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Single linear polymer chains in dilute solutions under good solvent conditions are studied by Monte Carlo simulations with the pruned-enriched Rosenbluth method up to the chain length $N \sim {\cal O}(10^4)$. Based on the standard simple…

Soft Condensed Matter · Physics 2015-06-24 Hsiao-Ping Hsu

Polymers are an effective test-bed for studying topological constraints in condensed matter due to a wide array of synthetically-available chain topologies. When linear and ring polymers are blended together, emergent rheological properties…

Soft Condensed Matter · Physics 2024-04-25 Daniel L. Vigil , Ting Ge , Michael Rubinstein , Thomas C. O'Connor , Gary S. Grest

The miscibility of polymer blends, a classical problem in polymer science, may be altered, if one or both of the component do not have chain ends. Based on the idea of {\it topological volume}, we propose a mean-field theory to clarify how…

Soft Condensed Matter · Physics 2016-05-04 Takahiro Sakaue , Chihiro H. Nakajima

Spontaneous formation of knots in long polymers at equilibrium is inevitable but becomes rare in sufficiently short chains. Here, we show that knotting and knot complexity increase by orders of magnitude in diblock polymers with a fraction…

Soft Condensed Matter · Physics 2024-07-11 Marin Vatin , Enzo Orlandini , Emanuele Locatelli

Scaling arguments are used to analyze the size of topologically constrained closed ring polymer with excluded volume. It is found that there exists a finite range of polymer thickness (excluded volume) in which self-avoidance is unimportant…

Soft Condensed Matter · Physics 2007-05-23 A. Yu. Grosberg

We investigate conformations and dynamics of a polymer considering its monomers to be active Brownian particles. This active polymer shows very intriguing physical behavior which is absent in an active Rouse chain. The chain initially…

Soft Condensed Matter · Physics 2020-04-13 Shalabh K. Anand , Sunil P. Singh

Topological entanglements are abundant, and often detrimental, in polymeric systems in biology and materials science. Here we theoretically investigate the topological simplification of knots by diffusing slip-links (SLs), which may…

Soft Condensed Matter · Physics 2020-11-02 Andrea Bonato , Davide Marenduzzo , Davide Michieletto

In this paper we investigate the problem of a long self-avoiding polymer chain immersed in a random medium. We find that in the limit of a very long chain and when the self-avoiding interaction is weak, the conformation of the chain…

Disordered Systems and Neural Networks · Physics 2009-11-07 Yadin Y. Goldschmidt , Yohannes Shiferaw

The conformational and electronic properties of conducting flexible random and self-avoiding walk polymer chains are under investigation. A Hamiltonian for conjugated flexible polymers is introduced and its physical consequences are…

Condensed Matter · Physics 2009-10-22 M. Otto , T. A. Vilgis

In this work we investigate the dynamics of random walk processes on scale-free networks in a short to moderate time scale. We perform extensive simulations for the calculation of the mean squared displacement, the network coverage and the…

Disordered Systems and Neural Networks · Physics 2009-11-10 Lazaros K. Gallos

We propose new polymer models for Monte Carlo simulation and apply them to a polymer chain confined in a relatively thin box which has both curved and flat sides, and show that either an ideal or an excluded-volume chain spends more time in…

Soft Condensed Matter · Physics 2007-05-23 Y. Y. Suzuki , T. Dotera , M. Hirabayashi

We investigate mutual local chain order in systems of fully flexible polymer melts in a simple generic bead-spring model. The excluded-volume interaction together with the connectivity leads to local ordering effects which are independent…

Soft Condensed Matter · Physics 2015-06-25 Roland Faller , Mathias Puetz , Florian Mueller-Plathe

Polymer entanglements lead to complicated topological constraints and interactions between neighbouring chains in a dense solution or melt. Entanglements can be treated in a mean field approach, within the famous reptation model, since they…

Soft Condensed Matter · Physics 2007-05-23 S. Kutter , E. M. Terentjev

We study the large-scale dynamics of event chain Monte Carlo algorithms in one dimension, and their relation to the true self-avoiding walk. In particular, we study the influence of stress, and different forms of interaction on the…

Computational Physics · Physics 2024-10-14 A. C. Maggs

We consider a fully directed self-avoiding walk model on a cubic lattice to mimic the conformations of an infinitely long confined flexible polymer chain; and the confinement condition is achieved by two parallel athermal plates. The…

Soft Condensed Matter · Physics 2021-06-21 P K Mishra

The study of the effect of random impurities on the collapse of a flexible polymer in dilute solution has had recent attention with consideration of semi-stiff interacting self-avoiding walks on the square lattice. In the absence of…

Statistical Mechanics · Physics 2022-07-20 C. J. Bradly , A. L. Owczarek

Primitive path analyses of entanglements are performed over a wide range of chain lengths for both bead spring and atomistic polyethylene polymer melts. Estimators for the entanglement length N_e which operate on results for a single chain…

Soft Condensed Matter · Physics 2015-05-13 Robert S. Hoy , Katerina Foteinopoulou , Martin Kröger

We use a bath of chaotic surface waves in water to mechanically and macroscopically mimic the thermal behavior of a short articulated chain with only nearest-neighbor interactions. The chaotic waves provide isotropic and random agitation to…

Soft Condensed Matter · Physics 2015-03-05 Kyle J. Welch , Clayton S. G. Kilmer , Eric I. Corwin

The mechanical properties of polymer knots under stretching in a bad or good solvent are investigated by applying a given force $F$ to a point of the knot while keeping another point fixed. The Monte Carlo sampling of the polymer…

Soft Condensed Matter · Physics 2015-12-15 Yani Zhao , Franco Ferrari

Large scale molecular dynamics simulations on graphic processing units (GPUs) are employed to study the scaling behavior of ring polymers with various topological constraints in melts. Typical sizes of rings containing $3_1$, $5_1$ knots…

Soft Condensed Matter · Physics 2015-09-04 Benjamin Trefz , Peter Virnau
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