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We exploit a plasmon mediated two-step momentum downconversion scheme to convert low-energy tunneling electrons into propagating photons. Surface plasmon polaritons (SPPs) propagating along an extended gold nanowire are excited on one end…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Palash Bharadwaj , Alexandre Bouhelier , Lukas Novotny

The junction of a scanning tunneling microscope (STM) operating in the tunneling regime was irradiated with femtosecond laser pulses. A photo-excited hot electron in the STM tip resonantly tunnels into an excited state of a single molecule…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Shiwei Wu , Wilson Ho

We theoretically study the electromagnetic energy transfer between donor and acceptor molecules near a graphene waveguide. The surface plasmons (SPs) supported by the structure provide decay channels which lead to an improvement in the…

Optics · Physics 2019-05-22 Julieta Olivo , Carlos J. Zapata--Rodríguez , Mauro Cuevas

We study the collective electronic excitations in metallic single- and bilayer transition metal dichalcogenides (TMDCs) using time dependent density functional theory in the random phase approximation. For very small momentum transfers…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Kirsten Andersen , Kristian S. Thygesen

Here, we introduce and experimentally demonstrate optical amplification and stimulated emission from a single optically pumped molecular tunneling junction of a scanning tunneling microscope. The gap between a sharp gold tip and a flat gold…

Optics · Physics 2014-01-09 K. Braun , A. M. Kern , X. Wang , H. Adler , H. Peisert , T. Chasse , D. Zhang , A. J. Meixner

Plasmonic catalysis holds significant promise for opening new reaction pathways inaccessible thermally, or for improving the efficiency of chemical processes. However, challenges persist in distinguishing photothermal effects from effects…

A rigorous theory of photon emission accompanied inelastic tunnelling inside the gap of plasmonic nanoantennas has been developed. The disappointingly low efficiency of the electrical excitation of surface plasmon polaritons in these…

The electronic excitation of molecules triggers diverse phenomena such as luminescence and photovoltaic effects, which are the bases of various energy-converting devices. Understanding and control of the excitations at the single-molecule…

Chemical Physics · Physics 2017-07-12 Hiroshi Imada , Kuniyuki Miwa , Miyabi Imai-Imada , Shota Kawahara , Kensuke Kimura , Yousoo Kim

Surface plasmon polaritons (SPPs) propagating along a waveguide working electrode are sensitive to changes in local refractive index, which follow changes in the concentration of reduced and oxidised species near the working electrode. The…

Optics · Physics 2022-06-23 Zohreh Hirbodvash , Elena A. Baranova , Pierre Berini

Excitation of finite chains of magnetic atoms adsorbed on a surface by tunnelling electrons from an STM (Scanning Tunnelling Microscope) tip is studied using a Heisenberg Hamiltonian description of the magnetic couplings along the chain and…

Strongly Correlated Electrons · Physics 2010-10-19 J. P. Gauyacq , N. Lorente

We develop a theory of electron tunneling accompanied by carrier-carrier scattering in graphene - insulator - graphene heterostructures. Due to the dynamic screening of Coulomb interaction, the scattering-aided tunneling is resonantly…

Mesoscale and Nanoscale Physics · Physics 2017-09-29 V. Enaldiev , A. Bylinkin , D. Svintsov

A scanning tunneling microscope (STM) can probe the inelastic spin excitations of single magnetic atoms in a surface via spin-flip assisted tunneling. A particular and intriguing case is the Mn dimer case. We show here that the existing…

Mesoscale and Nanoscale Physics · Physics 2022-08-31 F. Delgado , J. Fernández-Rossier

Surface and volume plasmons excited in a metal cluster by moving electron and corresponding inelastic scattering spectra are studied based on the hydrodynamic approach. Along with the bulk losses traditionally taken into account, the…

Plasma Physics · Physics 2016-04-20 V. B. Gildenburg , V. A. Kostin , I. A. Pavlichenko

The processes of generation of phonons and electron excitations with quantum oriented particle in crystal are considered. Expressions are obtained for the probability of emission of phonons and plasmons with channeled particle. The theory…

Other Condensed Matter · Physics 2015-12-09 Evgeny Mazur

A scanning tunneling microscope (STM) can do more than atomic imaging and manipulation. Its tunneling current can also be used for the excitation of light, converting electron energy to photon energy. STM based single-molecule…

Optics · Physics 2019-01-01 Yao Zhang , Yang Zhang , Zhenchao Dong

We study the energy and momentum of the surface plasmon-polariton (SPP) excited in a symmetric 3-layer "insulator-metal-insulator" structure, which is known to support the symmetric (S) mode with the negative group velocity as well as the…

Optics · Physics 2021-12-30 A. Y. Bekshaev , O. A. Angelsky

Self-oscillators are intriguing due to their ability to sustain periodic motion without periodic stimulus. They remain rare as achieving such behavior requires a balance of energy input, dissipation and non-linear feedback mechanism. Here,…

Optics · Physics 2025-11-03 Riccardo Zinelli , Zijia Wu , Christian A. Nijhuis , Qianqi Lin

We consider a scanning tunneling microscope (STM) such that tunneling occurs through two atomically sharp protrusions on its tip. When the two protrusions are separated by at least several atomic spacings, the differential conductance of…

Condensed Matter · Physics 2009-10-28 Michael E. Flatte' , Jeff M. Byers

The plasmonic tip of a scanning tunnelling microscope (STM) is functionalized with a single fluorescent molecule and is scanned on a plasmonic substrate. The tunneling current flowing through the tip-molecule-substrate junction generates a…

Two possible mechanisms of surface plasmon (SP) oscillations damping in metallic nanoparticles (MNPs), not connected with electron-phonon interaction are investigated theoretically: a) the radiation damping of SP, b) resonant coupling of SP…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Armen Melikyan , Hayk Minassian
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