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We studied the optical properties of antiferromagnetic ZnCr2Se4 by infrared spectroscopy up to 28,000 cm-1 and for temperatures from 5 to 295 K. At the magnetic phase transition at 21 K, one of the four phonon modes reveals a clear…

Strongly Correlated Electrons · Physics 2009-04-01 T. Rudolf , Ch. Kant , F. Mayr , M. Schmidt , V. Tsurkan , J. Deisenhofer , A. Loidl

The spin-phonon coupling in magnetic materials is due to the modulation of the exchange integral by lattice vibrations. BaFe12O19 M-type hexaferrite, which is the most used magnetic material as permanent magnet, transforms into ferromagnet…

Materials Science · Physics 2015-06-22 Flávio M. Silva Júnior , Carlos W. A. Paschoal

Including the orbital off-diagonal spin and charge condensates in the self consistent determination of magnetic order within a realistic three-orbital model for the $4d^4$ compound $\rm Ca_2 Ru O_4$, reveals a host of novel features…

Strongly Correlated Electrons · Physics 2021-07-05 Shubhajyoti Mohapatra , Avinash Singh

Using a combination of first-principles and magnetization-dynamics calculations, we study the effect of the intense optical excitation of phonons on the magnetic behavior in insulating magnetic materials. Taking the prototypical…

Strongly Correlated Electrons · Physics 2018-06-13 M. Fechner , A. Sukhov , L. Chotorlishvili , C. Kenel , J. Berakdar , N. A. Spaldin

Among hundreds of spinel oxides, LiTi2O4 (LTO) is the only one that exhibits superconductivity (Tc ~13 K). Although the general electron-phonon coupling is still the main mechanism for electron pairing in LTO, unconventional behaviors such…

The lattice dynamics and the effect of pressure on superconducting LiFeAs in both nonmagnetic (NM) and striped antiferromagnetic (SAF) phases are investigated using the plane-wave pseudopotential, density-functional-based method. While the…

Superconductivity · Physics 2010-07-13 G. Q. Huang , Z. W. Xing , D. Y. Xing

Exploring ultrafast magnetization control in two-dimensional (2D) magnets through optically driven coherent phonons has been well-established. Yet, the microscopic interplay between spin dynamics and lattice degrees of freedom remains less…

Computational Physics · Physics 2024-03-25 Zhaobo Zhou , Min Li , Thomas Frauenheim , Junjie He

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond…

The coupling between antiferromagnetic spins and infrared-active phonons in solids is responsible for many intriguing phenomena and is a field of intense research with extensive potential applications in the modern devices based on…

Synthetic antiferromagnet, comprised of two ferromagnetic layers separated by a non-magnetic layer, possesses two uniform precession resonance modes: in-phase acoustic mode and out-of-phase optic mode. In this work, we theoretically and…

Strongly Correlated Electrons · Physics 2021-03-19 Changting Dai , Fusheng Ma

The observation of strongly coupled lattice and spin dynamics in altermagnet CoF$_2$ is reported. On the background of the expected spin-phonon interaction leading to renormalization of all phonons at the Neel temperature an additional…

Materials Science · Physics 2024-05-14 M. A. Prosnikov , M. Bal , R. V. Pisarev , P. C. M. Christianen , A. M. Kalashnikova

We provide a theoretical demonstration of controllable non-relativistic spin splitting in both electronic and magnonic bands via targeted structural distortions tied to specific phonon modes. Using MnF$_2$ as a model system, we identify a…

Materials Science · Physics 2025-09-11 Subhadeep Bandyopadhyay , Anoop Raj , Philippe Ghosez , Sumiran Pujari , Sayantika Bhowal

Detailed far-infrared spectra of the optical phonons are reported for antiferromagnetic MnO. Eigenfrequencies, phonon damping and effective plasma frequencies are studied as a function of temperature. Special attention is paid to the phonon…

Strongly Correlated Electrons · Physics 2008-06-26 T. Rudolf , Ch. Kant , F. Mayr , A. Loidl

We employ polarization-resolved Raman spectroscopy and first-principles phonon calculations to study the lattice dynamics and spin-phonon coupling in the kagome spin ice compound HoAgGe. Upon cooling, HoAgGe shows transitions from a…

Strongly Correlated Electrons · Physics 2025-03-11 Shangfei Wu , Lingxiao Zhao , Wei Song , Mingshu Tan , Feng Jin , Tianping Ying , Jia-Xin Yin , Qingming Zhang

Strongly anisotropic spin-orbit coupling (SOC) renormalization and strongly enhanced orbital magnetic moments are obtained in the fully self consistent approach including the orbital off-diagonal spin and charge condensates. For moderate…

Strongly Correlated Electrons · Physics 2021-07-05 Shubhajyoti Mohapatra , Ritajit Kundu , Ashutosh Dubey , Debasis Dutta , Avinash Singh

Magnetic order typically emerges due to the short-range exchange interaction between the constituent electronic spins. Recent discoveries have found a crucial role for spin-phonon coupling in various phenomena from optical ultrafast…

Mesoscale and Nanoscale Physics · Physics 2024-05-16 Petros Andreas Pantazopoulos , Johannes Feist , Francisco J. García-Vidal , Akashdeep Kamra

In this Rapid Communication we investigate the coupling between excited electrons and phonons in the highly anisotropic electronic structure of the prototypical topological insulator Bi$_2$Te$_3$. Using time- and angle-resolved…

Mesoscale and Nanoscale Physics · Physics 2016-10-13 E. Golias , J. Sánchez-Barriga

Quantum coherent coupling between a zone-center phonon and two acoustic phonons was observed in two GaAs/AlAs superlattices (8 nm/8 nm and 5.4 nm/5.4 nm) at ambient temperature. Using degenerate coherent phonon spectroscopy, a multi-cycle…

Materials Science · Physics 2019-07-25 Feng He , Nathanial Sheehan , Seth R Bank , Raymond L Orbach , Yaguo Wang

The transport and magnetic properties of correlated La{0.53}Sr{0.47}MnO{3} ultrathin films, grown epitaxially on SrTiO{3}, show a sharp cusp at the structural transition temperature of the substrate. Using a combination of experiment and…

Materials Science · Physics 2011-09-09 Y. Segal , K. F. Garrity , C. A. F. Vaz , J. D. Hoffman , F. J. Walker , S. Ismail-Beigi , C. H. Ahn

The ScAu$_2$Al superconducting Heusler-type compound was recently characterized to have the highest critical temperature of $T_c = 5.12$ K and the strongest electron-phonon coupling among the Heusler family. In this work, the electronic…

Superconductivity · Physics 2023-12-04 Gabriel Kuderowicz , Bartlomiej Wiendlocha