Related papers: A cryofuge for cold-collision experiments with slo…
We discuss techniques to engineer effective long-range interactions between polar molecules using external static electric and microwave fields. We consider a setup where molecules are trapped in a two-dimensional pancake geometry by a…
Cold, continuous, high flux beams of benzonitrile, fluorobenzine, and anisole have been created. Buffer-gas cooling with a cryogenic gas provides the cooling and slow forward beam velocities. The beam of benzonitrile was measured to have a…
A novel two-stage helium buffer gas cooled beam source is introduced. The properties of the molecular beams produced from this source are investigated theoretically using the CaF as a test molecule. The gas-phase molecules are first…
We demonstrate simultaneous deceleration and trapping of a cold atomic and molecular mixture. This is the first step towards studies of cold atom-molecule collisions at low temperatures as well as application of sympathetic cooling. Both…
Cooling forces result from the retarded dipole interaction between an illuminated particle and its reflection. For a one-dimensional example, we find cooling times of milliseconds and limiting temperatures in the millikelvin range. The…
A quantum gas of ultracold polar molecules, with long-range and anisotropic interactions, would not only enable explorations of a large class of many-body physics phenomena, but could also be used for quantum information processing. We…
Thermophoresis moves molecules along temperature gradients, typically from hot to cold. We superpose fluid flow with thermophoretic molecule flow under well defined microfluidic conditions, imaged by fluorescence microscopy. DNA is trapped…
Stable ultracold ensembles of dipolar molecules hold great promise for many-body quantum physics, but high inelastic loss rates have been a long-standing challenge. Recently, it was shown that gases of fermionic molecules can be effectively…
Long-range intermolecular forces are able to steer polar molecules submerged in superfluid helium nanodroplets into highly polar metastable configurations. We demonstrate that the presence of such special structures can be identified, in a…
We show theoretically that ultracold hydrogen atoms have very favorable properties for sympathetic cooling of molecules to microkelvin temperatures. We calculate the potential energy surfaces for spin-polarized interactions of H atoms with…
We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and…
We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable…
A recent experiment reported for the first time the preparation of a Fermi degenerate gas of polar molecules and observed a suppression of their chemical reaction rate compared to the one expected from a purely classical treatment. While it…
We examine the prospects for utilizing the optical bichromatic force (BCF) to greatly enhance laser deceleration and cooling for near-cycling transitions in small molecules. We discuss the expected behavior of the BCF in near-cycling…
The study of cold and controlled molecular ions is pivotal for fundamental research in modern physics and chemistry. Investigations into cooling molecular anions, in particular, have proven to be of key consequence for the production of…
Molecular cooling is essential for studying the formation of sub-structure of dissipative dark-matter halos that may host compact objects such as black holes. Here, we analyze the reaction rates relevant for the formation, dissociation, and…
For the one-dimensional linear kinetic equations with collisional frequency of the molecules, proportional to the module velocity of molecules, analytical solutions of problems about temperature jump and weak evaporation (condensation) in…
We describe a method for cooling neutral molecules that have magnetic and electric dipole moments using collisions with cold ions. An external magnetic field is used to split the ground rovibrational energy levels of the molecule. The…
We introduce a new optical tool - a "two-dimensional optical centrifuge", capable of aligning molecules in extreme rotational states. Unlike the conventional centrifuge, which confines the molecules in the plane of their rotation, its…
We describe a novel type of interaction between open-shell polar molecules at sub-millikelvin temperatures. This hyperfine van der Waals interaction occurs between two molecules in two rotational states that differ by one quantum. Normally,…