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The energetic positions of molecular electronic states at molecule/electrode interfaces are crucial factors for determining the transport and optoelectronic properties of molecular junctions. Strong light--matter coupling offers a potential…

Mesoscale and Nanoscale Physics · Physics 2023-05-10 Kuniyuki Miwa , Souichi Sakamoto , Akihito Ishizaki

The rapidly developing and converging fields of polaritonic chemistry and quantum optics necessitate a unified approach to predict strongly-correlated light-matter interactions with atomic-scale resolution. Combining concepts from both…

Quantum Physics · Physics 2018-09-19 Johannes Flick , Prineha Narang

Electron transport in nanoscale devices can often result in nontrivial spatial patterns of voltage and current that reflect a variety of physical phenomena, particularly in nonlocal transport regimes. While numerous techniques have been…

Strongly driving a two-level quantum system with light leads to a ladder of Floquet states separated by the photon energy. Nanoscale quantum devices allow the interplay of confined electrons, phonons, and photons to be studied under strong…

Mesoscale and Nanoscale Physics · Physics 2016-11-09 J. Stehlik , Y. -Y. Liu , C. Eichler , T. R. Hartke , X. Mi , M. J. Gullans , J. M. Taylor , J. R. Petta

In the context of light-matter interactions between organic chromophores and confined photons of (plasmonic) nano-resonators, we introduce a general framework that couples ab initio QM/MM molecular dynamics with few-mode field quantization…

Optics · Physics 2025-11-06 Ruth H. Tichauer , Maksim Lednev , Gerrit Groenhof , Johannes Feist

Recent experiments on nanoscale conductors coupled to microwave cavities put in prospect transport investigations of electron-photon interplay in the deep quantum regime. Here we propose a pump-probe scheme to investigate the transient…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 T. L. van den Berg , C. Bergenfeldt , P. Samuelsson

Photocurrent in solids is an important phenomenon with many applications including the solar cells. In conventional photoconductors, the electrons and holes created by light irradiation are separated by the external electric field,…

Mesoscale and Nanoscale Physics · Physics 2017-03-13 Hiroaki Ishizuka , Naoto Nagaosa

Specific molecular interactions underlie unexpected and useful phenomena in nanofluidic systems, but require descriptions that go beyond traditional macroscopic hydrodynamics. In this letter, we demonstrate how equilibrium molecular…

Mesoscale and Nanoscale Physics · Physics 2023-06-07 Phillip Helms , Anthony R. Poggioli , David T. Limmer

Room temperature cavity quantum electrodynamics with molecular materials in optical cavities offers exciting prospects for controlling electronic, nuclear and photonic degrees of freedom for applications in physics, chemistry and materials…

Quantum Physics · Physics 2025-01-15 Felipe Herrera , William L. Barnes

Continuum simulation is employed to study ion transport and fluid flow through a nanopore in a solid-state membrane under an applied potential drop. Results show the existence of concentration polarization layers on the surfaces of the…

Fluid Dynamics · Physics 2015-06-16 Mao Mao , Sandip Ghosal , Guohui Hu

Using a model comprising a 2-level bridge connecting free electron reservoirs we show that coupling of a molecular bridge to electron-hole excitations in the leads can markedly effect the source-drain current through a molecular junction.In…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

The interplay between static and dynamic disorder and collective optical response in molecular ensembles is an important characteristic of nanoplasmonic and nanophotonic molecular systems. Here we investigate the cooperative superradiant…

The interaction between molecular (atomic) electron(s) and the vacuum field of a reflective cavity generates a significant interest thanks to the rapid developments in nanophotonics. Such interaction which lies within the realm of cavity…

Chemical Physics · Physics 2019-05-22 Alexander Semenov , Abraham Nitzan

In our recent paper [Mosallanejad et al., Phys. Rev. B 107(18), 184314, 2023], we have derived a Floquet electronic friction model to describe nonadiabatic molecular dynamics near metal surfaces in the presence of periodic driving. In this…

Quantum Physics · Physics 2023-09-19 Jingqi Chen , Wei Liu , Wenjie Dou

We analyze the coupling of atoms or atom-like emitters to nanophotonic waveguides in the presence of propagating acoustic waves. Specifically, we show that strong index modulations induced by such waves can drastically modify the effective…

Quantum Physics · Physics 2019-06-03 G. Calajo , M. J. A. Schuetz , H. Pichler , M. D. Lukin , P. Schneeweiss , J. Volz , P. Rabl

We perform a frequency-resolved analysis of electron dynamics in solids to obtain microscopic insight into linear and nonlinear optical phenomena. For the analysis, we first compute the electron dynamics under optical electric fields and…

Materials Science · Physics 2023-07-25 Shunsuke A. Sato

We have carried out calculations of electron transport through a metal-molecule-metal junction with metal nanoclusters taking the part of electrodes. We show that negative differential resistance peaks could appear in the current-voltage…

Materials Science · Physics 2008-10-22 Natalya A. Zimbovskaya , Mark R. Pederson

We developed the theory of elastic electron tunneling through a potential barrier driven by a strong high-frequency electromagnetic field. It is demonstrated that the driven barrier can be considered as a stationary two-barrier potential…

Mesoscale and Nanoscale Physics · Physics 2023-11-13 M. V. Boev , V. M. Kovalev , O. V. Kibis

Molecular conduction operating in dielectric solvent environments are often described using kinetic rates based on Marcus theory of electron transfer at a molecule-metal electrode interface. However, the successive nature of charge transfer…

Chemical Physics · Physics 2020-02-18 Henning Kirchberg , Michael Thorwart , Abraham Nitzan

The article reviews recent progress in the theoretical understanding of near-field surface electromagnetic phenomena in pristine and atomically doped carbon nanotubes. The phenomena involving strong coupling effects are outlined. They are…

Mesoscale and Nanoscale Physics · Physics 2010-11-01 I. V. Bondarev