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Research into the efficiency of photosynthetic light harvesting has focused on two factors: (1) entanglement of chromophores, and (2) environmental noise. While chromophores are conjugated $\pi$-bonding molecules with strongly correlated…

Biological Physics · Physics 2013-03-29 David A. Mazziotti

The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…

Atomic Physics · Physics 2021-11-24 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits…

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

Temporal correlations in pulsed electron beams reflect the microscopic dynamics of emission and interparticle interaction. In femtosecond electron emission from nanoscale field emitters, Coulomb interactions result in structured…

Mesoscale and Nanoscale Physics · Physics 2025-05-16 Rudolf Haindl , Valerio Di Giulio , Armin Feist , Claus Ropers

We present a theoretical study of atomic ionization due to an XUV pulse in the presence of an infrared laser. Within the strong field approximation and considering the periodicity and symmetry of the transition matrix we show that the…

Atomic Physics · Physics 2020-08-26 Renata Della Picca , Ana Alicia Gramajo , Sebastián López , Diego G Arbó

We investigate the ionization dynamics of Argon atoms irradiated by an ultrashort intense laser of a wavelength up to 3100 nm, addressing the momentum distribution of the photoelectrons with near-zero-energy. We find a surprising…

Atomic Physics · Physics 2014-03-04 Q. Z. Xia , D. F. Ye , L. B. Fu , X. Y. Han , J. Liu

We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…

Atomic Physics · Physics 2015-06-12 J. M. Dahlström , T. Carette , E. Lindroth

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

The cross section for single K-shell ionization by a high-energy photon is evaluated in the next-to-leading order of the nonrelativistic perturbation theory with respect to the electron-electron interaction. The screening corrections are of…

Atomic Physics · Physics 2009-11-11 A. I. Mikhailov , A. V. Nefiodov , G. Plunien

The multiphoton ionization rate of molecules depends on the alignment of the molecular axis with respect to the ionizing laser polarization. By studying molecular frame photo-electron angular distributions from N$_2$, O$_2$ and benzene, we…

Chemical Physics · Physics 2015-06-15 C T L Smeenk , L Arissian , A V Sokolov , M Spanner , K F Lee , A Staudte , D M Villeneuve , P B Corkum

We investigate the influence of relativistic nondipole effects on the photoelectron spectra of argon, particularly in the low kinetic energy region (0 eV - 5 eV). In our experiment, we use intense linearly polarised 800 nm laser pulse to…

Atomic Physics · Physics 2022-03-14 Nida Haram , Han Xu , Igor Ivanov , Dashavir Chetty , Igor Litvinyuk , R. T. Sang

We have considered the processes of excitation and ionization of light multicharged ions by impact of high-energy particles, which proceed with participation of the $ns$ electrons. The screening corrections to the energy levels and…

Atomic Physics · Physics 2009-11-13 A. V. Nefiodov , G. Plunien

We study the interconnection between the results of two qualitatively different approximate calculations of photoionization cross sections, $\sigma_{n\ell}$, for neutral atoms ($A$) or their cations ($A^+$), centrally confined inside a…

Atomic Physics · Physics 2024-09-19 V. K. Dolmatov , L. V. Chernysheva , V. G. Yarzhemsky

The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…

We demonstrate rather interesting manifestations of co-existence of resonance features in characteristics of the photoionization of 3d-electrons in Xe@C60. It is shown that the reflection of photoelectrons produced by the 3d Xe…

Atomic Physics · Physics 2009-11-13 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

Isotopic substitution in molecular systems can affect fundamental molecular properties including the energy position and spacing of electronic, vibrational and rotational levels, thus modifying the dynamics associated to their coherent…

We theoretically study how time- and angle-resolved photoemission spectroscopy can be applied for imaging coherent electron dynamics in molecules. We consider a process in which a pump pulse triggers coherent electronic dynamics in a…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Jochen Küpper , Robin Santra

We generalize the one electron attosecond streaking camera to time-resolve the correlated two-electron escape dynamics during a collision process involving a deep core electron. The collision process is triggered by an XUV attosecond pulse…

Atomic Physics · Physics 2010-03-09 A. Emmanouilidou , A. Staudte , P. B. Corkum

The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the…