Related papers: Pure Even Harmonic Generation from Oriented CO in …
We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…
We present single-molecule and macroscopic calculations showing that laser-induced Stark shifts contribute significantly to the phase of high-order harmonics from polar molecules. This is important for orbital tomography, where phases of…
The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…
It is shown that under optimal conditions, the generation of the 3rd, 5th, 7th, and 9th harmonics of the short-wave, ultraviolet or vacuum ultraviolet, laser field by helium atoms is mainly due to transitions between bound states, and the…
We utilize few-level model systems to analyze the polarization and phase properties of below-threshold harmonics generated from aligned molecules. In a two-level system, we find that the phase of emitted harmonics undergoes a distinct…
Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…
In the framework of linear optics, light fields do not interact with each other in a medium. Yet, when their field amplitude becomes comparable to the electron binding energies of matter, the nonlinear motion of these electrons emits new…
The generation of harmonic radiation through a non-linear mechanism driven by bunching at fundamental frequency is an important option in the operation of high gain Free-Electron Lasers (FELs). The use of harmonic generation at a large…
We report the observation of a novel nonlinear optical response from the prototypical three-dimensional topological insulator Bi$_2$Se$_3$ through the process of high-order harmonic generation. We find that the generation efficiency…
Electro-optical modulation of a continuous wave laser is a highly stable way to generate frequency combs, gaining popularity in telecommunication and spectroscopic applications. These combs are generated by modulating non-linear…
We report the first experimental observation of non-adiabatic field-free orientation of a heteronuclear diatomic molecule (CO) induced by an intense two-color (800 and 400 nm) femtosecond laser field. We monitor orientation by measuring…
An all-optical measurement of high-order fractional molecular echoes is demonstrated by using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser pulses, the signatures of full and high order fractional (1/2…
Synchronous extreme ultraviolet (XUV) and single-cycle terahertz (THz) bursts are generated in argon plasma induced by intense two-color femtosecond laser pulses. Correlations between the intensity of the even and odd high-harmonics and the…
High-order harmonic generation by the diffraction of an intense Laguerre-Gaussian (LG) laser beam through a small aperture is studied. It is found that the 2D peripheral electron dynamics on the rim can facilitate complex interplay between…
Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…
Circularly-polarized extreme UV and X-ray radiation provides valuable access to the structural, electronic and magnetic properties of materials. To date, this capability was available only at large-scale X-ray facilities such as…
The optical theorem is applied to the process of electron-positron pair creation in the superposition of a nuclear Coulomb and a strong laser field. We derive new representations for the total production rate as two-fold integrals, both for…
We investigate the second-order non-linear interaction as a means to generate entanglement between fields of differing wavelengths. And show that perfect entanglement can, in principle, be produced between the fundamental and second…
The enhancement and control of non-linear phenomena at a nanometer scale has a wide range of applications in science and in industry. Among these phenomena, high-harmonic generation in solids is a recent focus of research to realize next…
We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…