Related papers: Coherent dynamics in cavity femtochemistry: applic…
A coherent superposition of two electronic states of ozone (ground and Hartley B) is prepared with a UV pump pulse. Using the multiconfiguration time-dependent Hartree approach, we calculate the subsequent time evolution of the two…
Quantum mechanical phenomena, such as electronic coherence and entanglement, play a key role in achieving the unrivalled efficiencies of light-energy conversion in natural photosynthetic light-harvesting complexes, and triggered the growing…
The cause of decoherence in a quantum system can be traced back to the interaction with the environment. As it has been pointed out first by Dicke, in a system of N two-level atoms where each of the atoms is individually dipole coupled to…
The creation of light-matter hybrid states, polaritons, in a cavity offers new intriguing opportunities to manipulate the electronic structure and electron dynamics of atoms and molecules. Here, we investigate the effect of electronic…
We report on the fast excitation of a single atom coupled to an optical cavity using laser pulses that are much shorter than all other relevant processes. The cavity frequency constitutes a control parameter that allows the creation of…
Ultrafast laser pulse has provided a systematic way to inspect the dynamics of electrons in condensed matter systems. In this paper, by means of time-dependent density matrix renormalization group, we study an ultrafast laser driven Kondo…
Coherence and de-coherence are the most fundamental steps that follow the initial photo-excitation occurring in typical Pump&Probe experiments. Indeed, the initial external laser pulse transfers coherence to the system in terms of creation…
Nonperturbative coupling of light with condensed matter in an optical cavity is expected to reveal a host of coherent many-body phenomena and states. In addition, strong coherent light-matter interaction in a solid-state environment is of…
We present a quantum-state-diffusion equation to characterize the dynamics of a generic atomic system coupled to a leaky cavity mode. As quantum resources, the population, the coherence and even the entanglement of the system would…
We study the ultrafast dynamics initiated by a coherent superposition of core-excited states of nitrous oxide molecule. Using high-level \textit{ab-initio} methods, we show that the decoherence caused by the electronic decay and the nuclear…
Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…
Experimental studies indicate that optical cavities can affect chemical reactions, through either vibrational or electronic strong coupling and the quantized cavity modes. However, the current understanding of the interplay between…
Superradiance is the archetypical collective phenomenon where radiation is amplified by the coherence of emitters. It plays a prominent role in optics, where it enables the design of lasers with substantially reduced linewidths, quantum…
Photoionization using attosecond pulses can lead to the formation of coherent superpositions of the electronic states of the parent ion. However, ultrafast electron ejection triggers not only electronic but also nuclear dynamics---leading…
A recent discussion of quantum limitations to the fidelity with which superpositions of internal atomic energy levels can be generated by an applied, quantized, laser pulse is shown to be based on unrealistic physical assumptions. This…
We report on the transfer of coherence from a quantum-well electron-hole condensate to the light it emits. As a function of density, the coherence of the electron-hole pair system evolves from being full for the low density Bose-Einstein…
Recent experiments have demonstrated that molecular polaritons, hybrid states of light and matter formed by the strong coupling between molecular electronic or vibrational excitations and an optical cavity, can substantially modify the…
We perform a theoretical study of a continuous superradiant laser supporting its experimental realization at FEMTO-ST using two sequentially-emitting ensembles of ${}^{171}\mathrm{Yb}$ atoms coupled to the same Fabry-Perot cavity. Using an…
The development of reliable ab initio methods for light-matter strong coupling is necessary for a deeper understanding of molecular polaritons. The recently developed strong coupling quantum electrodynamics Hartree-Fock model (SC-QED-HF)…
We describe the decoherence-free subspace of N atoms in a cavity, in which decoherence due to the leakage of photons through the cavity mirrors is suppressed. We show how the states of the subspace can be entangled with the help of weak…