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We present a theoretical approach to include dynamical aspects of molecular structural fluctuations, such as, for example, forming and breaking hydrogen bonds, isomerizations, and dynamical supramolecular structures, in nonequilibrium…

Mesoscale and Nanoscale Physics · Physics 2022-10-18 Daniel S. Kosov

We develop a time dependent second order Green's function theory (GF2) for calculating neutral excited states in molecules. The equation of motion for the lesser Green's function (GF) is derived within the adiabatic approximation to the…

Chemical Physics · Physics 2022-01-19 Wenjie Dou , Joonho Lee , David R. Reichman , Roi Baer , Eran Rabani

Quantization of electrodynamics in curved space-time in the Lorenz gauge and with arbitrary gauge parameter makes it necessary to study Green functions of non-minimal operators with variable coefficients. Starting from the integral…

High Energy Physics - Theory · Physics 2009-11-10 Giuseppe Bimonte , Enrico Calloni , Luciano Di Fiore , Giampiero Esposito , Leopoldo Milano , Luigi Rosa

We present a solution to the problem of AC current partition in a multi-probe mesoscopic conductor within the nonequilibrium Green's function formalism. This allows the derivation of dynamic conductance which is appropriate for…

Condensed Matter · Physics 2009-10-31 Baigeng Wang , Jian Wang , Hong Guo

The Green-Kubo formula for linear response coefficients gets modified when dealing with nonequilibrium dynamics. In particular negative differential conductivities are allowed to exist away from equilibrium. We give a unifying framework for…

Statistical Mechanics · Physics 2013-11-12 Pieter Baerts , Urna Basu , Christian Maes , Soghra Safaverdi

Non-equilibrium Greens function techniques (NEGF) combined with Density Functional Theory (DFT) calculations have become a standard tool for the description of electron transport through single molecule nano-junctions in the coherent…

Materials Science · Physics 2009-11-13 R. Stadler , V. Geskin , J. Cornil

I review the quantum theory of the electron moving in a random environment. First, the quantum mechanics of individual particles scattered on a random potential is discussed. The quantum-mechanical description is extended to many-body…

Disordered Systems and Neural Networks · Physics 2021-09-13 Václav Janiš

The coupling of the charge carriers passing through a molecule bridging two bulky conductors with local vibrational modes of the molecule, gives rise to distinct features in the electronic transport properties on one hand, and to…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 A. Ueda , Y. Utsumi , Y. Tokura , O. Entin-Wohlman , A. Aharony

We have implemented time-propagation of the non-equilibrium Green function for atoms and molecules, by solving the Kadanoff-Baym equations within a conserving self-energy approximation. We here demonstrate the usefulnes of time-propagation…

Materials Science · Physics 2007-05-23 Nils Erik Dahlen , Robert van Leeuwen

We calculate the time-dependent non-linear transport current through an interacting quantum dot in the single-electron tunneling regime (SET). We show that an additional dc current is generated by the electron-electron interaction by…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Felix Reckermann , Janine Splettstoesser , Maarten R. Wegewijs

We show that the Green's functions in non-linear gauge in the theory of perturbative quantum gravity is expressed as a series in terms of those in linear gauges. This formulation is also holds for operator Green's functions. We further…

High Energy Physics - Theory · Physics 2015-07-22 Sudhaker Upadhyay , Bhabani Prasad Mandal

A method for deriving quantum kinetic equations with initial correlations is developed on the basis of the nonequilibrium Green's function formalism. The method is applicable to a wide range of correlated initial states described by…

Statistical Mechanics · Physics 2009-10-31 V. G. Morozov , G. Röpke

While the vast majority of calculations reported on molecular conductance have been based on the static non-equilibrium Green's function formalism combined with density functional theory, in recent years a few time-depedent approaches to…

We present consistent results for molecular conduction using two central-complementary approaches: the non-equilibrium Green's function technique and the quantum master equation method. Our model describes electronic conduction in a…

Mesoscale and Nanoscale Physics · Physics 2016-04-13 Bijay Kumar Agarwalla , Dvira Segal

The objective of this paper is to describe a simple phenomenological approach for including incoherent dephasing processes in quantum transport models. The presented illustrative numerical results show this model provides the flexibility of…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Roksana Golizadeh-Mojarad , Supriyo Datta

We present a combined theoretical approach to study the nonequilibrium transport properties of nanoscale systems coupled to metallic electrodes and exhibiting strong electron-phonon interactions. We use the Keldysh Green function formalism…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 R. C. Monreal , F. Flores , A. Martin-Rodero

We develop a theory for charge and spin current between two canted magnetic leads flowing through a quantum dot with an arbitrary local interaction. For a noncollinear magnetic configuration, we calculate equilibrium and nonequilibrium…

Mesoscale and Nanoscale Physics · Physics 2014-12-16 Silas Hoffman , Yaroslav Tserkovnyak

Theory of non-equilibrium Green's function (NGF) provides a practical framework for studying quantum many-body systems out of equilibrium. Extending the previous mean field approach developed for nuclear systems in one dimension with NGF,…

Nuclear Theory · Physics 2020-08-26 Hao Lin , Hossein Mahzoon , Arnau Rios , Pawel Danielewicz

We describe microscopic theory for the quantum transport through finite interacting systems connected to noninteracting leads. It can be applied to small systems such as quantum dots, quantum wires, atomic chain, molecule, and so forth. The…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Akira Oguri

We address theoretically adiabatic regime of charge transport for a model of two tunnel-coupled quantum dots connected in series. The energy levels of the two dots are harmonically modulated by an external potential with a constant phase…

Mesoscale and Nanoscale Physics · Physics 2008-12-18 Vyacheslavs Kashcheyevs