couplings. The spin-orbit interaction in Co(2+) spin-3/2 ions leads to a strong…

Strongly Correlated Electrons · Physics 2023-09-06 T. A. Soldatov , A. I. Smirnov , A. V. Syromyatnikov

CuAl2O4 is a normal spinel oxide having quantum spin, S=1/2 for Cu2+. It is a rather unique feature that the Cu2+ ions of CuAl2O4 sit at a tetrahedral position, not like the usual octahedral position for many oxides. At low temperatures, it…

Magnetization and neutron elastic scattering measurements under a hydrostatic pressure were performed on KCuCl3, which is a three-dimensionally coupled spin dimer system with a gapped ground state. It was found that an intradimer…

Collective behaviour of electrons, frustration induced quantum fluctuations and entanglement in quantum materials underlie some of the emergent quantum phenomena with exotic quasi-particle excitations that are highly relevant for…

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

Strongly Correlated Electrons · Physics 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato
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