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Mn doped semiconductors are extremely interesting systems due to their novel magnetic properties suitable for the spintronics applications. It has been shown recently by both theory and experiment that Mn doped GaN systems have a very high…

Materials Science · Physics 2016-08-31 B. Sanyal , O. Bengone , S. Mirbt

We have calculated the chemical trend of magnetic exchange parameters ($J_{dd}$, $N \alpha$, and $N \beta$) of Zn-based II-VI semiconductors ZnA (A=O, S, Se, and Te) doped with Co or Mn. We show that a proper treatment of electron…

Strongly Correlated Electrons · Physics 2015-05-13 T. Chanier , F. Virot , R. Hayn

We calculate the magnetic interactions between two nearest neighbor substitutional magnetic ions (Co or Mn) in ZnO by means of density functional theory and compare it with the available experimental data. Using the local spin density…

Materials Science · Physics 2007-05-23 Thomas Chanier , M. Sargolzaei , I. Opahle , R. Hayn , K. Koepernik

We present an experimental study for polycrystalline samples of the diluted magnetic semiconductor Mn(x)Ga(1-x)N (x<0.04) in order to address some of the existing controversial issues. Different techniques were used to characterize the…

Materials Science · Physics 2018-04-18 A. Furrer , K. W. Kraemer , A. Podlesnyak , V. Pomjakushin , D. Sheptyakov , O. V. Safonova

The magnetism in 12.5% and 25% Mn delta-doped cubic GaN has been investigated using the density-functional theory calculations. The results show that the single-layer delta-doping and half-delta-doping structures show robust ground state…

Materials Science · Physics 2009-01-20 Xingtao Jia , Wei Yang , Minghui Qin , Xinglai Zhang , Xindong Cui , Mingai Sun

Understanding the magnetic properties of the various Mn doping configurations that can be encountered in $2H$-MoS$_2$ monolayer could be beneficial for its use in spintronics. Using density functional theory plus Hubbard U (DFT$+$U)…

Materials Science · Physics 2019-09-04 Adlen Smiri , Iann Gerber , Samir Lounis , Sihem Jaziri

A ferromagnetic coupling between localized Mn spins was predicted in a series of \textit{ab initio} and tight binding calculations and experimentally verified for the dilute magnetic semiconductor Ga$_{1-x}$Mn$_x$N. In the limit of small Mn…

Materials Science · Physics 2020-12-30 D. Sztenkiel , K. Gas , J. Z. Domagala , D. Hommel , M. Sawicki

The properties of diluted Ga$_{1-x}$Mn$_x$As are calculated for a wide range of Mn concentrations within the local spin density approximation of density functional theory. M\"ulliken population analyses and orbital-resolved densities of…

Mesoscale and Nanoscale Physics · Physics 2025-06-10 Stefano Sanvito , Pablo Ordejon , Nicola A. Hill

We present a theoretical study of (Ga,Mn)(As,C) diluted magnetic semiconductors with high C acceptor density that combines insights from phenomenological model and microscopic approaches. A tight-binding coherent potential approximation is…

Materials Science · Physics 2007-05-23 T. Jungwirth , J. Masek , Jairo Sinova , A. H. MacDonald

We investigate the electronic and magnetic properties of Mn-doped CdTe nanocrystals (NCs) with 2 nm in diameter which can be experimentally synthesized with Mn atoms inside. Using the density-functional theory, we consider two doping cases:…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 C. Echeverría-Arrondo , J. Pérez-Conde , A. Ayuela

We study the possibility of d0 ferromagnetism in the compound MgO doped with nitrogen (N). The Haldane-Anderson impurity model is formulated within the tight-binding approximation for determining the host band-structure and the…

Materials Science · Physics 2009-11-13 Bo Gu , Nejat Bulut , Timothy Ziman , Sadamichi Maekawa

The magnetic coupling between doped Mn atoms in clusters as well as crystals of GaN has been studied from first principles using molecular orbital theory for clusters and linearized muffin tin orbitals-tight binding formulation (LMTO-TB)…

Materials Science · Physics 2009-11-07 G. P. Das , B. K. Rao , P. Jena

X-ray diffraction, resistivity, ac susceptibility and magnetization studies on La0.67Ca0.33Mn1-xRuxO3 (0 x < 0.1) were carried out. A significant increase in the lattice parameters indicated the presence of mixed valance state of Ru: Ru3+…

The percentage of substitutional doping of magnetic atoms (Mn) in group-IV-based dilute magnetic semiconductors (DMS) can be increased by co-doping with another conventional electronic dopant (e-dopant) [Zhu et al., Phys. Rev. Lett. 100,…

Materials Science · Physics 2009-06-04 Hua Chen , Wenguang Zhu , Efthimios Kaxiras , Zhenyu Zhang

The sign, magnitude, and range of the exchange couplings between pairs of Mn ions is determined for (Ga,Mn)N and (Ga,Mn)N:Si with x < 3%. The samples have been grown by metalorganic vapor phase epitaxy and characterized by secondary-ion…

Using first-principles density functional theory method, we have investigated the distribution and magnetism of doped Mn atoms in the vicinity of the 3 (112) grain boundary in Ge. We find that at low concentration, the substitutional sites…

Materials Science · Physics 2010-05-24 W. Wang , S. L. Zhang , Z. X. Tian , W. Xiao

Magnetic properties of Ga$_{1-x}$Mn$_x$N are studied theoretically by employing a tight binding approach to determine exchange integrals $J_{ij}$ characterizing the coupling between Mn spin pairs located at distances $R_{ij}$ up to the 16th…

Materials Science · Physics 2014-07-14 C. Simserides , J. A. Majewski , K. N. Trohidou , T. Dietl

After two decades from the discovery of ferromagnetism in Mn-doped GaAs, its origin is still debated, and many doubts are related to the electronic structure. Here we report an experimental and theoretical study of the valence electron…

Strongly Correlated Electrons · Physics 2014-07-29 I. Di Marco , P. Thunström , M. I. Katsnelson , J. Sadowski , K. Karlsson , S. Lebègue , J. Kanski , O. Eriksson

Using ab initio band structure and model calculations we studied magnetic properties of one of the Mn$_4$ molecular magnets (Mn4(hmp)6), where two types of the Mn ions exist: Mn3+ and Mn2+. The direct calculation of the exchange constants…

The mechanism for the ferromagnetic order of (Ga,Mn)As and (Ga,Mn)N is extensively studied over a vast range of Mn concentrations. We calculate the electronic structures of these materials using density functional theory in both the local…

Materials Science · Physics 2009-11-10 Malgorzata Wierzbowska , Daniel Sanchez-Portal , Stefano Sanvito
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