Related papers: Doppler-free coherent-control spectroscopy with a …
We report on an experimental test of the spin selection rule for two-photon transitions in atoms. In particular, we demonstrate that the $5S_{1/2}\to 6S_{1/2}$ transition rate in a rubidium gas follows a quadratic dependency on the helicity…
Light generation through optical harmonics plays a pivotal role in photonics, driving innovations in coherent light sources, biological imaging, and spectroscopy. Traditional methods for tuning optical harmonics, including electrostatic…
Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this…
Coherent control of individual two-level systems (TLSs) is at the basis of any implementation of quantum information. An impressive level of control is now achieved using nuclear, vacancies and charge spins. Manipulation of bright exciton…
Reprogrammable linear optical circuits are essential elements of photonic quantum technology implementations. Integrated optics provides a natural platform for tunable photonic circuits, but faces challenges when high dimensions and high…
We propose an efficient all-optical phase modulation based on a double-{\Lambda} system and demonstrate a {\pi} phase shift of a few-photon pulse induced by another few-photon pulse in cold rubidium atoms with this scheme. By changing the…
By studying the fluorescence and optical properties of a three-level system, we propose a new point of view on the coherent control of these spectra. With the definite phase difference between the fields of the air band and dielectric band…
Light interacting with metals elicits an ultrafast coherent many-body screening response on sub- to few-femtosecond time-scales, which makes its experimental observation challenging. Here, we describe the coherent two-dimensional (2D)…
We implement double electromagnetically-induced transparency (double EIT) in rubidium vapor, using a tripod-shaped energy level scheme consisting of hyperfine and magnetic sublevels of the 5S1/2 to 5P1/2 transition. We show experimentally…
A novel technique to sensitively and selectively isolate multiple-quantum coherences in a femtosecond pump-probe setup is presented. Detecting incoherent observables and imparting lock-in amplification, even weak signals of highly dilute…
The strong confinement of semiconductor excitons in a quantum dot gives rise to atom-like behavior. The full benefit of such a structure is best observed in resonant excitation where the excited state can be deterministically populated and…
New feasibity of coherent quantum control of four-wave mixing processes in a resonant Doppler-broadened medium are studied. We propose a technique which enables one to enhance the quantum efficiency of nonlinear optical conversion. At the…
Coherent control of ultrafast molecule making from colliding reactants is crucial for realizing coherent control of binary photoreactions (CCBP). To handle diverse excitation scenarios, feasibility with both weak and strong fields is…
Considering the problem of the control of a two-state quantum system by an external field, we establish a general and versatile method that allows the derivation of smooth pulses, suitable for ultrafast applications, that feature the…
Well controlled nonlinear interactions between light field pulses and single atoms could be used to implement optical quantum information technologies based on qubits encoded in superpositions of coherent states of light. Here, we…
In recent years nanoscale coherent imaging has emerged as an indispensable imaging modality allowing to surpass the resolution limit given by classical imaging optics. At the same time, attosecond science has experienced enormous progress…
Free electrons provide a powerful tool to probe material properties at atomic-scale spatial resolution. Recent advances in ultrafast electron microscopy enable the manipulation of free electron wavefunctions using laser pulses. It would be…
Multiphoton interference is an important phenomenon in modern quantum mechanics and experimental quantum optics, and it is fundamental for the development of quantum information science and technologies. Over the last three decades, several…
The coupling of laser light to matter can exert sub-cycle coherent control over material properties, with optically induced currents and magnetism shown to be controllable on ultrafast femtosecond time scales. Here, by employing laser light…
We introduce the first method to enable an optical amplification of a coherent Raman spectroscopy signal called radio frequency Doppler Raman spectroscopy. Doppler Raman measurements amplify the optical signals in coherent Raman…