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Motivated by the recent synthesis of two insulating Li$_2$IrO$_3$ polymorphs, where Ir$^{4+}$ $S_{eff}$=1/2 moments form 3D ("harmonic") honeycomb structures with threefold coordination, we study magnetic Hamiltonians on the resulting…

Strongly Correlated Electrons · Physics 2014-11-26 Itamar Kimchi , James G. Analytis , Ashvin Vishwanath

Magnetic moments arranged at the corners of a honeycomb lattice are predicted to form a novel state of matter, Kitaev quantum spin liquid, under the influence of frustration effects between bond-dependent Ising interactions. Some layered…

Strongly Correlated Electrons · Physics 2022-03-09 Sean K. Takahashi , Jiaming Wang , Alexandre Arsenault , Mykola Abramchuk , Fazel Tafti , Philip M. Singer , Takashi Imai

H3LiIr2O6 is the first honeycomb-lattice system without any signs of long-range magnetic order down to the lowest temperatures, raising the hope for the realization of an ideal Kitaev quantum spin liquid. Its honeycomb layers are coupled by…

Strongly Correlated Electrons · Physics 2020-05-13 K. Geirhos , P. Lunkenheimer , M. Blankenhorn , R. Claus , Y. Matsumoto , K. Kitagawa , T. Takayama , H. Takagi , I. Kézsmárki , A. Loidl

We derive and study a spin one-half Hamiltonian on a honeycomb lattice describing the exchange interactions between Ir$^{4+}$ ions in a family of layered iridates $A_2$IrO$_3$ ($A$=Li,Na). Depending on the microscopic parameters, the…

Strongly Correlated Electrons · Physics 2014-11-20 Jiri Chaloupka , George Jackeli , Giniyat Khaliullin

In the field of quantum magnetism, the exactly solvable Kitaev honeycomb model serves as a paradigm for the fractionalization of spin degrees of freedom and the formation of $\mathbb{Z}_2$ quantum spin liquids. An intense experimental…

Strongly Correlated Electrons · Physics 2019-02-07 Ciarán Hickey , Simon Trebst

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

In addition to the Kitaev ($K$) interaction, candidate Kitaev materials also possess Heisenberg ($J$) and off-diagonal symmetric ($\Gamma$) couplings. We investigate the quantum ($S = 1/2$) $K$-$J$-$\Gamma$ model on the honeycomb lattice by…

Strongly Correlated Electrons · Physics 2019-11-14 Jiucai Wang , B. Normand , Zheng-Xin Liu

We study the spin-1/2 Kitaev honeycomb gapless spin liquid in the presence of Stone-Wales-type local lattice defects with odd-sided plaquettes. While the clean Kitaev model has no finite-temperature phase transitions, we find that…

Strongly Correlated Electrons · Physics 2026-05-05 Arnab Seth , Fay Borhani , Itamar Kimchi

Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim

We report the discovery of a novel gapless quantum spin liquid in the S=1 honeycomb system Cu$_3$LiRu$_2$O$_6$ with Ru$^{4+}$ ($4d^4$) where moments remain dynamic down to 50 mK. Heat capacity measurements show no sign of magnetic ordering…

The exactly solvable spin-1/2 Kitaev model on a honeycomb lattice has drawn significant interest, as it offers a pathway to realizing the long-sought after quantum spin liquid. Building upon the Kitaev model, Yao and Lee introduced another…

Strongly Correlated Electrons · Physics 2025-03-12 Derek Churchill , Emily Z. Zhang , Hae-Young Kee

Quantum spin liquid involves fractionalized quasipariticles such as spinons and visons. They are expressed as itinerant Majorana fermions and $Z_2$ fluxes in the Kitaev model with bond-dependent exchange interactions on a honeycomb spin…

Strongly Correlated Electrons · Physics 2020-02-05 Y. Nagai , T. Jinno , Y. Yoshitake , J. Nasu , Y. Motome , M. Itoh , Y. Shimizu

A decade ago, Alexei Kitaev proposed an exactly solvable $S$ = 1/2 model on a two-dimensional honeycomb lattice, where the spins fractionalize into Majorana fermions and form a topological quantum spin liquid (QSL) in the ground state. It…

Strongly Correlated Electrons · Physics 2022-01-21 Hidenori Takagi , Tomohiro Takayama , George Jackeli , Giniyat Khaliullin , Stephen E. Nagler

We report discovery of a new iridate family K$_x$Ir$_y$O$_2$ with depleted triangular lattice planes made up of edge sharing IrO$_6$ octahedra separated by K planes. Such a material interpolates between the triangular and honeycomb lattices…

Strongly Correlated Electrons · Physics 2019-08-23 Kavita Mehlawat , Yogesh Singh

There have been tremendous experimental and theoretical efforts toward discovery of quantum spin liquid phase in honeycomb-based-lattice materials with strong spin-orbit coupling. Here the bond-dependent Kitaev interaction between local…

Strongly Correlated Electrons · Physics 2016-12-23 Heung-Sik Kim , Yong Baek Kim , Hae-Young Kee

Motivated by recent experiments on $\beta-$Li$_2$IrO$_3$, we study the phase diagram of the Heisenberg-Kitaev model on a three dimensional lattice of tri-coordinated Ir$^{4+}$, dubbed the hyperhoneycomb lattice by Takagi et. al. The lattice…

Strongly Correlated Electrons · Physics 2014-01-22 Eric Kin-Ho Lee , Robert Schaffer , Subhro Bhattacharjee , Yong Baek Kim

We present numerical evidence for the presence of a finite-temperature ($T$) phase transition separating paramagnet and quantum spin liquid in a three-dimensional variant of the Kitaev model defined on a hyperhoneycomb lattice in the limit…

Strongly Correlated Electrons · Physics 2015-06-17 J. Nasu , T. Kaji , K. Matsuura , M. Udagawa , Y. Motome

The recently discovered three-dimensional hyperhoneycomb iridate, $\beta$-Li$_2$IrO$_3$, has raised hopes for the realization of dominant Kitaev interaction between spin-orbit entangled local moments due to its near-ideal lattice structure.…

Strongly Correlated Electrons · Physics 2016-01-15 Heung-Sik Kim , Eric Kin-Ho Lee , Yong Baek Kim

The spin liquid phase is one of the prominent strongly interacting topological phases of matter whose unambiguous confirmation is yet to be reached despite intensive experimental efforts on numerous candidate materials. Recently, a new…

Strongly Correlated Electrons · Physics 2018-05-10 Andrei Catuneanu , Youhei Yamaji , Gideon Wachtel , Yong Baek Kim , Hae-Young Kee

Recent numerical studies indicate that the antiferromagnetic Kitaev honeycomb lattice model undergoes a magnetic-field-induced quantum phase transition into a new spin-liquid phase. This intermediate-field phase has been previously…

Strongly Correlated Electrons · Physics 2022-03-02 Shang-Shun Zhang , Gábor B. Halász , Cristian D. Batista
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