Related papers: Tailored Raman-resonant four-wave-mixing process
We demonstrate an efficient nonlinear process in which Stokes and anti-Stokes components are generated spontaneously in a Raman-like, near resonant media driven by low power counter-propagating fields. Oscillation of this kind does not…
A quantum model of the Raman process with the independent Stokes and anti-Stokes nonlinear interactions is developed to study nonclassical correlations between the photons in the Stokes and anti-Stokes fields. The role of the laser pump…
Three-color coherent anti-Stokes Raman scattering represents non-degenerate four wave mixing process that includes both a non-resonant and resonant processes, the contributions of which depend on how the molecular vibrational modes are…
The nonlinear optical response of materials to exciting light is enhanced by resonances between the incident laser frequencies and the energy levels of the excited material. Traditionally, in molecular nonlinear spectroscopy one tunes the…
Coherent control with shaped ultrafast pulses is a powerful approach for steering nonlinear light-matter interactions. Previous studies in quantum control have shown that, beyond transform-limited pulses, those with antisymmetric spectral…
We experimentally demonstrate stimulated four-wave mixing in two linearly uncoupled integrated Si$_3$N$_4$ micro-resonators. In our structure the resonance combs of each resonator can be tuned independently, with the energy transfer from…
We investigate the quantum properties of fields generated by resonantly enhanced wave mixing based on atomic coherence in Raman systems. We show that such a process can be used for generation of pairs of Stokes and anti-Stokes fields with…
Phase matching is essential for efficient energy transfer in nonlinear wave-mixing processes. Traditional methods, such as birefringent and quasi-phase matching, have remained conceptually unchanged since their discovery over 60 years ago,…
Phase-mismatch in nonlinear optical processes can severely limit the propagation and conversion efficiency of light fields. Here, we present an efficient optimal-control strategy to mitigate the detrimental effects of phase-mismatch in an…
To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…
We show how analogues of a large number of well-known nonlinear-optics phenomena can be realized with one or more two-level atoms coupled to one or more resonator modes. Through higher-order processes, where virtual photons are created and…
A major impediment of using Coherent Anti-Stokes Raman Scattering to identify biological molecules is that the illumination levels required to produce a measurable signal often also produce significant nonresonant background from the…
Recent remarkable progress in wave-front shaping has enabled control of light propagation inside linear media to focus and image through scattering objects. In particular, light propagation in multimode fibers comprises complex intermodal…
We present a self-consistent quantum optics approach to calculating the surface enhanced Raman spectrum of molecules coupled to arbitrarily shaped plasmonic systems. Our treatment is intuitive to use and provides fresh analytical insight…
We investigate the evolution of coherence property of noise-seeded Stokes wave in short (< 1 ps) and long pulse (> 1 ps) regimes. Nonlinear equations expressing the evolution of pump and Stokes wave are solved numerically for both the…
We show that useful non-instantaneous nonlinear phase shifts can be obtained from cascaded quadratic processes in the presence of group velocity mismatch. The two-field nature of the process permits responses that can be effectively…
The extraordinary properties of resonant four-wave mixing of backward waves in doped negative-index materials are investigated. The feasibility of independent engineering of negative refractive index and nonlinear optical response as well…
The process in which Raman scattering produces correlated Stokes and anti-Stokes radiation is known as Stokes--anti-Stokes (SaS) scattering. It has been shown recently that this process can generate entangled photon pairs, making it a…
The four-wave mixing produced with two ultrashort phase-locked w-3w laser pulses propagating coherently in a two-level system in the infrared spectral region is shown to depend on the pulses relative phase. The Maxwell-Bloch equations are…
We derive phase-matching conditions for four-wave mixing between solitons and linear waves in optical fibres with arbitrary dispersion and demonstrate resonant excitation of new spectral components via this process.