Related papers: Coherent Bichromatic Force Deflection of Molecules
We demonstrate the excitation, using a structured light beam carrying orbital angular momentum, of the center of mass motion of a single atom in the transverse direction to the beam's propagation. This interaction is achieved with a vortex…
A cryogenic buffer gas beam, an electrostatic hexapole lens, and 2D transverse Doppler laser cooling are combined to produce a bright beam of barium monofluoride ($^{138}$Ba$^{19}$F) molecules. Experimental results and trajectory…
Supersonic beams of polar molecules are deflected using inhomogeneous electric fields. The quantum-state selectivity of the deflection is used to spatially separate molecules according to their quantum state. A detailed analysis of the…
Several laser techniques have been suggested and demonstrated recently for preparing polarizable molecules in rapidly spinning states with a disc-like angular distribution. We consider motion of these spinning discs in inhomogeneous fields,…
We introduce and study coherent polarization self-rotation (CPSR), a two-photon light-matter interaction in dense alkali-metal vapors that enables both narrowband optical spectroscopy of magnetic transitions and coherent coupling between…
Optical forces allow manipulation of small particles and control of nanophotonic structures with light beams. Here, we describe a counter-intuitive lateral optical force acting on particles placed above a substrate, under uniform plane wave…
We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…
We investigate the transient coherent transmission of light through an optically thick cold stron-tium gas. We observe a coherent superflash just after an abrupt probe extinction, with peak intensity more than three times the incident one.…
We study the manipulation of slow light with an orbital angular momentum propagating in a cloud of cold atoms. Atoms are affected by four copropagating control laser beams in a double tripod configuration of the atomic energy levels…
We investigated the nanosecond-scale time decay of the blue-green light emitted by nominally pure SrTiO$_3$ following the absorption of an intense picosecond laser pulse generating a high density of electron-hole pairs. Two independent…
By analyzing the parameters of electronic transitions, we show how bosonic Sr atoms in planar optical lattices can be engineered to exhibit optical magnetism and other higher-order electromagnetic multipoles that can be harnessed for…
We demonstrate a left-right asymmetry control of the photo\-electron angular distribution in multi\-photon ionization of Li atoms by a bichromatic laser field. By delaying the fundamental (780 nm) and its second harmonic relative to each…
We propose an approach to probe coherent spin-state dynamics of molecules using circularly polarized hard x-ray pulses. For the dynamically aligned nitric oxide molecules in a coherent superposition spin-orbit coupled electronic state that…
Alignment and orientation of molecules by intense, ultrashort laser fields are crucial for a variety of applications in physics and chemistry. These include control of high harmonics generation, molecular orbitals tomography, control of…
A special class of molecules that are important to many subfields in molecular dynamics and chemical physics, namely free radical molecules, now enjoy a significant degree of center-of-mass motion control in the laboratory frame. The…
A Brownian particle's random motions can be rectified by a periodic potential energy landscape that alternates between two states, even if both states are spatially symmetric. If the two states differ only by a discrete translation, the…
Electric deflection measurements on liquid helium nanodroplets doped with individual polar molecules demonstrate that the cold superfluid matrix enables full orientation of the molecular dipole along the external field. This translates into…
Organic exciton-photon polariton lasers have recently been shown to be remarkable candidates for the realization of efficient sources of coherent light operating at room temperature. While their thresholds are now comparable with…
We report on a theoretical study of a Cs$_2$ molecule illuminated by two lasers and show how it can result in novel quantum dynamics. We reveal that these interactions facilitate the bypass of the non-crossing rule, forming Light-Induced…
We study the impact of double and triple scattering contributions on coherent backscattering of laser light from saturated isotropic atoms, in the helicity preserving polarization channel. Using the recently proposed diagrammatic pump-probe…