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Vibronic coupling has a dramatic influence over a large number of molecular processes, ranging from photo-chemistry, to spin relaxation and electronic transport. The simulation of vibronic coupling with multi-reference wavefunction methods…

Chemical Physics · Physics 2023-10-17 Lorenzo A. Mariano , Sourav Mondal , Alessandro Lunghi

We introduce a framework for designing Hamiltonian engineering pulse sequences that systematically accounts for the effects of higher-order contributions to the Floquet-Magnus expansion. Our techniques result in simple, intuitive decoupling…

Quantum Physics · Physics 2024-01-15 Matthew Tyler , Hengyun Zhou , Leigh S. Martin , Nathaniel Leitao , Mikhail D. Lukin

Interacting spins in quantum magnet can cooperate and exhibit exotic states like the quantum spin liquid. To explore the materialization of such intriguing states, the determination of effective spin Hamiltonian of the quantum magnet is…

Strongly Correlated Electrons · Physics 2021-09-01 Sizhuo Yu , Yuan Gao , Bin-Bin Chen , Wei Li

Optimal control techniques are applied for the decomposition of unitary quantum operations into a sequence of single-qubit gates and entangling operations. To this end, we modify a gradient-ascent algorithm developed for systems of coupled…

Quantum Physics · Physics 2009-01-15 V. Nebendahl , H. Haffner , C. F. Roos

Motivated by recent work on Heisenberg antiferromagnetic spin systems on various lattices made up of triangles, we examine the low-energy properties of a chain of antiferromagnetically coupled triangles of half-odd-integer spins. We derive…

Strongly Correlated Electrons · Physics 2009-10-31 C. Raghu , Indranil Rudra , S. Ramasesha , Diptiman Sen

Quantum simulation is a promising near term application for mesoscale quantum information processors, with the potential to solve computationally intractable problems at the scale of just a few dozen interacting quantum systems. Recent…

Quantum Physics · Physics 2014-08-14 David L. Hayes , Steven T. Flammia , Michael J. Biercuk

We derive an effective spin Hamiltonian for the one-dimensional half-filled asymmetric ionic Hubbard model with alternating on-site interaction in the limit of strong repulsion. It is shown that the effective Hamiltonian is that of a spin…

Strongly Correlated Electrons · Physics 2016-02-01 Inna Grusha , Mikheil Menteshashvili , George I. Japaridze

The need for strategies able to accurately manipulate quantum dynamics is ubiquitous in quantum control and quantum information processing. We investigate two scenarios where randomized dynamical decoupling techniques become more…

Quantum Physics · Physics 2009-11-13 Lorenza Viola , Lea F. Santos

Engineering strong interactions between quantum systems is essential for many phenomena of quantum physics and technology. Typically, strong coupling relies on short-range forces or on placing the systems in high-quality electromagnetic…

We propose a general framework to extract microscopic interactions from raw configurations with deep neural networks. The approach replaces the modeling Hamiltonian by the neural networks, in which the interaction is encoded. It can be…

Computational Physics · Physics 2020-08-19 Lingxiao Wang , Yin Jiang , Kai Zhou

Quantum spin networks having engineered geometries and interactions are eagerly pursued for quantum simulation and access to emergent quantum phenomena such as spin liquids. Spin-1/2 centers are particularly desirable because they readily…

Quantum control in large dimensional Hilbert spaces is essential for realizing the power of quantum information processing. For closed quantum systems the relevant input/output maps are unitary transformations, and the fundamental challenge…

Quantum Physics · Physics 2014-10-17 B. E. Anderson , H. Sosa-Martinez , C. A. Riofrío , I. H. Deutsch , P. S. Jessen

Recently, several platforms were proposed and demonstrated a proof-of-principle for finding the global minimum of the spin Hamiltonians such as the Ising and XY models using gain-dissipative quantum and classical systems. The implementation…

Emerging Technologies · Computer Science 2018-07-03 Kirill P. Kalinin , Natalia G. Berloff

For finite-dimensional quantum systems, such as qubits, a well established strategy to protect such systems from decoherence is dynamical decoupling. However many promising quantum devices, such as oscillators, are infinite dimensional, for…

Quantum Physics · Physics 2017-04-05 Christian Arenz , Robin Hillier , Daniel Burgarth

The electron spin of a nitrogen-vacancy center in diamond lends itself to the control of proximal $^{13}$C nuclear spins via dynamical decoupling methods, possibly combined with radio-frequency driving. Long-lived single-qubit states and…

Quantum Physics · Physics 2025-07-29 W. -R. Hannes , Regina Finsterhoelzl , Guido Burkard

The capacity to custom tailor the properties of quantum matter and materials is a central requirement for enlarging their range of possible functionalities. A particularly promising route is the use of driving protocols to engineer specific…

Quantum Physics · Physics 2025-02-19 Zhanpeng Fu , Roderich Moessner , Hongzheng Zhao , Marin Bukov

Spin Hamiltonians, like the Heisenberg model, are used to describe magnetic properties of exchange-coupled molecules and solids. For finite clusters, physical quantities such as heat capacities, magnetic susceptibilities or…

Strongly Correlated Electrons · Physics 2025-06-24 Shadan Ghassemi Tabrizi , Thomas D. Kühne

Quantum pseudorandomness, also known as unitary designs, comprise a powerful resource for quantum computation and quantum engineering. While it is known in theory that pseudorandom unitary operators can be constructed efficiently, realizing…

Quantum Physics · Physics 2019-07-24 Jun Li , Zhihuang Luo , Tao Xin , Hengyan Wang , David Kribs , Dawei Lu , Bei Zeng , Raymond Laflamme

We experimentally demonstrate an approach to scale up quantum devices by harnessing spin defects in the environment of a quantum probe. We follow this approach to identify, locate, and control two electron-nuclear spin defects in the…

Quantum Physics · Physics 2020-03-04 Alexandre Cooper , Won Kyu Calvin Sun , Jean-Christophe Jaskula , Paola Cappellaro

Simple constructions and protocols are demonstrated to allow the implementation of universal quantum computation on an arbitrarily large quantum system by controlling a fixed number of spins, vastly reducing the engineering requirements in…

Quantum Physics · Physics 2009-04-23 Alastair Kay
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