Related papers: Doppler-free coherent-control spectroscopy with a …
Direct frequency-comb spectroscopy is used to probe the absolute frequencies of $6S_{1/2}$-$8S_{1/2}$ two-photon transitions of atomic cesium in hot vapor environment. By utilizing the coherent control method of temporally splitting the…
Positronium and muonium, as purely leptonic atoms without internal structure, provide ideal systems for high-precision tests of quantum electrodynamics (QED) and measurements of fundamental constants. However, the high velocities of these…
Optical two-dimensional coherent spectroscopy (2DCS) has become a powerful tool for studying energy level structure, dynamics, and coupling in many systems including atomic ensembles. Various types of two-dimensional (2D) spectra, including…
We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.
We demonstrate numerically a method of focusing two-photon field inside one-dimensional random media. The approach is based on coherent control of backscattering achieved by adaptive spectral pulse shaping. The spectral phases of a…
Photoassociation of ultracold rubidium atoms with femtosecond laser pulses is studied theoretically. The spectrum of the pulses is cut off in order to suppress pulse amplitude at and close to the atomic resonance frequency. This leads to…
We report on the demonstration of a femtosecond all-optical modulator providing, without nonlinearity and therefore at arbitrarily low intensity, ultrafast light-by-light control. The device engages the coherent interaction of optical waves…
We report a new method of two-pathway coherent control using three narrow-band cw laser sources, phase locked in an optical phase-lock loop, to maintain the high degree of optical coherence required for the coherent control process. In…
It is demonstrated that the non-instantaneous response of the optically induced coherent polarization tremendously influences the real-space shift of electronic charges in semiconductors. The possibility to coherently control this…
Coherent control of two-state systems is traditionally achieved by resonant pulses of specific Rabi frequency and duration, by adiabatic techniques using level crossings or delayed pulses, or by sequences of pulses with precise relative…
We study an integrated silicon photonic chip, composed of several sub-wavelength ridge waveguides, and immersed in a micro-cell with rubidium vapor. Employing two-photon excitation, including a telecom wavelength, we observe that the…
We demonstrate spectral shaping of entangled photons with a six-channel microring-resonator-based silicon photonic pulse shaper. Through precise calibration of thermal phase shifters in a microresonator-based pulse shaper, we demonstrate…
We report on experimental and theoretical study of the nonlinear Faraday effect under conditions of electromagnetically induced transparency at the 5$S_{1/2} \to 5P_{3/2} \to 5D_{5/2}$ two-photon transition in rubidium vapors. These…
We demonstrate for the first time coherent control of bond making, a milestone on the way to coherent control of photo-induced bimolecular chemical reactions. In strong-field multiphoton femtosecond photoassociation experiments, we find the…
As optical two-dimensional coherent spectroscopy (2DCS) is extended to a broader range of applications, it is critical to improve the detection sensitivity of optical 2DCS. We developed a fast phase-cycling scheme in a non-collinear optical…
We present and implement a new scheme for independent control of both the final and the transient population utilizing the symmetry properties of the system. By proper pulse shaping, utilizing the invariance of the two-photon absorption to…
We introduce a new computational approach for femtosecond pulse propagation in the transparency region of gases that permits full resolution in three space dimensions plus time while fully incorporating quantum coherent effects such as…
Two-photon excitation (TPE) proceeds via a "virtual" pathway, which depends on the accessibility of one or more intermediate states, and, in the case of non-centrosymmetric molecules, an additional "dipole" pathway involving the…
We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a…
A theoretical investigation on the quantum control of optical coherent four-wave mixing interactions in two-level systems driven by two intense synchronized femtosecond laser pulses of central angular frequencies $\omega$ and $3\omega$ is…