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Related papers: Approximating Vibronic Spectroscopy with Imperfect…

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Spectroscopy is one of the most accurate probes of the molecular world. However, predicting molecular spectra accurately is computationally difficult because of the presence of entanglement between electronic and nuclear degrees of freedom.…

Accurately simulating molecular vibronic spectra remains computationally challenging due to the exponential scaling of required calculations. Here, we show that employing the linear coupling model within the gaussian boson sampling…

Quantum Physics · Physics 2025-08-07 I. Konyshev , R. Pradip , O. Page , C. Ünlüer , R. T. Nasibullin , V. V. Rybkin , W. Pernice , S. Ferrari

Quantum computers are expected to be more efficient in performing certain computations than any classical machine. Unfortunately, the technological challenges associated with building a full-scale quantum computer have not yet allowed the…

We have recently seen the first plausible claims for quantum advantage using sampling problems such as random circuit sampling and Gaussian boson sampling. The obvious next step is to channel the potential quantum advantage to solving…

Quantum Physics · Physics 2024-06-27 Changhun Oh , Youngrong Lim , Yat Wong , Bill Fefferman , Liang Jiang

We present a quantum algorithm for calculating the vibronic spectrum of a molecule, a useful but classically hard problem in chemistry. We show several advantages over previous quantum approaches: vibrational anharmonicity is naturally…

Quantum Physics · Physics 2019-08-02 Nicolas P. D. Sawaya , Joonsuk Huh

Quantum sensing encompasses highly promising techniques with diverse applications including noise-reduced imaging, super-resolution microscopy as well as imaging and spectroscopy in challenging spectral ranges. These detection schemes use…

Quantum Physics · Physics 2022-11-23 Felix Riexinger , Mirco Kutas , Björn Haase , Michael Bortz , Georg von Freymann

We provide general sufficient conditions for the efficient classical simulation of quantum-optics experiments that involve inputting states to a quantum process and making measurements at the output. The first condition is based on the…

Quantum Physics · Physics 2016-06-23 Saleh Rahimi-Keshari , Timothy C. Ralph , Carlton M. Caves

Photon losses are among the strongest imperfections affecting multi-photon interference. Despite their importance, little is known about their effect on boson sampling experiments. In this work we show that using classical computers, one…

Quantum Physics · Physics 2019-08-07 Raúl García-Patrón , Jelmer J. Renema , Valery Shchesnovich

BosonSampling is a problem where a quantum computer offers a provable speedup over classical computers. Its main feature is that it can be solved with current linear optics technology, without the need for a full quantum computer. In this…

Quantum Physics · Physics 2015-03-06 Anthony Leverrier , Raúl García-Patrón

Spectroscopy is the most important method for probing the structure of molecules. However, predicting molecular spectra on classical computers is computationally expensive, with the most accurate methods having a cost that grows…

Quantum Physics · Physics 2025-10-06 Liam P. Flew , Ivan Kassal

We discuss semiempirical approaches and parametric methods developed for modeling molecular vibronic spectra. These methods, together with databases of molecular fragments, have proved efficient and flexible for solving various problems…

Chemical Physics · Physics 2007-05-23 S. A. Astakhov , V. I. Baranov , L. A. Gribov

In previous work, we proposed a method for leveraging efficient classical simulation algorithms to aid in the analysis of large-scale fault tolerant circuits implemented on hypothetical quantum information processors. Here, we extend those…

Quantum Physics · Physics 2014-02-12 Daniel Puzzuoli , Christopher Granade , Holger Haas , Ben Criger , Easwar Magesan , D. G. Cory

There is a pressing need for more accurate computational simulations of the opto-electronic properties of defects in materials to aid in the development of quantum sensing platforms. In this work, we explore how quantum computers could be…

Quantum control is an essential tool for the operation of quantum technologies such as quantum computers, simulators, and sensors. Although there are sophisticated theoretical tools for developing quantum control protocols, formulating…

Quantum Physics · Physics 2013-04-02 Hanhan Li , Alireza Shabani , Mohan Sarovar , Birgitta K. Whaley

We propose a variational scheme to represent composite quantum systems using multiple parameterized functions of varying accuracies on both classical and quantum hardware. The approach follows the variational principle over the entire…

Quantum Physics · Physics 2024-06-21 Stefano Barison , Filippo Vicentini , Giuseppe Carleo

In this work, we simulate the behavior of photons in a laboratory experiment using a quantum computer and examine how the simulation results compare with the theoretical predictions. The experiment involves both protective and…

Quantum Physics · Physics 2025-08-13 Priyasheel Prasad , Marco Russo , Bartolomeo Montrucchio

We are concerned with numerical simulations of quantum optical circuits under certain realistic conditions, specifically that photon quantum states are not perfectly indistinguishable. The partial photon distinguishability presents a…

Quantum Physics · Physics 2023-07-14 Javier Osca , Jiri Vala

We present conditions for the efficient simulation of a broad class of optical quantum circuits on a classical machine: this class includes unitary transformations, amplification, noise, and measurements. Various proposed schemes for…

Quantum Physics · Physics 2007-05-23 Stephen D. Bartlett , Barry C. Sanders

The possibility of using time-resolved vibronic spectroscopy for spectral analysis of mixtures of chemical compounds with similar optical properties, when traditional methods are inefficient, is demonstrated by using the method of computer…

Chemical Physics · Physics 2007-05-23 S. A. Astakhov , V. I. Baranov

Quantum mechanics promises computational powers beyond the reach of classical computers. Current technology is on the brink of an experimental demonstration of the superior power of quantum computation compared to classical devices. For…

Quantum Physics · Physics 2019-04-02 Jelmer Renema , Valery Shchesnovich , Raul Garcia-Patron
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