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Single-shot ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics (FDSS) is demonstrated. These kinetics are sampled spectrally using linearly chirped pulses derived from a Ti:sapphire laser. A variable…

Optics · Physics 2007-05-23 Ilya A. Shkrob , Dmitri A. Oulianov , Robert A. Crowell

In this paper, we describe analytically the propagation of Airy-type pulses truncated by a finite-time aperture when second and third order dispersion effects are considered. The mathematical method presented here, based on the…

We demonstrate experimentally the isolation of single attosecond pulses at the carbon K- shell edge in the soft-X-ray water window. Attosecond pulses at photon energies that cover the principal absorption edges of the building blocks of…

Self-steepening of optical pulses arises due the dispersive contribution of the $\chi^{(3)}(\omega)$ Kerr nonlinearity. In typical structures this response is on the order of a few femtoseconds with a fixed frequency response. In contrast,…

Optics · Physics 2015-04-27 Chad Husko , Pierre Colman

The Pixel-Imaging Mass Spectrometry (PImMS) camera allows for 3D charged particle imaging measurements, in which the particle time-of-flight is recorded along with $(x,y)$ position. Coupling the PImMS camera to an ultrafast pump-probe…

Pulse propagation is studied in an EIT medium with the control field having a periodically varying phase (chirp). Based both on numerical calculations and on an approximate approach neglecting absorption and nonadiabatic effects, it is…

Quantum Physics · Physics 2016-08-24 Andrzej Raczynski , Jaroslaw Zaremba , Sylwia Zielinska-Raczynska

The time-resolved electron beam envelope parameters including sectional distribution and position are important and necessary for the study of beam transmission characteristics in the magnetic field and verifying the magnetic field setup…

Accelerator Physics · Physics 2015-02-10 Jiang Xiaoguo , Wang Yuan , Yang Zhiyong , Zhang Huang , Wang Yi , Wei Tao

We have monitored the space-time transformation of 150-fs pulse, undergoing self-focusing and filamentation in water, by means of the nonlinear gating tech- nique. We have observed that pulse splitting and subsequent recombination apply to…

We describe a setup to study ultrafast dynamics in gas-phase molecules using time-resolved photoelectron and photoion spectroscopy. The vacuum ultraviolet (VUV) probe pulses are generated via strong field high-order harmonic generation from…

Atomic and Molecular Clusters · Physics 2014-04-14 Markus Koch , Thomas J. A. Wolf , Jakob Grilj , Emily Sistrunk , Markus Gühr

We have developed a new coherent dedispersion mode to study the emission of Fast Radio Bursts that trigger the voltage capture capability of the Australian SKA Pathfinder (ASKAP) interferometer. In principle the mode can probe emission…

We present the development of a time- and angle-resolved photoemission spectroscopy based on a Yb-based femtosecond laser and a hemispherical electron analyzer. The energy of the pump photon is tunable between 1.4 and 1.9 eV, and the pulse…

Strongly Correlated Electrons · Physics 2020-03-03 Yuanyuan Yang , Tianwei Tang , Shaofeng Duan , Chaocheng Zhou , Duxing Hao , Wentao Zhang

We present a novel, straightforward method for spatiotemporal characterization of ultra-short laser pulses. The method employs far-field interferometry and inverse Fourier transform spectroscopy, built on the theoretical basis derived in…

The collective response of metal nanostructures to optical excitation leads to localized plasmon generation with nanoscale field confinement driving applications in e.g. quantum optics, optoelectronics, and nanophotonics, where a bottleneck…

Coherent manipulation of single-photon wave packets is essentially important for optical quantum communication and quantum information processing. In this paper, we realize controllable splitting and modulation of single-photon-level pulses…

Quantum Physics · Physics 2015-05-13 Sheng-Jun Yang , Xiao-Hui Bao , Jian-Wei Pan

High-energy, few-cycle laser pulses are essential for numerous applications in the fields of ultrafast optics and strong-field physics, due to their ultrafast temporal resolution and high peak intensity. In this work, different from the…

Ultrahigh peak power femtosecond laser pulses create extreme states of matter that are currently being probed with great interest. Plasma optics have been proposed for shaping and amplifying high-power pulses, but they are subject to huge…

Absorption of ultrashort laser pulses in a metallic grating deposited on a transparent sample launches coherent compression/dilatation acoustic pulses in directions of different orders of acoustic diffraction. Their propagation is detected…

Applied Physics · Physics 2018-02-14 Osamu Matsuda , Thomas Pezeril , Ievgeniia Chaban , Kentaro Fujita , Vitalyi Gusev

Frequency-multiplexed quantum communication usually requires a single-shot identification of the frequency mode of a single photon . In this paper, we propose a scheme that can identify the frequency mode with high-resolution even for…

Quantum Physics · Physics 2022-11-04 Daisuke Yoshida , Mayuka Ichihara , Takeshi Kondo , Feng-Lei Hong , Tomoyuki Horikiri

Time-resolved measurements of materials provide a wealth of information on quasiparticle dynamics, and have been the focus of optical studies for decades. In this paper, we develop a theory for explicitly evaluating time-resolved resonant…

Strongly Correlated Electrons · Physics 2019-03-27 Yuan Chen , Yao Wang , Chunjing Jia , Brian Moritz , Andrij M. Shvaika , James K. Freericks , Thomas P. Devereaux