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The variational inclusion of spin-orbit coupling in self-consistent field (SCF) calculations requires a generalised two-component framework, which permits the single-determinant wave function to completely break spin symmetry. The…

Chemical Physics · Physics 2023-03-29 Shadan Ghassemi Tabrizi , R. Rodríguez-Guzmán , Carlos A. Jiménez-Hoyos

Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…

Strongly Correlated Electrons · Physics 2012-02-02 S. S. Sosin , A. I. Smirnov , L. A. Prozorova , G. Balakrishnan , M. E. Zhitomirsky

Electron spin resonance (ESR) is usually interpreted as a single-particle phenomenon protected from the effect of many-body correlations. We show that this is not the case in a two-dimensional Fermi liquid (FL) with spin-orbit coupling…

Mesoscale and Nanoscale Physics · Physics 2016-02-17 Saurabh Maiti , Muhammad Imran , Dmitrii L. Maslov

We used electron spin resonance (ESR) combined with scanning tunneling microscopy (STM) to measure hydrogenated Ti (spin-1/2) atoms at low-symmetry binding sites on MgO in vector magnetic fields. We found strongly anisotropic g-values in…

The magnetic resonance spectrum of spin clusters formed in spin-Peierls magnets in the vicinity of impurity ions was investigated. The observed temperature dependences of the effective g-factor and the linewidth of the electron spin…

Strongly Correlated Electrons · Physics 2009-11-07 V. N. Glazkov , A. I. Smirnov , R. M. Eremina , G. Dhalenne , A. Revcolevschi

Electron paramagnetic resonance (EPR) spectroscopy interrogates unpaired electron spins in solids and liquids to reveal local structure and dynamics; for example, EPR has elucidated parts of the structure of protein complexes that have…

Other Condensed Matter · Physics 2012-05-08 S. Takahashi , L. -C. Brunel , D. T. Edwards , J. van Tol , G. Ramian , S. Han , M. S. Sherwin

Energy levels and electromagnetic properties of with $N=28\sim 30$ nuclides are studied in terms of a large-scale shell model calculation, which contains no newly adjusted parameters. The Kuo-Brown $G$-matrix interaction is shown to…

Nuclear Theory · Physics 2015-06-26 Hitoshi Nakada , Takashi Sebe , Takaharu Otsuka

ESR of the pure monocrystals of CuGeO3 is studied in the frequency range 9-75 GHz and in the temperature interval 1.2-25 K. The splitting of the ESR line into several spectral components is observed below 5 K, in the temperature range where…

Strongly Correlated Electrons · Physics 2009-10-31 A. I. Smirnov , V. N. Glazkov , L. I. Leonyuk , A. G. Vetkin , R. M. Eremina

The accurate electronic structure calculation for strongly correlated chemical systems requires an adequate description for both static and dynamic electron correlation, and is a persistent challenge for quantum chemistry. In order to…

Strongly Correlated Electrons · Physics 2020-08-18 Yinxuan Song , Yifan Cheng , Yingjin Ma , Haibo Ma

We construct a microscopic model for f-electron systems, composed of f-electron hopping, Coulomb interaction, and crystalline electric field (CEF) terms. In order to clarify the meaning of one f-electron state, here the j-j coupling scheme…

Strongly Correlated Electrons · Physics 2009-11-07 Takashi Hotta , Kazuo Ueda

The impurity-induced antiferromagnetic ordering of the doped Haldane magnet Pb(Ni{1-x}Mg{x})2V2O8 (0 < x <0.06) was studied by electron spin resonance (ESR) on ceramic samples in the frequency range 9-110 GHz. Below the N\'{e}el temperature…

Strongly Correlated Electrons · Physics 2009-11-07 A. I. Smirnov , V. N. Glazkov , H. -A. Krug von Nidda , A. Loidl , L. N. Demianets , A. Ya. Shapiro

The spin dynamics of the ferromagnetic Kondo lattice CeRuPO is investigated by Electron Spin Resonance (ESR) at microwave frequencies of 1, 9.4, and 34~GHz. The measured resonance can be ascribed to a rarely observed bulk Ce3+ resonance in…

Strongly Correlated Electrons · Physics 2010-10-13 T. Förster , J. Sichelschmidt , C. Krellner , C. Geibel , F. Steglich

Fe3+ ions in sapphire exhibit an Electron Spin Resonance (ESR) which interacts strongly with high-Q Whispering Gallery (WG) modes at microwave frequencies. We report the first observation of a third-order paramagnetic nonlinear…

Quantum Physics · Physics 2012-03-02 Daniel L. Creedon , Karim Benmessai , Warwick P. Bowen , Michael E. Tobar

An interacting spin system is an excellent testbed for fundamental quantum physics and applications in quantum sensing and quantum simulation. For these investigations, detailed information of the interactions, e.g., the number of spins and…

Quantum Physics · Physics 2024-11-12 Yuhang Ren , Susumu Takahashi

Electron spin resonance and magnetization data in magnetic fields up to 55 T of a novel multicenter paramagnetic molecular complex [L_2Ni_4(N_3)(O_2C Ada)_4](Cl O_4) are reported. In this compound, four Ni centers each having a spin S = 1…

We propose a new universal mechanism that makes it possible to drive an individual atomic spin using a spin polarized scanning tunnel microscope (STM) with an oscillating electric signal. We show that the combination of the distance…

Mesoscale and Nanoscale Physics · Physics 2017-11-15 J. L. Lado , A. Ferron , J. Fernandez-Rossier

A new method of computing multipolar exchange interaction in spin-orbit coupled systems is developed using multipolar tensor expansion of the density matrix in LDA+U electronic structure calculation. Within mean-field approximation,…

Strongly Correlated Electrons · Physics 2014-03-06 Shu-Ting Pi , Ravindra Nanguneri , Sergey Savrasov

Dynamical spin susceptibility is calculated for the generalized ferromagnetic Kondo model which describes itinerant $e_{g}$ electrons interacting with localized $t_{2g}$ electrons with antiferromagnetic coupling. The calculations done in…

Strongly Correlated Electrons · Physics 2016-08-31 N. B. Perkins , N. M. Plakida

We report the nanoscale spin detection and electron paramagnetic resonance (EPR) spectrum of copper (Cu$^{2+}$) ions via double electron-electron resonance with single spins in diamond at room temperature and low magnetic fields. We measure…

Quantum Physics · Physics 2022-01-06 Kai Zhang , Shreya Ghosh , Sunil Saxena , M. V. Gurudev Dutt

In this paper we use the Nuclear Magnetic Resonance (NMR) to write eletronic states of a ferromagnetic system into a high-temperature paramagnetic nuclear spins. Through the control of phase and duration of radiofrequency pulses we set the…