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Recent experimental evidence that fluorinated graphene creates local magnetic moments around F adatoms has not been supported by semilocal density-functional theory (DFT) calculations where the adsorption of an isolated F adatom induces no…

Mesoscale and Nanoscale Physics · Physics 2013-06-03 Hyun-Jung Kim , Jun-Hyung Cho

The issue of whether local magnetic moments can be formed by introducing adatoms into graphene is of intense research interest because it opens the window to fundamental studies of magnetism in graphene, as well as of its potential…

Mesoscale and Nanoscale Physics · Physics 2012-06-12 X. Hong , K. Zou , B. Wang , S. -H. Cheng , J. Zhu

We address the interaction of graphene with 3d transition metal adatoms and the formation of localized magnetic moments by means of first-principles calculations. By comparing calculations within the generalized gradient approximation (GGA)…

Strongly Correlated Electrons · Physics 2011-12-14 T. O. Wehling , A. I. Lichtenstein , M. I. Katsnelson

The electronic structure of selected rare-earth atoms adsorbed on a free-standing graphene was investigated using methods beyond the conventional density functional theory (DFT+U, DFT+HIA and DFT+ED). The influence of the electron…

Strongly Correlated Electrons · Physics 2016-09-12 Agnieszka L. Kozub , Alexander B. Shick , Frantisek Maca , Jindrich Kolorenc , Alexander I. Lichtenstein

Using magnetization measurements, we show that point defects in graphene - fluorine adatoms and irradiation defects (vacancies) - carry magnetic moments with spin 1/2. Both types of defects lead to notable paramagnetism but no magnetic…

Mesoscale and Nanoscale Physics · Physics 2012-05-23 R. R. Nair , M. Sepioni , I-Ling Tsai , O. Lehtinen , J. Keinonen , A. V. Krasheninnikov , T. Thomson , A. K. Geim , I. V. Grigorieva

We investigate the effect of an applied uniaxial strain on the ferromagnetic instability due to long- range Coulomb interaction between Dirac fermions in graphene. In case of undeformed graphene the ferromagnetic exchange instability occurs…

Strongly Correlated Electrons · Physics 2013-04-30 Anand Sharma , Valeri N. Kotov , Antonio H. Castro Neto

The electronic properties of graphene decorated with Ni, Co, Cu and Zn adatoms is studied with the density functional theory approach. Within the analysis the spin-orbit interaction is taken into account. We focus on the case when the…

Applied Physics · Physics 2019-03-01 Malgorzata Wawrzyniak-Adamczewska

Rare-earth (RE) atoms on top of 2D materials represent an interesting platform with the prospect of tailoring the magnetic anisotropy for practical applications. Here, we investigate the ground state and magnetic properties of selected…

Mesoscale and Nanoscale Physics · Physics 2024-07-25 Johanna P. Carbone , Juba Bouaziz , Gustav Bihlmayer , Stefan Blügel

We show that, in graphene with a small concentration of adatoms, the total magnetic moment $\mu_T$ can be switched on and off by varying the Fermi energy $E_F$, either by applying a gate voltage or by suitable chemical doping. Our…

Mesoscale and Nanoscale Physics · Physics 2014-08-08 N. A. Pike , D. Stroud

Graphene consists in a single-layer carbon crystal where 2$p_z$ electrons display a linear dispersion relation in the vicinity of the Fermi level, conveniently described by a massless Dirac equation in $2+1$ spacetime. Spin-orbit effects…

Mesoscale and Nanoscale Physics · Physics 2017-04-04 B. Berche , F. Mireles , E. Medina

We conduct a theoretical examination of the electronic and magnetic characteristics of end-modified 7-atom wide armchair graphene nanoribbons (AGNRs). Our investigation is performed within the framework of a single-band Hubbard model,…

Mesoscale and Nanoscale Physics · Physics 2025-03-21 Antoine Honet , Luc Henrard , Vincent Meunier

Motivated by recent studies reporting the formation of localized magnetic moments in doped graphene, we investigate the energetic cost for spin polarizing isolated impurities embedded in this material. When a well-known criterion for the…

Materials Science · Physics 2015-05-14 P. Venezuela , R. B. Muniz , A. T. Costa , D. M. Edwards , S. R. Power , M. S. Ferreira

By applying tight binding model of adatoms in graphene, we study theoretically the localized aspects of the interaction between transition metal atoms and graphene. Considering the electron-electron interaction by adding a Hubbard term in…

Strongly Correlated Electrons · Physics 2018-06-14 F. Escudero , J. S. Ardenghi , L. Sourrouille , P. Jasen , A. Juan

We investigate the electronic and magnetic properties of graphene channels ($2$--$4$~nm wide) embedded within fluorographene, focusing on two distinct interfaces: the fully fluorinated $\alpha$ interface and the half-fluorinated $\beta$…

Mesoscale and Nanoscale Physics · Physics 2024-10-01 R. M. Guzmán-Arellano , A. D. Hernández-Nieves , F. M. Peeters , Gonzalo Usaj

We examine the conditions necessary for the presence of localized magnetic moments on adatoms with inner shell electrons in graphene. We show that the low density of states at the Dirac point, and the anomalous broadening of the adatom…

Strongly Correlated Electrons · Physics 2008-07-13 Bruno Uchoa , Valeri N. Kotov , N. M. R. Peres , A. H. Castro Neto

We present a theoretical study of the optical conductivity of graphene with magnetic and nonmagnetic adatoms. First, by introducing alternating potential in a pure graphene, we demonstrate a gap formation in the density of states and the…

Strongly Correlated Electrons · Physics 2015-01-13 Muhammad Aziz Majidi , Syahril Siregar , Andrivo Rusydi

At the heart of current information nanotechnology lies the search for ideal platforms hosting the smallest possible magnets, i.e. single atoms with magnetic moments pointing out-of-plane, as requested in a binary-type of memory. For this…

Graphene is a unique two-dimensional material with rich new physics and great promise for applications in electronic devices. Physical phenomena such as the half-integer quantum Hall effect and high carrier mobility are critically dependent…

Graphene is a highly promising material in the field of spin electronics. Recent experiments on electron spin resonance have observed a reduction in the g-factor of graphene. In our previous paper [J. Phys. Soc. Jpn. 88, 094707 (2019)], we…

Materials Science · Physics 2021-10-04 Amit Shrestha , Katsuhiko Higuchi , Shunsuke Yoshida , Masahiko Higuchi

We study RKKY interactions between local magnetic moments for both doped and undoped graphene. We find in both cases that the interactions are primarily ferromagnetic for moments on the same sublattice, and antiferromagnetic for moments on…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 L. Brey , H. A. Fertig , S. Das Sarma
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