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We present a practical scheme to separate the contributions of the electric quadrupole-like and the magnetic dipole-like effects to the forbidden second order optical nonlinear response of graphene, and give analytic expressions for the…

Materials Science · Physics 2017-03-08 J. L. Cheng , N. Vermeulen , J. E. Sipe

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

We propose a novel method for controlling the high-harmonic generation (HHG) with a high dynamic range in single-layer graphene. We find that, by utilizing shear strain, a significant enhancement or quenching of HHG is possible over a range…

Mesoscale and Nanoscale Physics · Physics 2023-03-02 Tomohiro Tamaya , Hidefumi Akiyama , Takeo Kato

Tuning the macroscopic dielectric response on demand holds potential for actively tunable metaphotonics and optical devices. In recent years, graphene has been extensively investigated as a tunable element in nanophotonics. Significant…

Applied Physics · Physics 2019-10-23 Jeremy Brouillet , Georgia T. Papadakis , Harry A. Atwater

We present a finite-temperature diagrammatic perturbation theory of third harmonic generation (THG) in doped graphene. We carry out calculations of the third-order conductivity in the scalar potential gauge, highlighting a subtle…

Mesoscale and Nanoscale Physics · Physics 2016-05-04 Habib Rostami , Marco Polini

We propose a new concept to generate efficient one-third harmonic light from an unseeded third harmonic process in optical fibers. Our concept is based on the dynamic constant (Hamiltonian) of the nonlinear third harmonic generation in…

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The…

The unique linear and massless band structure of graphene, in a purely two-dimensional Dirac fermionic structure, have led to intense research spanning from condensed matter physics to nanoscale device applications covering the electrical,…

The linear electrodynamic properties of graphene -- the frequency-dependent conductivity, the transmission spectra and collective excitations -- are briefly outlined. The non-linear frequency multiplication effects in graphene are studied,…

Mesoscale and Nanoscale Physics · Physics 2009-05-27 S. A. Mikhailov

It is commonly believed that weak light-matter interactions in low-mobility graphene dramatically limits tunability of graphene-based optoelectronic devices, such as tunable absorbers or switches. In this paper, we develop and use a simple…

Optics · Physics 2018-12-11 Xuchen Wang , Sergei A. Tretyakov

We demonstrate that the broadband nonlinear optical response of graphene can be resonantly enhanced by more than an order of magnitude through hybridization with a plasmonic metamaterial,while retaining an ultrafast nonlinear response time…

The modulation of the optical transmittance in multilayer graphene by means of an electrical signal in the simple configuration of coplanar electrodes is reported. Besides the fundamental frequency of modulation, higher harmonics also…

Mesoscale and Nanoscale Physics · Physics 2013-08-26 J. L. Benítez , D. Mendoza

We report on theoretical study of second harmonic generation in graphene. Phenomenological analysis based on symmetry arguments is carried out. It is demontrated, that in ideal graphene samples second harmonic generation is possible only if…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 M. M. Glazov

Among its many outstanding properties, graphene supports terahertz surface plasma waves -- sub-wavelength charge density oscillations connected with electromagnetic fields that are tightly localized near the surface[1,2]. When these waves…

It is shown that the massless energy spectrum of electrons and holes in graphene leads to the strongly non-linear electromagnetic response of this system. We predict that the graphene layer, irradiated by electromagnetic waves, emits…

Mesoscale and Nanoscale Physics · Physics 2007-07-24 S. A. Mikhailov

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

Materials Science · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

In a semiconductor illuminated by a strong terahertz field, optically excited electron-hole pairs can recombine to emit light in a broad frequency comb evenly spaced by twice the terahertz frequency. Such high-order terahertz sideband…

Mesoscale and Nanoscale Physics · Physics 2015-01-20 J. A. Crosse , Xiaodong Xu , Mark S. Sherwin , R. B. Liu

Strong inter-particle interactions between polaritons have traditionally stemmed from their exciton component. In this work, we impart a strong photonic nonlinearity to a polaritonic mode by embedding a nonlinear polymethine dye within a…

The nonlinear response of electrons (holes) in doped graphene on ac pumping is considered theoretically for the frequency region above the energy relaxation rate but below the momentum and carrier-carrier scattering rates.…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 F. T. Vasko

Graphene, a unique two-dimensional material of carbon in a honeycomb lattice, has brought remarkable breakthroughs across the domains of electronics, mechanics, and thermal transport, driven by the quasiparticle Dirac fermions obeying a…