Related papers: Frustration-induced internal stresses are responsi…
Since the discovery of spin glasses in dilute magnetic systems, their study has been largely focused on understanding randomness and defects as the driving mechanism. The same paradigm has also been applied to explain glassy states found in…
The low-frequency vibrations of glasses are markedly different from those of crystals. These vibrations have recently been categorized into two types: spatially extended vibrations, whose vibrational density of states (vDOS) follows a…
Recent studies point out far-reaching connections between the topological characteristics of structural glasses and their material properties, paralleling results in quantum physics that highlight the relevance of the nature of the…
The effect of ring stiffness and pressure on the glassy dynamics of a thermal assembly of two-dimensional ring polymers is investigated using extensive coarse-grained molecular dynamics simulations. In all cases, dynamical slowing down is…
Many systems, including polymers and molecular liquids, when adequately cooled and/or compressed, solidify into a disordered solid, i.e., a glass. The~transition is not abrupt, featuring progressive decrease of the microscopic mobility and…
We study the vibrational spectra and the specific heat of disordered systems using an effective hydrodynamic framework. We consider the contribution of diffusive modes, i.e. the 'diffusons', to the density of states and the specific heat.…
In glass, starting from a dependence of the Angell's fragility on the Poisson ratio [V. N. Novikov and A. P. Sokolov, Nature 431, 961 (2004)], and a dependence of the Poisson ratio on the atomic packing density [G. N. Greaves et al., Nat.…
The structural description for the intriguing link between the fast vibrational dynamics and slow diffusive dynamics in glass-forming systems is one of the most challenging issues in physical science. Here, in a model of metallic…
Understanding how frustration and disorder shape relaxation in complex systems is a central problem in statistical physics and quantum annealing. Spin-glass models provide a natural framework to explore this connection, as their energy…
We present a finite-size study of the athermal quasistatic yielding transition in structural glasses featuring a wide range of mechanical disorder. We find a crossover from gradual yielding in small systems, to a macroscopic discontinuous…
We compare the harmonic and anharmonic properties of the vibrational modes in 3-dimensional jammed packings of frictionless spheres interacting via repulsive, finite range potentials. A crossover frequency is apparent in the density of…
We examine the structural relaxation of glassy materials at finite temperatures, considering the effect of activated rearrangements and long-range elastic interactions. Our three-dimensional mesoscopic relaxation model shows how the…
Geometric frustration describes the inability of a local molecular arrangement, such as icosahedra found in metallic glasses and in model atomic glass-formers, to tile space. Local icosahedral order however is strongly frustrated in…
We study the viscoelastic response of amorphous polymers using theory and simulations. By accounting for internal stresses and considering instantaneous normal modes (INMs) within athermal non-affine theory, we make parameter-free…
Glasses are mechanically rigid, still undergo structural relaxation which changes their properties and affects potential technological applications. Understanding the underlying physical processes is a problem of broad theoretical and…
In spin-glass systems, frustration can be adjusted continuously and considerably, without changing the antiferromagnetic bond probability p, by using locally correlated quenched randomness, as we demonstrate here on hypercubic lattices and…
Understanding how topological constraints affect the dynamics of polymers in solution is at the basis of any polymer theory and it is particularly needed for melts of rings. These polymers fold as crumpled and space-filling objects and,…
In the three-dimensional Heisenberg spin glass in a random field we study the properties of the inherent structures that are obtained by an instantaneous cooling from infinite temperature. For not too large field the density of states…
We study topology of frustration in $d$-dimensional Ising spin glasses with $d\ge 2$ with nearest-neighbor interactions. We prove the following: For any given spin configuration, the domain walls on the unfrustration network are all…
The transition of a fluid to a rigid glass upon cooling is a common route of transformation from liquid to solid that embodies the most poorly understood features of both phases1,2,3. From the liquid perspective, the puzzle is to understand…