Related papers: Optical chirality in high harmonic generation
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
Vectorial nonlinear optics refers to the investigation of optical processes whose nonlinear polarization (NP) undergoes spin-orbit coupling (SOC) interactions where, in general, the driving light field or the new field generated by the…
We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…
Chirality is a universal feature in nature, as observed in fermion interactions and DNA helicity. Much attention has been given to chiral interactions of light, not only regarding its physical interpretation but also focusing on intriguing…
For paraxial light beams and electromagnetic fields, the Stokes vector and polarization matrix provide equivalent scalar measures of optical chirality, widely used in linear optics. However, growing interest in non-paraxial fields, with…
Chirality is a ubiquitous phenomenon in the natural world. Many biomolecules without inversion symmetry such as amino acids and sugars are chiral molecules. Measuring and controlling molecular chirality at a high precision down to the…
Chiral optical effects are generally quantified along some specific incident directions of exciting waves (especially for extrinsic chiralities of achiral structures) or defined as direction-independent properties by averaging the responses…
We systematically investigate the generation of optical chirality patterns by applying the superposition of two waves in three scenarios, namely plane waves in free space, evanescent waves of totally reflected light at dielectric interface…
Chiral nonlinear response has been explored for decades due to its extreme sensitivity to molecular and structural dissymmetry. Conventional approaches often require bulky systems and produce only static nonlinear chirality. Here, we report…
Molecular chirality is conventionally understood as space-inversion-symmetry breaking in the equilibrium structure of molecules. Less well known is that achiral molecules can be made chiral through extreme rotational excitation. Here, we…
The phenomenon of molecular optical activity manifests itself as the rotation of the plane of linear polarization when light passes through chiral media. Measurements of optical activity and its wavelength dependence, optical rotatory…
Chirality is a fundamental concept in physics that underpins various phenomena in nonlinear optics, quantum physics, and topological photonics. Although the spin of a photon naturally brings chirality, orbital angular momentum can also…
Synthetic chiral light enables ultrafast and highly efficient imaging of molecular chirality. Unlike standard circularly polarized light, the handedness of synthetic chiral light does not rely on the spatial structure of the light field: it…
Chirality is a fundamental asymmetry phenomenon, with chiral optical elements exhibiting asymmetric response in reflection or absorption of circularly polarized light. Recent realizations of such elements include nanoplasmonic systems with…
This paper presents a first-principle and global perspective of electromagnetic chirality. It follows for this purpose a bottom-up construction, from the description of chiral particles or metaparticles (microscopic scale), through the…
Optical chirality density is widely used as a scalar measure of the chiral properties of electromagnetic fields and their interaction with matter. However, in anisotropic and structured media, a single scalar quantity is generally…
Optical chirality density is a measure of the local handedness of electromagnetic fields. Like energy density, it may be absorbed or scattered through the interaction between light and matter. Here, we utilize the conservation of optical…
Chirality is at the origin of life and is ubiquitous in nature. An object is deemed chiral if it is non-superimposable with its own mirror image. This relates to how circularly polarized light interacts with such object, a circular…
We implement a paraxial azimuthally-radially polarized beam (ARPB), a novel class of structured light beams that can be optimal chiral (OC), leading to maximum chirality density at a given energy density. By using vectorial light shaping…
Structural chirality can induce counter-intuitive optical forces due to inherent symmetry properties. While optical forces on a single chiral particle in the Rayleigh regime have been well studied, optical forces in coupled chiral particles…