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We employ an optical pump-probe technique to study coherent phonon oscillations in Ca$_2$RuO$_4$. We find that oscillation-amplitude of an $A_g$ symmetric phonon mode is strongly suppressed at 260 K, a putative transition point of orbital…

Strongly Correlated Electrons · Physics 2018-10-24 Min-Cheol Lee , Choong H. Kim , Inho Kwak , J. Kim , S. Yoon , Byung Cheol Park , Bumjoo Lee , F. Nakamura , C. Sow , Y. Maeno , T. W. Noh , K. W. Kim

The lattice dynamic properties and spin-phonon coupling in DyMn$_2$O$_5$ are studied by using the density-functional theory. The calculated phonon frequencies are in very good agreement with experiments. We then compare the phonon modes…

Materials Science · Physics 2009-11-13 Tianqi Shen , Kun Cao , Guang-Can Guo , Lixin He

The temperature dependence of eigenfrequencies and intensities of the IR active modes has been investigated for the antiferromagnetic chromium spinel compounds CdCr2O4, ZnCr2O4, ZnCr2S4, ZnCr2Se4, and HgCr2S4 by IR spectroscopy for…

Strongly Correlated Electrons · Physics 2007-07-05 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

We study the magnetically-induced phonon splitting in cubic ACr$_2$O$_4$ (A=Mg, Zn, Cd, Hg) spinels from first principles, and demonstrate that the sign of the splitting, which is experimentally observed to be opposite in CdCr$_2$O$_4$…

Materials Science · Physics 2016-05-04 Aleksander L. Wysocki , Turan Birol

Raman study on a select few orthochromites, RCrO$_3$ (R = Y, Lu, Gd, Eu and Sm) shows that the phonon behavior at TN in compounds with magnetic R-ion (Gd and Sm) is remarkably different from that of non-magnetic R-ion (Y, Lu and Eu). While…

Materials Science · Physics 2013-06-11 Venkata Srinu Bhadram , B. Rajeswaran , A. Sundaresan , Chandrabhas Narayana

Band calculations show that a stripe-like anti-ferromagnetic spin wave is enforced by a 'half-breathing' phonon distortion within the CuO plane of HgBa_2CuO_4. This spin-phonon coupling is increased further by shear distortion and by…

Superconductivity · Physics 2009-11-10 T. Jarlborg

Magnetic order parameters in altermagnets can couple to quantized lattice vibration via both piezomagnetic and magnetoelastic effects, leading to the renormalization of phonon dispersion. Here, we demonstrate photo-induced dynamic frequency…

Spin-phonon coupling and magnetodielectric effects of ZnCr2Se4 were investigated by means of infrared (IR) spectroscopy as a function of temperature and magnetic field. ZnCr2Se4 is dominated by ferromagnetic exchange but undergoes…

Strongly Correlated Electrons · Physics 2007-07-05 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

We demonstrate that the onset of complex spin orders in ACr$_2$O$_4$ spinels with magnetic A$=$Co, Fe and Cu ions lowers the lattice symmetry. This is clearly indicated by the emergence of anisotropic lattice dynamics -- as evidenced by the…

Strongly Correlated Electrons · Physics 2014-01-15 S. Bordacs , D. Varjas , I. Kezsmarki , G. Mihaly , L. Baldassarre , A. Abouelsayed , C. A. Kuntscher , K. Ohgushi , Y. Tokura

New surprises continue to be revealed about La$_2$CuO$_4$, the parent compound of the original cuprate superconductor. Here we present neutron scattering evidence that the structural symmetry is lower than commonly assumed. The static…

The infrared phonon spectrum of the spinel CdCr2O4 is measured as a function temperature from 6 K to 300K. The triply degenerate Cr phonons soften in the paramagnetic phase as temperature is lowered below 100 K and then split into a singlet…

Materials Science · Physics 2009-11-13 R. Valdés Aguilar , A. B. Sushkov , Y. J. Choi , S-W. Cheong , H. D. Drew

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The…

Strongly Correlated Electrons · Physics 2019-04-23 Kousik Samanta , Danilo Rigitano , Pascoal Jose Giglio Pagliuso , Eduardo Granado

We study the effect of spin-phonon coupling in small magnetic clusters, concentrating on a S=1/2 ring of 4 spins coupled antiferromagnetically. If the phonons are treated as classical variables, there is a critical value of the spin-phonon…

Strongly Correlated Electrons · Physics 2009-11-11 M. Elhajal , F. Mila

MnV$_2$O$_4$ in the spinel structure is known to exhibit coupled orbital and spin ordering, and its Raman spectra show interesting anomalies in its low-temperature phase. With a goal to explain this behavior involving coupled spins and…

Materials Science · Physics 2020-05-27 Dibyendu Dey , T. Maitra , U. V. Waghmare , A. Taraphder

While the dominant magnetic interaction in La$_2$CuO$_4$ is superexchange between nearest-neighbor Cu moments, the pinning of the spin direction depends on weak anisotropic effects associated with spin-orbit coupling. The symmetry of the…

Strongly Correlated Electrons · Physics 2023-03-17 Xiao Hu , A. Sapkota , V. O. Galea , G. D. Gu , I. A. Zaliznyak , J. M. Tranquada

The magnon disp ersion in Ca2RuO4 has been determined by inelastic neutron scattering on single crytals containing 1% of Ti. The dispersion is well described by a conventional Heisenberg model suggesting a local moment model with nearest…

Strongly Correlated Electrons · Physics 2015-12-16 S. Kunkemöller , D. Khomskii , P. Steffens , A. Piovano , A. Nugroho , M. Braden

In order to explore the consequences of spin-orbit coupling on spin-phonon interactions in a set of chemically-similar mixed metal oxides, we measured the infrared vibrational properties of Co$_4B_2$O$_9$ ($B$ = Nb, Ta) as a function of…

Materials Science · Physics 2023-05-26 K. Park , J. Kim , S. Choi , S. Fan , C. Kim , D. G. Oh , N. Lee , S. -W. Cheong , V. Kiryukhin , Y. J. Choi , D. Vanderbilt , J. H. Lee , J. L. Musfeldt

We used polarization-resolved Raman scattering to study the magneto-elastic coupling in the parent compounds of several families of Fe-based superconductors (BaFe2As2, EuFe2As2, NaFeAs, LiFeAs, FeSe and LaFeAsO). We observe an emergent…

We study spin relaxation and decoherence in a GaAs quantum dot due to spin-orbit interaction. We derive an effective Hamiltonian which couples the electron spin to phonons or any other fluctuation of the dot potential. We show that the spin…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Vitaly N. Golovach , Alexander Khaetskii , Daniel Loss

Multifunctional properties in quantum systems require the interaction between different degrees of freedom. As such, spin-phonon coupling emerges as an ideal mechanism to tune multiferroicity, magnetism, and magnetoelectric response. In…

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