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The intraband electromagnetic transitions in the framework of collective Hamiltonian for chiral and wobbling modes are calculated. By going beyond the mean field approximation on the orientations of rotational axis, the collective…

Nuclear Theory · Physics 2021-06-08 X. H. Wu , Q. B. Chen , P. W. Zhao , S. Q. Zhang , J. Meng

We calculate the rate of the spontaneous magnetic dipole radiation transitions from ortho- to para-states of the hydrogen molecule at the room temperature with the radiation wavelengths about 0.01 - 0.1 cm. Exponentially small differences…

Atomic Physics · Physics 2018-11-19 A. M. Ishkhanyan , V. P. Krainov

Energies of np (n=6-9), ns (n=7-9), nd (n=6-8), and nf (n=5-6) states in Tl I and Pb II are obtained using relativistic many-body perturbation theory. Reduced matrix elements, oscillator strengths, transition rates, and lifetimes are…

Atomic Physics · Physics 2009-11-10 U. I. Safronova , M. S. Safronova , W. R. Johnson

Exact solutions for vibrational levels of diatomic molecules via the Morse potential are obtained by means of the asymptotic iteration method. It is shown that, the numerical results for the energy eigenvalues of $^{7}Li_{2}$ are all in…

Quantum Physics · Physics 2009-11-13 T. Barakat , K. Abodayeh

The hydrogen molecule has become a test ground for quantum electrodynamical calculations in molecules. Expanding beyond studies on stable hydrogenic species to the heavier radioactive tritium-bearing molecules, we report on a measurement of…

Chemical Physics · Physics 2018-04-25 T. Madhu Trivikram , M. Schlösser , W. Ubachs , E. J. Salumbides

Chirped-Pulse millimetre-Wave (CPmmW) rotational spectroscopy provides a new class of information about photolysis transition state(s). Measured intensities in rotational spectra determine species-isomer-vibrational populations, provided…

By making use of the quantization rule of Raab and Friedrich [P. Raab and H. Friedrich, Phys. Rev. A 78, 022707 (2008)], we derive simple and accurate formulae for the number of rotational states supported by a weakly-bound vibrational…

Atomic Physics · Physics 2009-06-08 Mikhail Lemeshko , Bretislav Friedrich

Potential energy curves for excited leptonic states of the helium-antihydrogen system are calculated within Ritz' variational approach. An explicitly correlated ansatz for the leptonic wave function is employed describing accurately the…

Atomic Physics · Physics 2015-05-13 V. Sharipov , L. Labzowsky , G. Plunien

The water molecule occurs in two nuclear-spin isomers that differ by the value of the total nuclear spin of the hydrogen atoms, i.e., $I=0$ for para-H$_2$O and $I=1$ for ortho-H$_2$O. Spectroscopic transitions between rovibrational states…

Atomic Physics · Physics 2022-06-08 Andrey Yachmenev , Guang Yang , Emil Zak , Sergei Yurchenko , Jochen Küpper

Spectrally-resolved observations of three pure rotational lines of H$_2$, conducted with the EXES instrument on SOFIA toward the classic bow shock HH7, reveal systematic velocity shifts between the S(5) line of ortho-H$_2$ and the two…

Astrophysics of Galaxies · Physics 2019-06-19 David A. Neufeld , Curtis DeWitt , Pierre Lesaffre , Sylvie Cabrit , Antoine Gusdorf , Le Ngoc Tram , Matthew Richter

Vibrational overtones in deeply bound molecules are sensitive probes for variation of the proton-to-electron mass ratio $\mu$. In nonpolar molecules, these overtones may be driven as two-photon transitions. Here, we present procedures for…

Atomic Physics · Physics 2019-01-03 Ryan Carollo , Alexander Frenett , David Hanneke

The electronic, rotational, and vibrational components of the ultrafast optical nonlinearity in H$_2$ and D$_2$ are measured directly and absolutely at intensities up to the ionization threshold of $\sim$10$^{14}$ W/cm$^2$. As the most…

The visible part ($\approx 550 \div 696$ nm) of the multiline electronic-vibro-rotational emission spectrum of the $D_2$ molecule was recorded with moderate resolution (line widths $\approx 0.013$ nm). The resolution was limited by Doppler…

Chemical Physics · Physics 2012-05-14 B. P. Lavrov , I. S. Umrikhin

The absorption spectrum of CO$_2$ in the wavelength range 120\,nm --- 160\,nm is analyzed by means of quantum mechanical calculations performed using vibronically coupled PESs of five singlet valence electronic states and the coordinate…

Chemical Physics · Physics 2015-06-15 Sergy Yu. Grebenshchikov

Using APEX-1 and APEX-2 observations, we have detected and studied the rotational lines of the HC$_3$N molecule (cyanoacetylene) in the powerful outflow/hot molecular core G331.512-0.103. We identified thirty-one rotational lines at $J$…

By combining a recent precise measurement of the ionization energy of $^{87}$Rb with previous measurements of electronic and hyperfine structure, an accurate value for the $^{85}\textrm{Rb}-^{87}\textrm{Rb}$ isotope shift of the…

Atomic Physics · Physics 2015-05-30 L. Aldridge , P. L. Gould , E. E. Eyler

We have used the Herschel-HIFI instrument to observe both nuclear spin symmetries of amidogen (NH2) towards the high-mass star-forming regions W31C (G10.6-0.4), W49N (G43.2-0.1), W51 (G49.5-0.4) and G34.3+0.1. The aim is to investigate the…

Using the polarisation labelling spectroscopy, we performed the detailed analysis of the level structure of excited electronic states of the $^{39}$KCs molecule in the excitation energy interval between 17500~cm$^{-1}$ and 18600~cm$^{-1}$…

The electron transfer kinetics of mixed-valence systems is studied via solving the eigen-structure of the two-state non-adiabatic diffusion operator for a wide range of electronic coupling constants and energy bias constants. The calculated…

Chemical Physics · Physics 2007-05-23 Y. Jung , R. J. Silbey , J. Cao

Spectra of methyl cyanide were recorded to analyze interactions in low-lying vibrational states and to construct line lists for radio astronomical observations as well as for infrared spectroscopic investigations of planetary atmospheres.…