Related papers: Coherent Bichromatic Force Deflection of Molecules
The decay of field-free rotational dynamics is experimentally studied in two complementary methods: laser-induced molecular alignment and terahertz-field-induced molecular orientation. Comparison between the decay rates of different…
The interaction of a solenoid with a passing charged particle can be treated within classical or quantum physics. If charged particles pass around both sides of a solenoid, there is an experimentally-observed Aharonov-Bohm deflection of the…
We report a strong-field detection method for magnetic materials, based on the characterization of crystal time-reversal symmetry through the elliptical dichroism of harmonics. The consistency of the low-order harmonics driven by laser…
We demonstrate laser cooling of barium monofluoride (138BaF) molecules. We use serrodynes to synthesize time-sequenced optical spectra that can be precisely tailored to the hyperfine structure of this heaviest non-radioactive alkaline earth…
Efficient excitation of a single two-level system usually requires that the driving field is at the same frequency as the atomic transition. However, the scattered laser light in solid-state implementations can dominate over the single…
We demonstrate and characterize Zeeman-Sisyphus (ZS) deceleration of a beam of ytterbium monohydroxide (YbOH). Our method uses a combination of large magnetic fields ($\sim$ 2.5 T) and optical spin-flip transitions to decelerate molecules…
The dichroism and birefringence effects in stumulated Raman scattering (SRS) in polyatomic molecules were studied theoretically. General expressions have been derived describing the change of the intensity and polarization of the probe…
We show that the momentum of light can be reversed via the atomic coherence created by another light with one or two orders of magnitude lower frequency. Both the backward retrieval of single photons from a timed Dicke state and the…
We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and…
We report on the realization of a transversely loaded two-dimensional magneto-optical trap serving as a source for cold strontium atoms. We analyze the dependence of the source's properties on various parameters, in particular the intensity…
In the quest to find a favourable triatomic molecule for detecting electric dipole moment of an electron (eEDM), we identify mercury hydroxide (HgOH) as an extremely attractive candidate from both experimental and theoretical viewpoints.…
We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…
We theoretically investigate the laser cooling of fermionic barium monofluoride (137BaF) molecules, which are promising candidates for precision studies of weak parity violation and nuclear anapole moments. This molecular species features…
Optical cycling transitions and direct laser cooling have recently been demonstrated for a number of alkaline-earth dimers and trimer molecules. This is made possible by diagonal Franck-Condon factors between the vibrational modes of the…
We compare two different models of transport of light in a disordered system with a spherical Gaussian distribution of scatterers. A coupled dipole model, keeping into account all interference effects, is compared to an incoherent model,…
A matrix representation is introduced for stationary beam-like light fields that allows for simultaneous treatment of the orbital angular momentum (OAM) and the second-order state of spatial coherence. This Coherence-OAM matrix is a…
We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear…
Optical diffraction tomography is an indispensable tool for studying objects in three-dimensions due to its ability to accurately reconstruct scattering objects. Until now this technique has been limited to coherent light because spatial…
We demonstrate a Magneto-Optical Trap (MOT) configuration which employs optical forces due to light scattering between electronically excited states of the atom. With the standard MOT laser beams propagating along the {\it x}- and {\it y}-…
Collective coherent light scattering by polarizable particles creates surprisingly strong, long range inter-particle forces originating from interference of the light scattered by different particles. While for monochromatic laser beams…