Related papers: Superhyperfine interactions in Ce3+ doped LiYF4 cr…
While electron microscopy offers crucial atomic-resolution insights into structure-property relationships, radiation damage severely limits its use on beam-sensitive materials like proteins and 2D materials. To overcome this challenge, we…
High-field electron spin resonance (ESR) experiments have been carried out in single crystals of La_{1-x}Sr_xMnO_3 in the concentration range 0 \le x \le 0.175. Different quasioptical arrangements have been utilized in the frequency range…
Electron spin resonance (ESR) experiments were performed with antiferromagnetic MnO confined within a porous vycor-type glass and within MCM-type channel matrices. A signal from confined MnO shows two components from crystallized and…
High resolution low-temperature absorption spectra of 0.2% Pr^3+ doped CsCdBr_3 were measured in the spectral region 2000--7000 cm-1. Positions and widths of the crystal field levels within the 3H5, 3H4, 3F2, and 3F3 multiplets of the Pr^3+…
Exotic spin-multipolar ordering in spin transition metal insulators has so far eluded unambiguous experimental observation. A less studied, but perhaps more feasible fingerprint of multipole character emerges in the excitation spectrum in…
The research investigates coherent interactions between sub-GeV electrons and oriented scintillator crystals, leading to enhanced electromagnetic (EM) radiation. Experiments at Mainz Mikrotron (MAMI) involved PWO, BGO, and CsI crystals…
For coherent electron spins, hyperfine coupling to nuclei in the host material can either be a dominant source of unwanted spin decoherence or, if controlled effectively, a resource allowing storage and retrieval of quantum information. To…
Improved values of hyperfine coefficients related to the electronic spin-orbit and electron-nucleus spin-spin tensor interactions in the HD$^+$ molecular ion are obtained through numerical calculation of relativistic corrections at the…
The results of studies of Y$_{2}$Ti$_2$O$_7$ single crystals doped with Er$^{3+}$ and Yb$^{3+}$ ions by means of electron paramagnetic resonance (EPR) and dc-magnetometry are reported. EPR signals of the trigonal centers with the…
Quantum memories are integral parts of both quantum computers and quantum communication networks. Naturally, such a memory is embedded into a hybrid quantum architecture, which has to meet the requirements of fast gates, long coherence…
The hyperfine interactions at the uranium site in the antiferromagnetic USb2 compound were calculated within the density functional theory (DFT) employing the augmented plane wave plus local orbital (APW+lo) method. We investigated the…
Erbium-doped crystals offer a versatile platform for hybrid quantum devices because they combine magnetically-sensitive electron-spin transitions with telecom-wavelength optical transitions. At the high doping concentrations necessary for…
Single-spin magnetic resonance spectroscopy promises to yield structural and chemical information at the level of individual atoms or molecules, in a non-invasive way. Here, we use an Er3+ paramagnetic center in a CaWO4 crystal, detected by…
We use complementary optical spectroscopy methods to directly measure the lowest crystal-field energies of the rare-earth quantum magnet LiY$_{1-x}$Ho$_{x}$F$_{4}$, including their hyperfine splittings, with more than 10 times higher…
Interfacing superconducting quantum processors, working in the GHz frequency range, with optical quantum networks and atomic qubits is a challenging task for the implementation of distributed quantum information processing as well as for…
We report sensitive detection of the nuclear quadrupolar interaction of the 14N nuclear spin of the nitrogen-vacancy (NV) center using the electron spin echo envelope modulation technique. We applied a weak transverse magnetic field to the…
We investigate the magnetic and crystal electric field (CEF) states of the Kondo lattice system CeCuGa3 by muon spin relaxation (muSR), neutron diffraction, and inelastic neutron scattering (INS) measurements. A noncentrosymmetric…
We experimentally demonstrate an approach to scale up quantum devices by harnessing spin defects in the environment of a quantum probe. We follow this approach to identify, locate, and control two electron-nuclear spin defects in the…
In Er$^{3+}$:Y$_2$SiO$_5$, we demonstrate the selective optical addressing of the $^{89}$Y$^{3+}$ nuclear spins through their superhyperfine coupling with the Er$^{3+}$ electronic spins possessing large Land\'e $g$-factors. We…
Rare earth doped crystals are promising systems for quantum information processing. In particular paramagnetic rare earths could be used to build coherent interfaces with optical and microwave photons. In addition, isotopes with non zero…