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Breaking space-time symmetries in two-dimensional crystals (2D) can dramatically influence their macroscopic electronic properties. Monolayer transition-metal dichalcogenides (TMDs) are prime examples where the intrinsically broken crystal…

Mesoscale and Nanoscale Physics · Physics 2015-09-04 Edbert J. Sie , James W. McIver , Yi-Hsien Lee , Liang Fu , Jing Kong , Nuh Gedik

The coherent manipulation of spin and pseudospin underlies existing and emerging quantum technologies, including NMR, quantum communication, and quantum computation. Valley polarization, associated with the occupancy of degenerate, but…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 Ziliang Ye , Dezheng Sun , Tony F. Heinz

Semiconducting transition metal dichalcogenide monolayers have emerged as promising candidates for future valleytronics-based quantum information technologies. Two distinct momentum-states of tightly-bound electron-hole pairs in these…

Mesoscale and Nanoscale Physics · Physics 2017-03-16 Gerd Plechinger , Tobias Korn , John M. Lupton

Coherent optical dressing of quantum materials offers technological advantages to control their electronic properties, such as the electronic valley degree of freedom in monolayer transition metal dichalcogenides (TMDs). Here, we observe a…

Mesoscale and Nanoscale Physics · Physics 2017-03-14 Edbert J. Sie , Chun Hung Lui , Yi-Hsien Lee , Jing Kong , Nuh Gedik

Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these…

Semiconductor transition metal dichalcogenides (TMDs) have equivalent dynamics for their two spin/valley species. This arises from their energy-degenerated spin states, connected via time-reversal symmetry. When an out-of-plane magnetic…

Increasing the speed limits of conventional electronics requires innovative approaches to manipulate other quantum properties of electrons besides their charge. An alternative approach utilizes the valley degree of freedom in…

Mesoscale and Nanoscale Physics · Physics 2023-03-29 A. O. Slobodeniuk , P. Koutenský , M. Bartoš , F. Trojánek , P. Malý , T. Novotný , M. Kozák

Monolayer transition metal dichalcogenides (TMDCs) constitute the core group of materials in the emerging semiconductor technology of valleytronics. While the coupled spin-valley physics of pristine TMDC materials and their heterstructures…

Mesoscale and Nanoscale Physics · Physics 2023-11-14 Chumki Nayak , Suvadip Masanta , Sukanya Ghosh , Shubhadip Moulick , Atindra Nath Pal , Indrani Bose , Achintya Singha

A new degree of freedom, the valley pseudospin, emerges in atomically thin two-dimensional transition metal dichalcogenides (MX2) and has attracted great scientific interest. The capability to manipulate the valley pseudospin, in analogy to…

Mesoscale and Nanoscale Physics · Physics 2014-12-10 Jonghwan Kim , Xiaoping Hong , Chenhao Jin , Su-Fei Shi , Chih-Yuan S. Chang , Ming-Hui Chiu , Lain-Jong Li , Feng Wang

Manipulation of spin and valley degrees of freedom is a key step towards realizing novel quantum technologies, for which atomically thin transition metal dichalcogenides (TMDCs) have been established as promising candidates. In monolayer…

Monolayer transition metal dichalcogenides (TMD) have immense potential for future spintronic and valleytronic applications due to their two-dimensional nature and long spin/valley lifetimes. We investigate the origin of these long-lived…

Magneto-optical spectroscopy based on the transverse magneto-optical Kerr effect (TMOKE) is a sensitive method for investigation of magnetically-ordered media. However, in magnetic materials the optical transitions are usually characterized…

Coherent light-matter interaction can be used to manipulate the energy levels of atoms, molecules and solids. When light with frequency {\omega} is detuned away from a resonance {\omega}o, repulsion between the photon-dressed (Floquet)…

Mesoscale and Nanoscale Physics · Physics 2017-03-22 Edbert J. Sie , Chun Hung Lui , Yi-Hsien Lee , Liang Fu , Jing Kong , Nuh Gedik

Selective control over the emission pattern of valley-polarized excitons in monolayer transition metal dichalcogenides is crucial for developing novel valleytronic, quantum information, and optoelectronic devices. While significant progress…

In single-layer WSe$_2$, a paradigmatic semiconducting transition metal dichalcogenide, a circularly polarized laser field can selectively excite electronic transitions in one of the inequivalent $K^{\pm}$ valleys. Such selective valley…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Alejandro Molina-Sánchez , Davide Sangalli , Ludger Wirtz , Andrea Marini

Single-layer semiconducting transition-metal dichalcogenides, lacking point inversion symmetry, provide an efficient platform for valleytronics, where the electronic, magnetic, valley and lattice degrees of freedom can be selectively…

Mesoscale and Nanoscale Physics · Physics 2024-11-19 Emmanuele Cappelluti , Habib Rostami , Federico Cilento

Achieving spatiotemporal control of light at subwavelength and subcycle scales is an important milestone in the development of new photonic materials and technologies. Ultrafast spatiotemporal light modulation currently relies on electronic…

Optics · Physics 2025-11-07 Claudio U. Hail , Lior Michaeli , Harry A. Atwater

Valley-selective optical selection rules and a spin-valley locking in transition-metal dichalcogenide (TMDC) monolayers are at the heart of "valleytronic physics", which exploits the valley degree of freedom and has been a major research…

In monolayer transition metal dichalcogenides time-reversal symmetry, combined with space-inversion symmetry, defines the spin-valley degree of freedom. As such, engineering and control of time-reversal symmetry by optical or magnetic…

Chiral interaction between light and two-dimensional transition metal dichalcogenides (2D-TMDs) has recently drawn enormous scientific attention. The optical selection rules of these atomically thin semiconductors allow the attribution of a…

Optics · Physics 2021-06-08 Irina Komen , Sabrya E. van Heijst , Sonia Conesa-Boj , L. Kuipers
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