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We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

Strongly Correlated Electrons · Physics 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

We report the first experimental observation of frequency shift in high order harmonic generation (HHG) from isotopic molecules H2 and D2 . It is found that harmonics generated from the isotopic molecules exhibit obvious spectral red shift…

Atomic Physics · Physics 2016-04-25 Lixin He , Pengfei Lan , Chunyang Zhai , Feng Wang , Wenjing Shi , Qingbin Zhang , Xiaosong Zhu , Peixiang Lu

The optimal design for infrared second harmonic generation (SHG) is determined for a GaAs-based quantum device using a recently developed genetic approach. Both compositional parameters and electric field are simultaneously optimized, and…

Materials Science · Physics 2009-10-31 Guido Goldoni

High-order harmonic generation (HHG) provides a broad spectral bandwidth for synthesizing attosecond pulses. However, in the current HHG schemes, only part of the harmonics can be phase-locked, which limits the ability to achieve shorter…

Optics · Physics 2024-06-18 ShiJun Wang , XuanYang Lai , XiaoJun Liu

We theoretically investigate high-order harmonic generation (HHG) in graphene under mid-infrared (MIR) and terahertz (THz) fields based on a quantum master equation. Numerical simulations show that MIR-induced HHG in graphene can be…

Materials Science · Physics 2023-07-03 Wenwen Mao , Angel Rubio , Shunsuke A. Sato

High-order sideband generation (HSG), as an analogue of the interband processes in high-harmonic generation (HHG) in solids, is a nonperturbative nonlinear optical phenomenon in semiconductors that are simultaneously driven by a relatively…

Optics · Physics 2023-05-31 Qile Wu , Mark S. Sherwin

We present theoretical predictions of high-order harmonic generation (HHG) resulting from the interaction of short femtosecond laser pulses with metal nanotips. It has been demonstrated that high energy electrons can be generated using…

Quantum-optical descriptions of strong-field processes have attracted significant attention in recent years. Typically, the theoretical modeling has been conducted in the Schr\"odinger picture, where results are only obtainable under…

High harmonic generation (HHG) spectra have the potential to show novel signatures of ordered phases in condensed matter. We studied the femtosecond laser-driven electronic response of monolayer NbSe2 using state-of-the-art computational…

Materials Science · Physics 2020-12-21 Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

We theoretically investigate the effects of the excitation frequency on the plateau of high-order terahertz sideband generation (HSG) in semiconductors driven by intense terahertz (THz) fields. We find that the plateau of the sideband…

Mesoscale and Nanoscale Physics · Physics 2014-01-17 Xiao-Tao Xie , Bang-Fen Zhu , Ren-Bao Liu

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately…

High-order harmonic generation (HHG) in solids - the frequency up-conversion of an optical signal - is governed by symmetries. At terahertz (THz) frequencies, HHG is a key technology to access high frequency spectral windows that are…

The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal…

We study high-harmonic generation (HHG) in the one-dimensional Hubbard model in order to understand its relation to elementary excitations as well as the similarities and differences to semiconductors. The simulations are based on the…

Strongly Correlated Electrons · Physics 2021-01-13 Yuta Murakami , Shintaro Takayoshi , Akihisa Koga , Philipp Werner

The generation of high-order harmonics in finite, hexagonal nanoribbons is simulated. Ribbons with armchair and zig-zag edges are investigated by using a tight-binding approach with only nearest neighbor hopping. By turning an alternating…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Hannah Jürß , Dieter Bauer

High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…

The long standing issue of separating resonant from non-resonant processes in extreme nonlinear optics is resolved. The theoretical formalism is applied to high harmonic generation (HHG) in solids and reveals a deeper view into the dominant…

Optics · Physics 2022-06-03 A. Thorpe , N. Boroumand , A. M. Parks , E. Goulielmakis , T. Brabec

Here, we study the possibility of selective high-harmonic generation (HHG) based on the concept of charge transfer plasmons (CTP) in bridged nanoparticle assemblies. By choosing plasmonic dimer nanoantenna, as a fundamental member of…

Optics · Physics 2018-01-16 Burak Gerislioglu , Arash Ahmadivand , Nezih Pala

In this work, the nonlinear optical response, and in particular, the high harmonic generation of semiconductors is addressed by using the Wannier gauge. One of the main problems in the time evolution of the Semiconductor Bloch equations…

Mesoscale and Nanoscale Physics · Physics 2019-11-20 R. E. F. Silva , F. Martín , M. Ivanov