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The functional properties of transition metal perovskite oxides are known to result from a complex interplay of magnetism, polarization, strain, and stoichiometry. Here, we show that for materials with a cooperative Jahn-Teller distortion,…

Materials Science · Physics 2021-01-04 Chiara Ricca , Nicolas Niederhauser , Ulrich Aschauer

We use density-functional theory with the local-density approximation to study the structural and ferroelectric properties of SrTiO$_3$ under misfit strains. Both the antiferrodistortive (AFD) and ferroelectric (FE) instabilities are…

Materials Science · Physics 2009-11-11 Chien-Hung Lin , Chih-Meng Huang , G. Y. Guo

Recent years have seen tremendous progress in experimental techniques to create uniaxial strain. Motivated by these advances we investigate the effect of uniaxial strain on LaMnO$_3$ employing ab-initio dynamical mean-field theory, and put…

Strongly Correlated Electrons · Physics 2024-02-23 Florian P. Lindner , Markus Aichhorn , Hrishit Banerjee

We use first principles density functional theory calculations to investigate the effect of biaxial strain in the low-temperature structural and ferroelectric properties of [111]-oriented SrTiO$_3$. We find that [111] biaxial strain,…

Materials Science · Physics 2019-03-27 Sebastian E. Reyes-Lillo , Karin M. Rabe , Jeffrey B. Neaton

The interaction of coexisting structural instabilities in multiferroic materials gives rise to intriguing coupling phenomena and extraordinarily rich phase diagrams, both in bulk materials and strained thin films. Here we investigate the…

BaBiO3 is a material where formally Bi4+ ions with the half-filled 6s-states form the alternating set of Bi3+ and Bi5+ ions resulting in a charge ordered insulator. The charge ordering is accompanied by the breathing distortion of the BiO6…

Strongly Correlated Electrons · Physics 2012-09-28 Dm. Korotin , V. Kukolev , A. V. Kozhevnikov , D. Novoselov , V. I. Anisimov

First principles calculations are used to investigate the effects of epitaxial strain on the structure of the perovskite oxide CaTiO$_3$, with particular focus on the stabilization of a ferroelectric phase related to a polar instability…

Materials Science · Physics 2013-05-29 C. -J. Eklund , C. J. Fennie , K. M. Rabe

The Jahn-Teller effect refers to the symmetry-lowering geometrical distortion in a crystal (or non-linear molecule) due to the presence of a degenerate electronic state. Usually, the Jahn-Teller distortion is not polar. Recently, GaV4S8…

Materials Science · Physics 2015-10-28 Ke Xu , H. J. Xiang

High-pressure optical-absorption measurements performed in CuWO4 up to 20 GPa provide experimental evidence of the persistence of the Jahn-Teller (JT) distortion in the whole pressure range both in the low-pressure triclinic and in the…

Materials Science · Physics 2012-04-20 J. Ruiz-Fuertes , A. Segura , F. Rodriguez , D. Errandonea , M. N. Sanz-Ortiz

Jahn-Teller (JT) electron-phonon coupling effects in the colossal magnetoresistance perovskite compounds $La_{1-x}A_xMnO_3$ are investigated. Electron-electron correlations between two degenerate Mn $e_g$ orbitals are studied in the…

Condensed Matter · Physics 2009-10-28 Jun Zang , A. R. Bishop , H. Roder

Using first-principles calculations, we investigated the magnetic, electronic, and structural properties of oxygen-substituted NaMnF3 (NaMnF1.5O1.5) with in-plane biaxial strain. For simplicity, a structure containing an oxygen octahedron…

Materials Science · Physics 2022-01-19 Wenning Ren , Kuijuan Jin , Erjia Guo , Chen Ge , Can Wang , Xiulai Xu , Hongbao Yao , Litong Jiang , Guozhen Yang

We investigate the effect of epitaxial strain on the Mott metal-insulator transition (MIT) in perovskite systems with d^1 and d^2 electron configuration of the transition metal (TM) cation. We first discuss the general trends expected from…

Strongly Correlated Electrons · Physics 2016-12-14 Gabriele Sclauzero , Krzysztof Dymkowski , Claude Ederer

First-principles calculations were performed to investigate the ferroelectric properties of barium titanate and bismuth ferrite, as well as phonon dispersion of BaTiO3, using density functional theory and density functional perturbation…

Materials Science · Physics 2014-12-08 Hong-Jian Feng

The Jahn-Teller effect in the charge-ordered (CO) state for La1-xCaxMnO3 (0.5<x<0.87) was studied by measuring the low-temperature powder x-ray diffraction, internal friction, and shear modulus. We find that the electron-lattice interaction…

Strongly Correlated Electrons · Physics 2009-11-07 R. K. Zheng , R. X. Huang , A. N. Tang , G. Li , X. G. Li , J. N. Wei , J. P. Shui , Z. Yao

We investigate the origin of the orbital ordering in the paramagnetic phase of KCrF$_3$. All previous studies described structural parameters of the paramagnetic phase using a magnetic ordering in the compound. Our simulations of real…

Strongly Correlated Electrons · Physics 2016-08-24 D. Novoselov , Dm. M. Korotin , V. I. Anisimov

In perovskite-type compounds, the interplay of cooperative Jahn-Teller effect, electronic correlations and orbital degree of freedom leads to intriguing properties. $\mathrm{NaCrF_{3}}$ is a newly synthesized Jahn-Teller active…

Materials Science · Physics 2021-01-04 Jianghan Bao , Di Wang , Hai-Zhou Lu , Xiangang Wan

By means of first-principles electronic structure calculations, we hereby investigate the structural transitions induced by epitaxial strain in (111)-oriented (LaMnO$_3$)$_{2n}|$(SrMnO$_3$)$_n$ superlattices, with $n=2,4,6$. All…

Materials Science · Physics 2026-03-04 Imran Ahamed , Shivalika Sharma , Fabrizio Cossu , Igor Di Marco

In the isostructural oxides Ca3CoMO6 (M = Co, Rh, Ir), the CoMO6 chains made up of face-sharing CoO6 trigonal prisms and MO6 octahedra are separated by Ca atoms. We analyzed the magnetic and electronic properties of these oxides on the…

Strongly Correlated Electrons · Physics 2011-01-05 Yuemei Zhang , Erjun Kan , Hongjun Xiang , Antoine Villesuzanne , Myung-Hwan Whangbo

First-principles calculations based on density functional theory + Hubbard U (DFT+U) approach have been carried out to study the strain induced variations in the optical and transport properties of the correlated perovskite SrVO$_3$. By…

Materials Science · Physics 2023-06-28 Maitreyo Biswas , Debolina Misra , Tarun K. Kundu

We investigate the effect of epitaxial strain on [001]-oriented LaAlO3 using first-principles density functional calculations. We find a series of structural phase transitions between states characterized by distinct patterns of tilting of…

Materials Science · Physics 2010-11-22 Alison J. Hatt , Nicola A. Spaldin