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The $4f-5d$ transition rates for rare-earth ions in crystals can be calculated with an effective transition operator acting between model $4f^N$ and $4f^{N-1}5d$ states calculated with effective Hamiltonian, such as semi-empirical crystal…

Materials Science · Physics 2007-05-23 Chang-Kui Duan , Michael F. Reid

Ca$_3$Ru$_2$O$_7$ undergoes an antiferromagnetic transition at $T_{\text{N}}=56 $K, followed by a Mott-like (MI) transition at $T_{\text{MI}}=48$ K. This nonmetallic ground state, with a charge gap of 0.1 eV, is suppressed by a highly…

Strongly Correlated Electrons · Physics 2007-05-23 G. Cao , L. Balicas , Y. Xin , E. Dagotto , J. E. Crow , C. S. Nelson , J. P. Hill

Transition frequencies between low-lying energy levels in a single trapped $^{138}$Ba$^{+}$ ion have been measured with laser spectroscopy referenced to an optical frequency comb. By extracting the frequencies of one-photon and two-photon…

Atomic Physics · Physics 2016-01-29 E. A. Dijck , M. Nuñez Portela , A. T. Grier , K. Jungmann , A. Mohanty , N. Valappol , L. Willmann

We report the detection of the 1_{10}-1_{11} ground state transition of ortho-H_2D^+ at 372.421 GHz in emission from the young stellar object NGC 1333 IRAS 4A. Detailed excitation models with a power-law temperature and density structure…

Astrophysics · Physics 2009-10-31 Ronald Stark , Floris F. S. van der Tak , Ewine F. van Dishoeck

We report a precise measurement of the isotope shifts in the $4^2$S$_{1/2} \rightarrow 3^2$D$_{5/2}$ electric quadrupole transition at 729~nm in the $^{40 - 42,44,48}$Ca$^+$. The measurement has been made via high-resolution laser…

Atomic Physics · Physics 2023-05-24 Felix W. Knollmann , Ashay N. Patel , S. Charles Doret

The magnetic-dipole transition probabilities between the fine-structure levels (1s^2 2s^2 2p) ^2P_1/2 - ^2P_3/2 for B-like ions and (1s^2 2s 2p) ^3P_1 - ^3P_2 for Be-like ions are calculated. The configuration-interaction method in the…

Lanthanides in the trivalent oxidation state are typically described using an ionic picture that leads to localized magnetic moments. The hierarchical energy scales associated with trivalent lanthanides produce desirable properties for…

The increased spectral resolution allowed by the use of extremely thin vapor cells has led to the observation of interesting behaviour of alkali transitions when placed in a magnetic field. Particularly, transitions obeying an apparent…

Atomic Physics · Physics 2022-04-06 Armen Sargsyan , Arevik Amiryan , Ara Tonoyan , Emmanuel Klinger , David Sarkisyan

Magnetic field-induced giant modification of probabilities for seven components of 6S1/2 (Fg=3) - 6P3/2 (Fe=5) transition of Cs D2 line forbidden by selection rules is observed experimentally for the first time. For the case of excitation…

Atomic Physics · Physics 2015-06-18 A. Sargsyan , A. Tonoyan , G. Hakhumyan , A. Papoyan , E. Mariotti , D. Sarkisyan

The 3D ternary Li$_2$GeO$_3$ compound, which could serve as the electrolyte material in Li+-based batteries, exhibits an unusual lattice symmetry (orthorhombic crystal), band structure, charge density distribution and density of states. The…

LiV_2 O_4 is one of the most puzzling compounds among transition metal oxides because of its heavy fermion like behavior at low temperatures. In this paper we present results for the orbital state and magnetic properties of LiV_2 O_4…

Strongly Correlated Electrons · Physics 2009-11-07 I. A. Nekrasov , Z. V. Pchelkina , G. Keller , Th. Pruschke , K. Held , A. Krimmel , D. Vollhardt , V. I. Anisimov

We report on the magnetic properties of HoCo dimers as a model system for the smallest intermetallic transition metal-lanthanide compound. The dimers are adsorbed on ultrathin MgO(100) films grown on Ag(100). New for $4f$ elements, we…

Atomic and Molecular Clusters · Physics 2018-12-26 A. Singha , F. Donati , F. D. Natterer , C. Wäckerlin , S. Stavrić , Z. S. Popović , {Ž}. {Š}ljivan{č}anin , F. Patthey , H. Brune

The dynamic polarizabilities of the atomic states with angular momentum $j> \frac12$ are sensitive to the angle between the quantization axis $\hat{e}_z$ and the polarization vector $\hat{\mathbf{\epsilon}}$ owing to the contribution of…

Atomic Physics · Physics 2019-03-27 Jun Jiang , Li Jiang , Z. W. Wu , Deng-Hong Zhang , Lu-You Xie , Chen-Zhong Dong

Many-body perturbation theory in the GW approach is applied to lanthanide oxides, using the local-density approximation plus a Hubbard U correction (LDA+U) as the starting point. Good agreement between the G0W0 density of states and…

Materials Science · Physics 2009-11-13 Hong Jiang , Ricardo I. Gomez-Abal , Patrick Rinke , Matthias Scheffler

The visible spectrum of Mo$^{15+}$ ions was measured using a high-temperature superconducting electron-beam ion trap at the Shanghai EBIT Laboratory, with an electron beam energy $E_{e}$=400 eV, significantly lower than the ionization…

Atomic Physics · Physics 2025-04-21 Cunqiang Wu , Xiaobin Ding , Qi Guo , Ke Yao , Jialin Liu , Yunqing Fu , Chenzhong Dong

We present a theoretical model of the "isostructural" \gamma-\alpha phase transition in Ce which is based on quadrupolar interactions due to coupled charge density fluctuations of 4f electrons and of conduction electrons. Conduction…

Strongly Correlated Electrons · Physics 2009-10-31 A. V. Nikolaev , K. H. Michel

The appropriateness of including Hg among the transition metals has been debated for a long time. Although the synthesis of HgF$_{4}$ molecules in gas phase was reported before, the molecules show strong instabilities and dissociate.…

Materials Science · Physics 2012-06-14 Xiaoli Wang , Haiqing Lin , Yanming Ma , Mao-Sheng Miao

We report measurements and theoretical calculations of the fine-structure splittings in all three $1s2s\,^3\!S_1\rightarrow\,1s2p\,^3\!P_{0,1,2}$ transitions in the heliumlike systems of the isotopes $^{12,13,14}$C. The metastable triplet…

As an important step towards an atomic parity violation experiment in one single trapped Ra$^+$ ion, laser spectroscopy experiments were performed with on-line produced short-lived $^{212,213,214}$Ra$^+$ ions. The isotope shift of the…

The goals of this study are 1) to test the best theoretical transition probabilities for Ca I (a relatively light alkaline earth spectrum) from a modern ab initio calculation using configuration interaction plus many body perturbation…

Solar and Stellar Astrophysics · Physics 2021-08-18 E. A. Den Hartog , J. E. Lawler , C. Sneden , J. J. Cowan , I. U. Roederer , J. Sobeck