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Chalcogenide perovskites provide a promising avenue for non-toxic, stable thermoelectric materials. Here, thermal transport and thermoelectric properties of BaZrS$_3$ as a typical orthorhombic perovskite are investigated. An extremely low…

Materials Science · Physics 2023-12-14 Yu Wu , Ying Chen , Qiaoqiao Li , Kui Xue , Hezhu Shao , Hao Zhang , Liujiang Zhou

The potential of lead-halide perovskites for realistic applications is currently hindered by their limited long-term stability under functional activation. While the role of lattice flexibility in the thermal response of perovskites has…

Theoretical DFT calculations using GGA+U and HSE06 frameworks enabled vibrational mode assignment and partial (atomic) phonon DOS determination in KAgF3 perovskite, a low-dimensional magnetic fluoroargentate(II). Twelve bands in the spectra…

Materials Science · Physics 2021-01-20 Kacper Koteras , Jakub Gawraczynski , Mariana Derzsi , Zoran Mazej , Wojciech Grochala

The insulating ferrimagnet Cu2OSeO3 shows a rich variety of phases such as skyrmion lattice and helical magnetism controlled by interplay of different exchange interactions which can be tuned by external pressure. In this work we have…

Inorganic halide perovskites have emerged as a promising platform in a wide range of applications from solar energy harvesting to computing, and light emission. The recent advent of epitaxial thin film growth of halide perovskites has made…

Mesoscale and Nanoscale Physics · Physics 2021-08-16 K. Nasyedkin , I. King , L. Zhang , P. Chen , L. Wang , R. J. Staples , R. R. Lunt , J. Pollanen

Under external stimuli, lead halide perovskites exhibit large atomic fluctuations, impacting optical and electron transport properties that affect device performance in operational settings. However, a thorough understanding of the atomic…

The anomalous thermal expansion in a layered 3$d$-5$d$ based triple perovskite iridate Ba$_{3}$CoIr$_{2}$O$_{9}$ is investigated using high resolution synchrotron diffraction. Below the magneto-structural transition at 107\,K, the onset of…

Strongly Correlated Electrons · Physics 2021-04-21 Charu Garg , Antonio Cervellino , Sunil Nair

Tin-based halide perovskites have emerged as promising lead-free alternatives for optoelectronic applications, yet their structural stability and phase behavior at finite temperatures remain challenging to predict. Here, we assess the…

Materials Science · Physics 2026-05-18 Thiago Puccinelli , Lucas Martin Farigliano , Gustavo Martini Dalpian

The centrosymmetric halide perovskites undergo a continuous phase transition from a normal insulator to a topological insulator at the critical value of strain. Contrarily, in noncentrosymmetric halide perovskites, this phase transition is…

Materials Science · Physics 2023-02-28 Ankita Phutela , Sajjan Shoeran , Saswata Bhattacharya

Newly synthesized perovskite NaOsO3 shows Curie-Weiss metallic nature at high temperature and suddenly goes into an antiferromagnetically insulating state at 410 K on cooling. Electronic specific heat at the low temperature limit is absent,…

Strongly Correlated Electrons · Physics 2015-05-14 Y. G. Shi , Y. F. Guo , S. Yu , M. Arai , A. A. Belik , A. Sato , K. Yamaura , E. Takayama-Muromachi , H. F. Tian , H. X. Yang , J. Q. Li , T. Varga , J. F. Mitchell , S. Okamoto

Using path-integral Monte Carol simulations and an ab initio effective Hamiltonian, we study the effects of quantum fluctuations on structural phase transitions in the cubic perovskite compounds SrTiO3 and BaTiO3. We find quantum…

mtrl-th · Physics 2009-10-28 W. Zhong , David Vanderbilt

Several experiments conducted over decades have revealed that the perovskite-structured BaCeO3 goes through a series of temperature-induced structural phase transitions. However, it has been frequently observed that the number of phases and…

Chalcogenide perovskites are lead-free materials for potential photovoltaic or thermoelectric applications. BaZrS$_3$ is the most studied member of this family due to its superior thermal and chemical stability, desirable optoelectronic…

Materials Science · Physics 2025-02-10 Prakriti Kayastha , Erik Fransson , Paul Erhart , Lucy D. Whalley

Metal halide perovskites are multifunctional semiconductors with tunable structures and properties. They are highly dynamic crystals with complex octahedral tilting patterns and strongly anharmonic atomic behaviour. In the higher…

In recent years, quantum phase transitions have attracted the interest of both theorists and experimentalists in condensed matter physics. These transitions, which are accessed at zero temperature by variation of a non-thermal control…

Condensed Matter · Physics 2009-11-10 Matthias Vojta

Low temperature properties of BaZrO3 are revealed by combining experimental techniques (X-ray diffraction, neutron scattering and dielectric measurements) with theoretical first-principles-based methods (total energy and linear response…

Materials Science · Physics 2009-11-11 A. R. Akbarzadeh , I. Kornev , C. Malibert , L. Bellaiche , J. M. Kiat

With the development of electronic structure theory, a new class of materials - quantum ones has been recognized by the community. Traditionally, it has been believed that the properties of such compounds cannot be described within the…

Materials Science · Physics 2023-11-10 Himanshu Joshi , Mateusz Wlazło , Harshan Reddy Gopidi , Oleksandr I. Malyi

We report the single-crystal X-ray analysis and magnetic properties of a new double-layered perovskite antiferromagnet, Cs$_3$Cu$_2$Cl$_4$Br$_3$. This structure is composed of Cu$_2$Cl$_4$Br$_3$ double layers with elongated CuCl$_4$Br$_2$…

Strongly Correlated Electrons · Physics 2015-06-25 F. Yamada , T. Ono , H. Tanaka , J. Yamaura

Magnetometry, electrical transport, and neutron scattering measurements were performed on single crystals of the Fe^{4+}-containing perovskite-related phase Sr_3Fe_2O_7-x as a function of oxygen content. Although both the crystal structure…

Strongly Correlated Electrons · Physics 2013-06-12 D. C. Peets , J. -H. Kim , P. Dosanjh , M. Reehuis , A. Maljuk , N. Aliouane , C. Ulrich , B. Keimer

Transition-metal perovskite oxides constitute a series of functional material systems for electronics, catalysis and energy-conversion processes, in which oxygen migration and evolution play a key role. However, the stable metal-oxygen…

Materials Science · Physics 2021-11-02 Qian Wang , Youdi Gu , Wenxuan Zhu , Lei Han , Feng Pan , Cheng Song