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We investigate the physical mechanisms for spin-dependent recombination of a strongly bound pair of triplet excitons generated by singlet fission and forming a spin quintet (total spin of two) bi-exciton. For triplet excitons the…

Mesoscale and Nanoscale Physics · Physics 2024-02-16 Yan Sun , L. R. Weiss , V. Derkach , J. E. Anthony , M. Monteverde , A. D. Chepelianskii

We present a practical semiclassical method for computing the electron spin dynamics of a radical in which the electron spin is hyperfine coupled to a large number of nuclear spins. This can be used to calculate the singlet and triplet…

Chemical Physics · Physics 2014-07-09 David E. Manolopoulos , P. J. Hore

The effect of exchange interactions within spin pairs on spin-dependent transport and recombination rates through localized states in semiconductors during coherent electron spin resonant excitation is studied theoretically. It is shown…

Materials Science · Physics 2008-01-09 A. Gliesche , C. Michel , V. Rajevac , K. Lips , S. D. Baranovskii , F. Gebhard , C. Boehme

It is shown that coherent spin motion of electron-hole pairs localized in band gap states of silicon can influence charge carrier recombination. Based on this effect, a readout concept for silicon based solid-state spin--quantum computers…

Quantum Physics · Physics 2007-05-23 Christoph Boehme , Klaus Lips

The recombination of electron-hole pairs injected in extended conjugated systems is modeled as a multi-pathway vibron-driven relaxation in monoexcited state-space. The computed triplet-to-singlet ratio of exciton formation times $r =…

Materials Science · Physics 2009-11-07 Stoyan Karabunarliev , Eric. R. Bittner

We present a theoretical study of optical electron-spin orientation and spin-dependent Shockley-Read-Hall recombination taking into account the hyperfine coupling between the bound-electron spin and the nuclear spin of a deep paramagnetic…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 E. L. Ivchenko , L. A. Bakaleinikov , V. K. Kalevich

We address the problem of relative frequencies of singlet and triplet recombinations in a multiparticle system, which consists of spin-correlated radical ion pairs. The nonlocal swapping of spin correlations due to cross-recombinations is…

Quantum Physics · Physics 2009-03-04 L. V. Il'ichov , S. V. Anishchik

We study theoretically the recombination within a pair of two polarons in magnetic field subject to a strong linearly polarized ac drive. Strong drive implies that the Zeeman frequencies of the pair-partners are much smaller than the Rabi…

Mesoscale and Nanoscale Physics · Physics 2017-10-11 R. K. Malla , M. E. Raikh

In this paper we outline a physically motivated framework for describing spin-selective recombination processes in chiral systems, from which we derive spin-selective reaction operators for recombination reactions of donor-bridge-acceptor…

Chemical Physics · Physics 2023-03-09 Thomas P. Fay , David T. Limmer

We theoretically study the $(1,1)$ triplet to $(0,2)$ singlet relaxation rate in a lateral gate-defined double quantum dot tuned to the regime of Pauli spin blockade. We present a detailed derivation of the effective phonon density of…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 J. Danon

The standard quantum mechanical expressions for the singlet and triplet survival probabilities and product yields of a radical pair recombination reaction involve a trace over the states in a combined electronic and nuclear spin Hilbert…

Chemical Physics · Physics 2017-01-02 Alan M. Lewis , Thomas P. Fay , David E. Manolopoulos

We investigate static charge and spin density modulation patterns along a ferromagnet/semiconductor single junction quantum wire in the presence of spin-orbit coupling. Coherent scattering theory is used to calculate the charge and spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Minchul Lee , Christoph Bruder

A spin-charge recombination route to superconductivity, proposed earlier (1992)], is examined using the Schwinger boson representation of the t-J model. The representation is known to work well at half-filling. It was shown in the earlier…

Condensed Matter · Physics 2007-05-23 Sanjoy K. Sarker

Charge separation from the $(4,0)$ to the $(3,1)$ state in a Si/SiGe double quantum dot is commonly used for initialization of spin qubits and Pauli-spin-blockade readout. It was used in recent experiments involving creation of the $(3,1)$…

Mesoscale and Nanoscale Physics · Physics 2026-04-28 Łukasz Cywiński , Mats Volmer , Tom Struck , Giordano Scappucci , Lars R. Schreiber

Spin-dependent processes play a crucial role in organic electronic devices. Spin coherence can give rise to spin mixing due to a number of processes such as hyperfine coupling, and leads to a range of magnetic field effects. However, it is…

Mesoscale and Nanoscale Physics · Physics 2016-09-07 Marzieh Kavand , Douglas Baird , Kipp van Schooten , Hans Malissa , John M. Lupton , Christoph Boehme

The unique properties of organic semiconductors make them versatile base materials for many applications ranging from light emitting diodes to transistors. The low spin-orbit coupling typical for carbon-based materials and the resulting…

We describe how the semiclassical theory of radical pair recombination reactions recently introduced by two of us [D. E. Manolopoulos and P. J. Hore, J. Chem. Phys. 139, 124106 (2013)] can be generalised to allow for different singlet and…

Chemical Physics · Physics 2014-07-28 Alan M. Lewis , David E. Manolopoulos , P. J. Hore

We have evaluated hyperfine-induced electron spin dynamics for two electrons confined to a double quantum dot. Our quantum solution accounts for decay of a singlet-triplet correlator even in the presence of a fully static nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 W. A. Coish , Daniel Loss

Low-field (6-110 mT) magnetic resonance of bismuth (Bi) donors in silicon has been observed by monitoring the change in photoconductivity induced by spin dependent recombination. The spectra at various resonance frequencies show signal…

Materials Science · Physics 2012-10-10 P. A. Mortemousque , T. Sekiguchi , C. Culan , M. P. Vlasenko , R. G. Elliman , L. S. Vlasenko , K. M. Itoh

Recently, graphene triangulene chains have been synthesized and their magnetic response has been analyzed by STM methods by Mishra and coworkers (Nature 598, 287 (2021)). Motivated by this study, we determine the exchange bilinear and…

Mesoscale and Nanoscale Physics · Physics 2023-02-17 Gabriel Martínez-Carracedo , László Oroszlány , Amador García-Fuente , László Szunyogh , Jaime Ferrer
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