Related papers: Continuous regional trace gas source attribution u…
Continuous monitoring of oil and gas infrastructure is of interest for improving emissions and safety by enabling rapid identification and repair of emission sources, especially large sources that are responsible for the bulk of total…
We demonstrate coherent dual frequency-comb spectroscopy for detecting variations in greenhouse gases. High signal-to-noise spectra are acquired spanning 5990 to 6260 cm^-1 (1600 to 1670 nm) covering ~700 absorption features from CO2, CH4,…
Open-path dual-comb spectroscopy provides multi-species atmospheric gas concentration measurements with high precision. Here, we extend open-path dual comb spectroscopy to the mid-infrared 5 {\mu}m atmospheric window, enabling atmospheric…
Cavity-enhanced direct frequency comb spectroscopy (CE-DFCS) has demonstrated powerful potential for trace gas detection based on its unique combination of high bandwidth, rapid data acquisition, high sensitivity, and high resolution, which…
Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…
Advances in mid-infrared (MIR) dual-comb spectroscopy (DCS) have significantly enhanced molecular detection in recent years. The capability of DCS to precisely identify and quantify atmospheric trace gases makes it attractive for field…
We describe a method for detecting, locating and quantifying sources of gas emissions to the atmosphere using remotely obtained gas concentration data; the method is applicable to gases of environmental concern. We demonstrate its…
Open-path dual-comb spectroscopy (DCS) significantly enhances our understanding of regional trace gases. However, due to technical challenges, cost considerations, and eye-safety regulations, its sensing range and flexibility remain…
We present gapless, high-resolution absorption and dispersion spectra obtained with quantum cascade laser frequency combs covering 55 cm$^{-1}$. Using phase-sensitive dual comb design, the comb lines are gradually swept over 10 GHz,…
Dual-frequency comb spectroscopy has emerged as a disruptive technique for measuring wide-spanning spectra with high resolution, yielding a particularly powerful technique for sensitive multi-component gas analysis. We present a…
The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…
Providing an accurate, representative sample of mass flux across large open areas for atmospheric studies or the extreme conditions of a hypersonic engine is challenging for traditional intrusive or point-based sensors. Here, we demonstrate…
Frequency combs, broadband light sources whose spectra consist of coherent, discrete modes, have become essential in many fields. Miniaturizing frequency combs would be a significant advance in these fields, enabling the deployment of…
This work presents a procedure that can quickly identify and isolate methane emission sources leading to expedient remediation. Minimizing the time required to identify a leak and the subsequent time to dispatch repair crews can…
A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…
The article addresses the possibility of robust detection of geometrically small, low emission sources on a significantly stronger background. This problem is important for homeland security. A technique of detecting such sources using…
Satellite-based greenhouse gases (GHG) sensing technologies play a critical role in the study of global carbon emissions and climate change. However, none of the existing satellite-based GHG sensing technologies can achieve the measurement…
Frequency combs, spectra of evenly-spaced narrow phase-coherent laser lines, have revolutionized precision measurements. On-chip frequency comb generators hold much promise for fully-integrated instruments of time and frequency metrology.…
Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…
Recent findings suggest that abnormal operating conditions of equipment in the oil and gas supply chain represent a large fraction of anthropogenic methane emissions. Thus, effective mitigation of emissions necessitates rapid identification…