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We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

We perform a detailed analysis of how high-order harmonic generation (HHG) and above-threshold ionization (ATI) can be controlled by a time-delayed attosecond-pulse train superposed to a strong, near-infrared laser field. In particular we…

Atomic Physics · Physics 2009-11-11 C. Figueira de Morisson Faria , P. Salieres , P. Villain , M. Lewenstein

Using real-space view of high harmonic generation (HHG) in solids, we develop a physically transparent and gauge-invariant approach for distinguishing intraband and interband HHG mechanisms. Our approach relies on resolving the harmonic…

Recent advancements in the generation of mid-infrared and terahertz laser pulses have enabled us to observe strong-field driven non-perturbative high-harmonic generation (HHG) from semiconductors, dielectrics, and semimetals. HHG has added…

Optics · Physics 2022-03-22 M. S. Mrudul

Generation of high-order harmonics in gases enabled to probe the attosecond electron dynamics in atoms and molecules with unprecedented resolution. Extending the techniques developed originally for atomic and molecular gases to solid state…

Optics · Physics 2020-02-04 Mrudul M. S. , Nicolas Tancogne-Dejean , Angel Rubio , Gopal Dixit

Charged excitons (trions) are essential for the optical spectra in low dimensional doped monolayers (ML) of transitional metal dichalcogenides (TMDC). Using a direct diagonalization of the three-body Hamiltonian, we explore the low-lying…

Materials Science · Physics 2023-01-23 Yaroslav V. Zhumagulov , Alexei Vagov , Dmitry R. Gulevich , Vasili Perebeinos

We report observation of strong and anisotropic third harmonic generation (THG) in monolayer and multilayer ReS$_2$. The third-order nonlinear optical susceptibility of monolayer ReS$_2$, $\left| \chi^{(3)} \right|$ is on the order of…

Materials Science · Physics 2017-04-12 Qiannan Cui , Rodrigo A. Muniz , J. E. Sipe , Hui Zhao

Single layers of transition metal dichalcogenides (TMDs) are direct gap semiconductors with nondegenerate valley indices. An intriguing possibility for these materials is the use of their valley index as an alternate state variable. Several…

Layered transition metal dichalcogenides (TMDCs) host a variety of strongly bound exciton complexes that control the optical properties in these materials. Apart from spin and valley, layer index provides an additional degree of freedom in…

Mesoscale and Nanoscale Physics · Physics 2019-05-08 Sarthak Das , Garima Gupta , Kausik Majumdar

Monolayers of transition-metal dichalcogenides have shown that uniaxial strain changes both the photoluminescence emission energy and intensity. The changes are attributed to the band-structure evolution under tensile strain where both the…

Materials Science · Physics 2026-05-19 Lee Grimberg , Svyatoslav Kostyukovets , Moshe G. Harats

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

Two-dimensional (2D) transition metal dichalcogenides (TMDCs) have attracted great attention due to their physical and chemical properties that make them promising in electronics and optoelectronics. Because of the difficulties in…

Applied Physics · Physics 2020-07-20 Lei Tang , Tao Li , Yuting Luo , Simin Feng , Zhengyang Cai , Hang Zhang , Bilu Liu , Hui-Ming Cheng

Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these…

Although the frequency shift and odd-even intensity modulation in high-order harmonic generation (HHG) have both been observed for asymmetric laser-target systems, they are typically studied as two separate phenomena. In this Letter, we…

Optics · Physics 2024-06-14 Doan-An Trieu , Van-Hoang Le , Ngoc-Loan Phan

Transition metal dichalcogenides (TMDs) are promising candidates for a wide variety of ultrascaled electronic, quantum computation, and optoelectronic applications. The exponential decay of electronic density of states into the bandgap,…

Mesoscale and Nanoscale Physics · Physics 2023-08-04 Prasad Sarangapani , James Charles , Tillmann Kubis

High-harmonic generation in solids has emerged as a powerful probe of ultrafast electron dynamics and lattice motion, and recent theoretical work has suggested that thermally driven lattice fluctuations can act as an effective source of…

Two-dimensional transition metal dichalcogenides (TMDCs) have recently become attractive semiconductor materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and…

Optics · Physics 2018-07-04 Alex Krasnok , Sergey Lepeshov , Andrea Alú

High harmonic generation (HHG) in gaseous media provides a robust method for producing coherent extreme-ultraviolet (EUV) radiation and attosecond pulses. However, the spectral and temporal properties of these pulses -- such as bandwidth…

We investigate an excitonic peak appearing in low-temperature photoluminescence of monolayer transition metal dichalcogenides (TMDCs), which is commonly associated with defects and disorder. First, to uncover the intrinsic origin of…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 Kyrylo Greben , Sonakshi Arora , Moshe G. Harats , Kirill I. Bolotin

We consider the interaction of gapped graphene in the two-band approximation using an explicit time-dependent approach. In addition to the full high-order harmonic generation (HHG) spectrum, we also obtain the perturbative harmonic response…

Materials Science · Physics 2017-02-01 Darko Dimitrovski , Lars Bojer Madsen , Thomas Garm Pedersen