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The tin sulfides represent a materials platform for earth-abundant semiconductor technologies. We present a first-principles study of the five known and proposed phases of SnS together with SnS2 and Sn2S3. Lattice-dynamics techniques are…

Materials Science · Physics 2017-03-17 Jonathan M. Skelton , Lee A. Burton , Fumiyasu Oba , Aron Walsh

Sn(1-x)In(x)Te is a possible candidate for topological superconductivity. Previous work has shown that substitution of In for Sn in the topological crystalline insulator SnTe results in superconductivity, with the transition temperature,…

Superconductivity · Physics 2013-07-29 R. D. Zhong , J. A. Schneeloch , X. Y. Shi , Z. J. Xu , C. Zhang , J. M. Tranquada , Q. Li , G. D. Gu

Since there is both strong electron-phonon coupling during a ferroelectric/FE transition and superconducting/SC transition, it has been an important topic to explore superconductivity from the FE instability. Sn$_2$P$_2$Se$_6$ arouses broad…

Superconductivity · Physics 2024-02-27 He Zhang , Wei Zhong , Xiaohui Yu , Binbin Yue , Fang Hong

Synchrotron X-ray diffraction and Raman spectroscopy have been used to study chemical reactions of molecular hydrogen (H2) with sulfur (S) at high pressures. We find theoretically predicted Cccm and Im-3m H3S to be the reaction products at…

Superconductivity · Physics 2017-04-19 Alexander F. Goncharov , Sergey S. Lobanov , Vitali B. Prakapenka , Eran Greenberg

Tin sulfide (SnS) was successfully synthesized in single crystals by a melt and slow-cooling method. The obtained sample was characterized by an X-ray diffraction, an energy dispersive spectrometry, and an X-ray photoelectron spectroscopy.…

Silicon undergoes a phase transition from the semiconducting diamond phase to the metallic beta-Sn phase under pressure. We use quantum Monte Carlo calculations to predict the transformation pressure and compare the results to density…

Materials Science · Physics 2014-04-23 R. G. Hennig , A. Wadehra , K. P. Driver , W. D. Parker , C. J. Umrigar , J. W. Wilkins

The compression of SH$_2$ and its subsequent decomposition to SH$_3$, presumably in a cubic Im$\overline{3}$m structure, has lead to the discovery of conventional superconductivity with the highest measured and confirmed $T_c$ to date, 203…

Materials Science · Physics 2019-02-20 Maximilian Amsler

Binary tin sulfides are appealing because of their simple stoichiometry and semiconducting properties and are potentially cost-effective optoelectronic materials. The multivalency of Sn allows yet more intermediate compositions,…

Materials Science · Physics 2019-04-30 Xueting Wang , Zhun Liu , Xin-Gang Zhao , Jian Lv , Koushik Biswas , Lijun Zhang

The high-pressure behavior of silicon telluride (Si2Te3), a two-dimensional (2D) layered material, was investigated using synchrotron X-ray powder diffraction in a diamond anvil cell to 11.5 GPa coupled with first-principles theory. Si2Te3…

Materials Science · Physics 2024-10-10 Bohan Li , Frank Cerasoli , Ethan Chen , Martin Kunz , Davide Donadio , Kristie J. Koski

Density functional theory based study of the pressure dependent physical properties of binary SnS compound has been carried out. The computed elastic constants reveal that SnS is mechanically stable and brittle under ambient conditions.…

Materials Science · Physics 2022-10-31 Ayesha Tasnim , Md. Mahamudujjaman , Md. Asif Afzal , R. S. Islam , S. H. Naqib

The transition metal dichalcogenide $1T$-TiSe$_2$ is a quasi-two-dimensional layered material with a phase transition towards a commensurate charge density wave (CDW) at a critical temperature T$_{c}\approx 200$K. The relationship between…

The existence of second-order structural phase transition in the SnS at a pressure of 16 GPa has been proved theoretically. The calculation is performed using the plane-wave pseudopotential approach to density-functional theory within the…

Materials Science · Physics 2015-06-19 F. M. Hashimzade , D. A. Huseinova , Z. A. Jahangirli , B. H. Mehdiyev

Candidates for new thermoelectric and superconducting materials, which have narrow band gap and flat bands near band edges, were searched by the high-throughput first-principles calculation from an inorganic materials database. The…

We report the characterization of the misfit compound (Pb1-xSnxSe2)1.16(TiSe2)2, in which a [100] rocksalt bilayer of Pb1-xSnxSe, which is a topological crystalline insulator in bulk form, alternates with a double layer of the normally…

Superconductivity · Physics 2016-05-25 Huixia Luo , Kai Yan , Weiwei Xie , Brendan F. Phelan , R. J. Cava

SnSe monolayers experience a temperature induced two-dimensional Pnm2$_1 \to$ P4/nmm structural transformation precipitated by the softening of vibrational modes. The standard theoretical treatment of thermoelectricity---which relies on a…

Materials Science · Physics 2021-01-22 John W. Villanova , Salvador Barraza-Lopez

Polycrystalline Sb 2 Te 3-x Se x (0.0 < x < 1.0) samples were synthesized by the solid state reaction method. The structural analysis showed that up to the maximal concentration of Se, the samples possess the Rhombohedral crystal symmetry…

Exploring the chemistry of materials at high pressures has lead to the discovery of previously unknown exotic compounds. Here, we systematically search for all thermodynamically stable Sr-C compounds under pressure (up to 100 GPa) using the…

Materials Science · Physics 2025-06-30 Nikita Rybin , Evgeny Moerman , Pranab Gain , Artem R. Oganov , Alexander Shapeev

A systematic ab initio search for low enthalpy phases of disilane (Si_2H_6) at high pressures was performed based on the minima hopping method. We found a novel metallic phase of disilane with Cmcm symmetry, which is enthalpically more…

Iron-chalcogenide superconductor Fe$_{1.03}$Se$_{0.5}$Te$_{0.5}$ has been investigated under high pressure using synchrotron based x-ray diffraction and mid-infrared reflectance measurements at room temperature. Pressure dependence of the…

Materials Science · Physics 2013-08-16 Pallavi S. Malavi , S. Karmakar , N. N. Patel , Surinder M. Sharma

Recent experiments showed the distinct observations on the transition metal ditelluride NiTe$_2$ under pressure: one reported a superconducting phase transition at 12 GPa, whereas another observed a sign reversal of Hall resistivity at 16…

Superconductivity · Physics 2021-07-14 Jian-Feng Zhang , Yawen Zhao , Kai Liu , Yi Liu , Zhong-Yi Lu