Related papers: Shaping Long-lived Electron Wavepackets for Custom…
The study of electronic transitions within a molecule connected to the absorption or emission of light is a common task in the process of the design of new materials. The transitions are complex quantum mechanical processes and a detailed…
The internal electric field of a Rydberg atom electron can bind a polar molecule to form a giant ultralong-range stable polyatomic molecule. Such molecules not only share their properties with Rydberg atoms, they possess huge permanent…
An electromagnetic wave-packet propagating in a linear, homogeneous, and isotropic medium changes shape while its envelope travels with different velocities at different points in spacetime. In general, a wave-packet can be described as a…
Engineering the electromagnetic environment of a quantum emitter gives rise to a plethora of exotic light-matter interactions. In particular, photonic lattices can seed long-lived atom-photon bound states inside photonic band gaps. Here we…
Rydberg blockade physics in optically dense atomic media under the conditions of electromagnetically induced transparency (EIT) leads to strong dissipative interactions between single photons. We introduce a new approach to analyzing this…
Resonant dipole-dipole interaction modifies the energy and decay rate of electronic excitations for finite one dimensional chains of ultracold atoms in an optical lattice. We show that collective excited states of the atomic chain can be…
Coupling light to ensembles of strongly interacting particles has emerged as a promising route toward achieving few photon nonlinearities. One specific way to implement this kind of nonlinearity is to interface light with highly excited…
Graph states are versatile resources for quantum computation and quantum-enhanced measurement. Their generation illustrates a high level of control over entanglement. We report on the generation of continuous-variable graph states of atomic…
Shaping the electron wavefunction in three dimensions may prove to be an indispensable tool for research involving atomic-sized particle trapping, manipulation, and synthesis. We utilize computer-generated holograms to sculpt electron…
Van der Waals interactions, as a result of the exchange of photons between particles, can be altered by modifying the environment through which these photons propagate. As a consequence, phenomena such as the Rydberg blockade mechanism…
We consider free electrons in rectangular quantum dots, with either hard wall boundary conditions or anharmonic confinement. In both cases, due to finite size effects, a homogeneous electric field applied along one of the rectangular axis…
Controlling free-electron momentum states is of high interest in electron microscopy to achieve momentum and energy resolved probing and manipulation of physical systems. Free-electron and light interactions have emerged as a powerful…
We propose a wave packet basis for storing and processing several qubits of quantum information in a single multilevel atom. Using radially localized wave packet states in the Rydberg atom, we construct an orthogonal basis that is related…
Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…
We present a comprehensive study of the diverse properties of heteronuclear Rydberg molecules, placing a special emphasis on those composed of the light alkali atoms, Li, Na, and K. Electron-atom scattering phase shifts, which determine the…
It is common knowledge that atoms can form molecules if they attract each other. Here, we show that it is possible to create molecules where bound states of the atoms are not the result of attractive interactions but have the topological…
Obtaining full control over the internal and external quantum states of molecules is the central goal of ultracold chemistry and allows for the study of coherent molecular dynamics, collisions and tests of fundamental laws of physics. When…
A few-body approach relying on static line broadening theory is developed to treat the spectroscopy of a single Rydberg excitation to a trilobite-like state immersed in a high density ultracold medium. The present theoretical framework…
We show here that the photonic states emitted by ensembles of multilevel atoms via a superradiance process exhibit entanglement in the modal (frequency) degree of freedom, making this collective emission process a favorable candidate for a…
The properties and behaviour of a Ring Rydberg Composite are explicated. This system consists of a ring of ground state atoms centered on a Rydberg atom, whose electron elastically scatters off the ground state atoms. We transform the…