English
Related papers

Related papers: Assessing Excited State Energy Gaps with Time-Depe…

200 papers

We propose a new method of calculating electronically excited states that combines a density functional theory (DFT) based ground state calculation with a linear response treatment that employs approximations used in the time-dependent…

Chemical Physics · Physics 2016-05-11 Robert Rüger , Erik van Lenthe , Thomas Heine , Lucas Visscher

In this paper benchmark results are presented on the calculation of vertical electronic excitation energies using a long-range second-order polarisation propagator approximation (SOPPA) description with a short-range density functional…

Chemical Physics · Physics 2025-09-24 Juliane H. Fuglsbjerg , Dániel Nagy , Hans Jørgen Aa. Jensen , Stephan P. A. Sauer

Density functional calculations are performed for twelve $2l2l'$n$l"$ (n$\geq$2) triply excited hollow resonance series of Li, {\em viz.,} 2s$^2$ns $^2$S$^e$, 2s$^2$np $^2$P$^o$, 2s$^2$nd $^2$D$^e$, 2p$^2$ns $^2$D$^e$,$^4$P$^e$, 2s2pns…

Chemical Physics · Physics 2015-06-16 Amlan K. Roy

Semi-local density functionals for the exchange-correlation energy of electrons are extensively used as it produce realistic and accurate results for finite and extended systems. The choice of techniques play crucial role in constructing…

Materials Science · Physics 2017-11-01 Subrata Jana , Prasanjit Samal

Energy levels and transition rates for electric-dipole, electric-quadrupole, electric-octupole, magnetic-dipole, and magnetic-quadrupole transitions among the levels arising from the $n\ \leq$ 5 configurations in B-like Kr XXXII are…

Atomic Physics · Physics 2020-05-20 Yanting Li , Ra Si , Jinqing Li , Chunyu Zhang , Ke Yao , Kai Wang , Mingfeng Gu , Chongyang Chen

This chapter gives an introduction to qualitative and quantitative topological analyses of molecular electronic transitions. Among the possibilities for qualitatively describing how the electronic structure of a molecule is reorganized upon…

Chemical Physics · Physics 2018-11-27 Thibaud Etienne

We use the density functional method to examine the properties of the nonuniform (two-phase) fluid of two-level atoms, a part of which is excited. Basing on the analysis of the equation of state of a gas of two-level atoms, a part of which…

Soft Condensed Matter · Physics 2007-05-23 Oleg Derzhko , Vasyl Myhal

We introduce an orbital free electron density functional approximation based on alchemical perturbation theory. Given convergent perturbations of a suitable reference system, the accuracy of popular self-consistent Kohn-Sham density…

Chemical Physics · Physics 2020-05-27 Guido Falk von Rudorff , O. Anatole von Lilienfeld

We present an approach based on density-functional theory for the calculation of fundamental gaps of both finite and periodic two-dimensional (2D) electronic systems. The computational cost of our approach is comparable to that of total…

Materials Science · Physics 2021-08-11 Alberto Guandalini , Alice Ruini , Esa Räsänen , Carlo Andrea Rozzi , Stefano Pittalis

We investigate the time an electronic excitation travels in a supermolecular setup using a measurement process in an open quantum-system framework. The approach is based on the stochastic Schr\"odinger equation and uses a Hamiltonian from…

Materials Science · Physics 2013-12-09 Dirk Hofmann , Heiko Appel , Massimiliano Di Ventra , Stephan Kümmel

We demonstrate that, rather than resorting to high-cost dynamic correlation methods, qualitative failures in excited-state potential energy surface predictions can often be remedied at no additional cost by ensuring that optimal molecular…

Chemical Physics · Physics 2020-06-18 Lan Nguyen Tran , Eric Neuscamman

We study the energy spectrum of a system of localized states coupled to a 2D electron gas in strong magnetic field. If the energy levels of localized states are close to the electron energy in the plane, the system exhibits a kind of…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 T. V. Shahbazyan , S. E. Ulloa

Excitation energies and transition probabilities of the first $2^+$ excitations in even tin and lead isotopes as well as the quadrupole moments of odd neighbors of these isotopes are calculated within the self-consistent Theory of Finite…

Nuclear Theory · Physics 2013-05-29 S. V. Tolokonnikov , S. Kamerdzhiev , D. Voytenkov , S. Krewald , E. E. Saperstein

We compute energy gaps for spin-polarized fractional quantum Hall states in the lowest Landau level at filling fractions nu=1/3, 2/5,3/7 and 4/9 using exact diagonalization of systems with up to 16 particles and extrapolation to the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. H. Morf , N. d'Ambrumenil , S. Das Sarma

Ca$_{3}$Ru$_{2}$O$_{7}$ is a fascinating material that displays physical properties governed by spin-orbit interactions and structural distortions, showing a wide range of remarkable electronic phenomena. Here, we present a…

Materials Science · Physics 2023-10-23 A. M León , J. W. González , H. Rosner

We report a local, weight-dependent correlation density-functional approximation that incorporates information about both ground and excited states in the context of density-functional theory for ensembles (eDFT). This density-functional…

Chemical Physics · Physics 2020-06-05 Pierre-François Loos , Emmanuel Fromager

We present a spin-dependent localized Hartree-Fock (SLHF) density-functional approach for the treatment of the inner-shell excited-state calculation of atomic systems. In this approach, the electron spin-orbitals in an electronic…

Atomic Physics · Physics 2009-11-11 Zhongyuan Zhou , Shih-I Chu

Motivated by neutral excitations in disordered electronic materials and systems of trapped ultracold particles with long-range interactions, we study energy-level statistics of quasiparticles with the power-law hopping Hamiltonian $\propto…

Disordered Systems and Neural Networks · Physics 2018-07-25 Paraj Titum , Victor L. Quito , Sergey V. Syzranov

A combination of classical molecular dynamics (MM/MD) and quantum chemical calculations based on the density functional theory (DFT) was performed to describe conformational properties of diphenylethyne (DPE), methylated-DPE and poly para…

Mesoscale and Nanoscale Physics · Physics 2016-12-21 Behnaz Bagheri , Björn Baumeier , Mikko Karttunen

Analytic potentials are built for all four $^{2S+1}\Pi_{u/g}$ states of Li$_{2}$ dissociating to Li$(2S)$ + Li$(3P)$: $3b(3^{3}\Pi_{u})$, $3B(3^{1}\Pi_{u})$, $3C(3^{1}\Pi_{g}),$ and $3d(3^{3}\Pi_{g})$. These potentials include the effect of…

Chemical Physics · Physics 2015-09-24 Nikesh S. Dattani