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Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…

Optics · Physics 2016-07-22 Martin Weismann , Nicolae C. Panoiu

High harmonic generation(HHG) is one of the most commonly studied nonlinear optical phenomena, originating in the ultrafast dynamics of electrons in atomic gasses and semiconductors. It has attracted much attention because of its…

Optics · Physics 2023-09-08 Akira Kofuji , Robert Peters

We theoretically study the interaction of an ultrafast intense linearly polarized optical pulse with monolayers of transition metal dichalcogenides (TMDCs). Such a strong pulse redistributes electrons between the bands and generates…

Mesoscale and Nanoscale Physics · Physics 2021-04-21 S. Azar Oliaei Motlagh , Vadym Apalkov , Mark I. Stockman

Recent techniques have allowed transition metal dichalcogenides (TMD) monolayers to be grown and adequately characterised. Of particular interest, their nonlinear optical response presents many promising opportunities for future…

Mesoscale and Nanoscale Physics · Physics 2020-03-06 David N. Carvalho , Fabio Biancalana

Atomically thin layers of transition metal dichalcogenides (TMDCs) exhibit exceptionally strong Coulomb interaction between charge carriers due to the two-dimensional carrier confinement in connection with weak dielectric screening. The van…

Materials Science · Physics 2018-07-18 A. Steinhoff , T. O. Wehling , M. Rösner

Monolayer transition metal dichalcogenides (TMDs) exhibit high nonlinear optical (NLO) susceptibilities. Experiments on MoS$_2$ have indeed revealed very large second-order ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) optical…

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

Since the seminal work on MoS2 monolayers, photoexcitation in atomically-thin transition metal dichalcogenides (TMDCs) has been assumed to result in excitons with large binding energies (~ 200-600 meV). Because the exciton binding energies…

We investigate High-harmonic generation (HHG) in a dimerized Kitaev chain. The dimerization in the model is introduced through a site-dependent modulating potential, determined by a parameter $\lambda \in [-1:1]$. This parameter also…

Other Condensed Matter · Physics 2025-06-06 Nivash R. , S. Srinidhi , Jayendra N. Bandyopadhyay , Amol R. Holkundkar

High harmonic generation (HHG) is an extremely nonlinear effect, where a medium is driven by a strong laser field, generating coherent broadband radiation with photon energies ranging up to the X-ray and pulse durations reaching attosecond…

Optics · Physics 2020-10-20 Alexey Gorlach , Ofer Neufeld , Nicholas Rivera , Oren Cohen , Ido Kaminer

Monolayers of transition metal dichalcogenides (TMdC) are promising candidates for realization of a new generation of optoelectronic devices. The optical properties of these two-dimensional materials, however, vary from flake to flake, or…

Materials Science · Physics 2020-01-22 Pavel V. Kolesnichenko , Qianhui Zhang , Changxi Zheng , Michael S. Fuhrer , Jeffrey A. Davis

We theoretically investigate high-harmonic generation (HHG) in honeycomb-lattice graphene models when subjected to a DC electric field. By integrating the quantum master equation with the Boltzmann equation, we develop a numerical method to…

Mesoscale and Nanoscale Physics · Physics 2024-07-16 Minoru Kanega , Masahiro Sato

We theoretically study high-harmonic generation (HHG) from transition metal elements Mn and Mn$^+$, using full-dimensional, all-electron, first-principles simulations. The HHG spectra calculated with the time-dependent complete-active-space…

Atomic Physics · Physics 2019-06-26 Imam S. Wahyutama , Takeshi Sato , Kenichi L. Ishikawa

We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…

Mesoscale and Nanoscale Physics · Physics 2013-06-12 Sung-Young Hong , Jerry I. Dadap , Nicholas Petrone , Po-Chun Yeh , James Hone , Richard M. Osgood

High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under…

Quantum Physics · Physics 2024-09-25 Javier Rivera-Dean

High-harmonic generation (HHG) in two-dimensional materials offers a compelling route toward compact extreme ultraviolet sources and probing electron dynamics on the attosecond scale. However, achieving precise control over the emission and…

Computational Physics · Physics 2026-05-19 Zhenjiang Zhao , Zhihua Zheng , Zhiyi Xu , Xing Ran , Xiaolong Yao , Fangping Ouyang

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

Quantum Physics · Physics 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

We find that a donor-doped band-gap material can enhance the overall high-order harmonic generation (HHG) efficiency by several orders of magnitude, compared with undoped and acceptor-doped materials. This significant enhancement, predicted…

Optics · Physics 2019-01-30 Chuan Yu , Kenneth K. Hansen , Lars Bojer Madsen

Transition metal dichalcogenide (TMDC) monolayers present a remarkable multifunctional material with potential to enable the development of a wide range of novel devices. However, the functionalities observed often fall short of the…

High-order harmonic generation (HHG) in solids is profoundly influenced by the dephasing of the coherent electron-hole motion driven by an external laser field. The exact physical mechanisms underlying this dephasing, crucial for accurately…