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We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

Atomic Physics · Physics 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

The process of nonsequential two-photon double ionization of helium is studied by two complementary numerical approaches. First, the time-dependent Schr{\"o}dinger equation is solved and the final wave function is analyzed in terms of…

Quantum Physics · Physics 2010-09-13 Sølve Selstø , Tore Birkeland , Simen Kvaal , Raymond Nepstad , Morten Førre

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…

Atomic Physics · Physics 2021-06-02 Yimeng Wang , Chris H. Greene

We illustrate how attosecond light pulses can be used to directly mapping out the time-dependence of the correlated motion of two excited atomic electrons, discuss how the two-electron correlations manifest themselves in realistic…

Atomic Physics · Physics 2007-05-23 Toru Morishita , Shinichi Watanabe , C. D. Lin

We have developed a perturbative method to model the resonant ionization of atomic systems in fluctuating laser fields. The perturbative method is based on an expansion in terms of the multitime cumulants, a suitable combination of moments…

Atomic Physics · Physics 2020-11-25 Tejaswi Katravulapally , L. A. A. Nikolopoulos

The autocorrelation function, A(t), measures the overlap (in Hilbert space) of a time-dependent quantum mechanical wave function, psi(x,t), with its initial value, psi(x,0). It finds extensive use in the theoretical analysis and…

Quantum Physics · Physics 2009-11-10 R. W. Robinett , L. C. Bassett

We consider the two-photon ionization of Hydrogen-like atoms. We find an approximate expression of the long-range phase based on an asymptotic expansion of the continuum eigenfunctions within the Wentzel-Kramers-Brillouin approximation.…

Ionization is a fundamental process in intense laser-matter interactions, and is known to cause plasma defocusing and intensity clamping. Here, we investigate theoretically the propagation dynamics of an intense laser pulse in a helium gas…

Optics · Physics 2020-11-25 Xiaohui Gao , Bonggu Shim

A theoretical investigation of the radiative capture of an electron into a bound state of heavy, hydrogen-like ion is presented. Special attention is paid to the question of how the linear polarization of the emitted radiation is affected…

Atomic Physics · Physics 2015-05-28 A. Surzhykov , A. N. Artemyev , V. A. Yerokhin

We investigate the angle-resolved photoelectron spectra from laser-assisted photoionization for helium and neon atoms using an \textit{ab initio} method based on time-dependent surface flux and configuration interaction singles. We find…

Atomic Physics · Physics 2020-08-26 Mattias Bertolino , David Busto , Felipe Zapata , Jan Marcus Dahlström

Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process. In this work, we investigate this multiplexing via computation of the…

Atomic Physics · Physics 2016-05-30 Paul Hockett , Matthias Wollenhaupt , Thomas Baumert

During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we…

Atomic Physics · Physics 2020-02-19 Benjamin Willenberg , Jochen Maurer , Benedikt W. Mayer , Ursula Keller

When intense light irradiates a quantum system, an ionizing electron recollides with its parent ion within the same light cycle and, during that very brief (few femtosecond) encounter, its kinetic energy sweeps from low to high energy and…

Atomic Physics · Physics 2020-10-13 Graham G. Brown , Dong Hyuk Ko , Chunmei Zhang , P. B. Corkum

We present accurate time-dependent ab initio calculations on fully differential and total integrated (generalized) cross sections for the nonsequential two-photon double ionization of helium at photon energies from 40 to 54 eV. Our…

Atomic Physics · Physics 2008-05-07 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

Atomic Physics · Physics 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

Few-photon induced breakup of helium is studied using a newly developed ab initio numerical framework for solving the six-dimensional time-dependent Schroedinger equation. We present details of the method and calculate (generalized) cross…

Atomic Physics · Physics 2010-06-11 R. Nepstad , T. Birkeland , M. Førre

Photoionization of atoms by high-order harmonics in the presence of a laser may lead to quantum interference from which information about the photoionization dynamics or the light fields can be extracted. Traditionally, this interference…

Reionization is a process whereby hydrogen (and helium) in the Universe is ionized by the radiation from first luminous sources. Theoretically, the importance of the reionization lies in its close coupling with the formation of first cosmic…

Cosmology and Nongalactic Astrophysics · Physics 2014-11-18 T. Roy Choudhury

The analysis of the spatiotemporal picture of particle radiation in relativistic heavy-ion collisions in terms of correlation femtoscopy scales, emission and source functions allows one to probe the character of evolution of the system…

Nuclear Theory · Physics 2023-10-26 Yu. M. Sinyukov , V. M. Shapoval , M. D. Adzhymambetov
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