English
Related papers

Related papers: Demonstrating that the non orthogonal orbital opti…

200 papers

Approximate full configuration interaction (FCI) calculations have recently become tractable for systems of unforeseen size thanks to stochastic and adaptive approximations to the exponentially scaling FCI problem. The result of an FCI…

Strongly Correlated Electrons · Physics 2017-10-25 Susi Lehtola , Norm M. Tubman , K. Birgitta Whaley , Martin Head-Gordon

Unitary Coupled Cluster (UCC) theory is a promising variational method for electronic structure calculations, especially for strongly correlated systems and quantum computers. However, its practical application is limited by the steep…

Chemical Physics · Physics 2026-02-05 Prateek Vaish , Brenda Rubenstein

The construction of a general effective lagrangian consistent with the symmetries of QCD and intended for applications to finite-density systems is discussed. The low-energy structure of the composite nucleon is described within the theory…

Nuclear Theory · Physics 2007-05-23 R. J. Furnstahl , Hua-Bin Tang

It is shown how to adapt the non-perturbative coupled cluster method of many-body theory so that it may be successfully applied to Hamiltonian lattice $SU(N)$ gauge theories. The procedure involves first writing the wavefunctions for the…

High Energy Physics - Lattice · Physics 2009-10-22 C. H. Llewellyn Smith , N. J. Watson

In truncated coupled-cluster (CC) theories, non-variational and/or generally complex ground-state energies can occur. This is due to the non-Hermitian nature of the similarity transformed Hamiltonian matrix in combination with CC…

Chemical Physics · Physics 2023-09-22 Tanner Culpitt , Erik I. Tellgren , Fabijan Pavosevic

Introducing an active space approximation is inevitable for the quantum computations of chemical systems. However, this approximation ignores the electron correlations related to non-active orbitals. Here, we propose a computational method…

Quantum Physics · Physics 2024-06-06 Luca Erhart , Yuichiro Yoshida , Viktor Khinevich , Wataru Mizukami

A previously proposed computational procedure for constructing a set of nonorthogonal strongly localised one-electron molecular orbitals (O. Danyliv, L. Kantorovich - physics/0401107) is applied to a perfect $\alpha$-quartz crystal…

Chemical Physics · Physics 2009-11-10 Oleh Danyliv , Lev Kantorovich

A unitary coupled-cluster (UCC) form for the wavefunction in the variational quantum eigensolver has been suggested as a systematic way to go beyond the mean-field approximation and include electron correlation in solving quantum chemistry…

Quantum Physics · Physics 2018-09-12 Ilya G. Ryabinkin , Tzu-Ching Yen , Scott N. Genin , Artur F. Izmaylov

We develop a biorthogonal linear-scaling algorithm for a transcorrelated method based on the localized nature of transformed orbitals. The transcorrelated method, which employs a similarity-transformed Hamiltonian referred to as a…

Strongly Correlated Electrons · Physics 2009-06-17 Masashi Kojo , Kikuji Hirose

The congruent transformation of the electronic Hamiltonian is developed to address the electron correlation problem in many-electron systems. The central strategy presented in this method is to perform transformation on the electronic…

Chemical Physics · Physics 2012-12-21 Jennifer M. Elward , Johannes Hoja , Arindam Chakraborty

We present a numerical implementation of the gauge-invariant time-dependent configuration interaction singles (TDCIS) method [Appl. Sci. 8, 433 (2018)] for three-dimensional atoms. In our implementation, orbital-like quantity called channel…

Atomic Physics · Physics 2019-10-09 Takuma Teramura , Takeshi Sato , Kenichi L. Ishikawa

We investigate the accuracy of a number of wavefunction based methods at the heart of quantum chemistry for metallic systems. Using Hartree-Fock as a reference, perturbative (M{\o}ller-Plesset, MP) and coupled cluster (CC) theories are used…

Chemical Physics · Physics 2013-10-24 James J. Shepherd , Andreas Grüneis

Non-unitary theories are commonly seen in the classical simulations of quantum systems. Among these theories, the method of moments of coupled-cluster equations (MMCCs) and the ensuing classes of the renormalized coupled-cluster (CC)…

Quantum Physics · Physics 2022-12-13 Bo Peng , Karol Kowalski

We derive a microscopic relativistic point-coupling model of nuclear many-body dynamics constrained by in-medium QCD sum rules and chiral symmetry. The effective Lagrangian is characterized by density dependent coupling strengths,…

Nuclear Theory · Physics 2009-11-10 P. Finelli , N. Kaiser , D. Vretenar , W. Weise

A Quark-Meson Coupling (QMC) model is extended to finite nuclei in the relativistic mean-field or Hartree approximation. The ultra-relativistic quarks are assumed to be bound in non-overlapping nucleon bags, and the interaction between…

Nuclear Theory · Physics 2008-11-26 Peter G. Blunden , Gerald A. Miller

These lecture notes address a central problem of theoretical nuclear physics: how to establish a relationship between low-energy, non-perturbative QCD and nuclear phenomenology which includes both nuclear matter and finite nuclei. We…

Nuclear Theory · Physics 2017-01-25 Dario Vretenar , Wolfram Weise

We present a wide-reaching revamp of the generalized many-body expanded full configuration interaction (MBE-FCI) method. First, we outline how to automatize the selection of reference active spaces whereby the inherent bias introduced…

Chemical Physics · Physics 2024-06-18 Jonas Greiner , Jürgen Gauss , Janus J. Eriksen

The configuration interaction relativistic Hartree-Fock (CI-RHF) model is developed in this work. Compared to the conventional configuration interaction shell model (CISM), the CI-RHF model can be applied to study the structural properties…

Nuclear Theory · Physics 2025-04-14 Jia Liu , Yi Fei Niu , Wen Hui Long

The convergence of no-core shell model (NCSM) calculations using renormalization group evolved low-momentum two-nucleon interactions is studied for light nuclei up to Li-7. Because no additional transformation was used in applying the NCSM…

Nuclear Theory · Physics 2008-11-26 S. K. Bogner , R. J. Furnstahl , P. Maris , R. J. Perry , A. Schwenk , J. P. Vary

The variational method and the Hamiltonian formalism of QCD are used to derive relativistic, momentum space integral equations for a quark-antiquark system with an arbitrary number of gluons present. As a first step, the resulting infinite…

High Energy Physics - Phenomenology · Physics 2009-10-31 L. Di Leo , J. W. Darewych