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Transition metal dichalcogenides (TMDs) are known to support complex excitonic states. Revealing the differences in relaxation dynamics among different excitonic species and elucidating the transition dynamics between them may provide…

Mesoscale and Nanoscale Physics · Physics 2021-04-07 Anran Wang , Yuhan Wang , Jianfei Li , Ning Xu , Songlin Li , Xinran Wang , Yi Shi , Fengqiu Wang

Transition metal dichalcogenide (TMD) monolayers are two-dimensional semiconductors with two valleys in their band structure that can be selectively addressed using circularly polarized light. Their photoluminescence spectrum is…

Mesoscale and Nanoscale Physics · Physics 2020-10-26 Joris J. Carmiggelt , Michael Borst , Toeno van der Sar

Atomically thin semiconducting transition-metal dichalcogenides provide novel insights into the physics of many-body effects mediated by Coulomb interactions. Here, we report on temperature-dependent ($T$ = 7-295 K) reflectance contrast and…

Mesoscale and Nanoscale Physics · Physics 2016-12-14 J. Jadczak , J. Kutrowska-Girzycka , P. Kapuscinski , J. Debus , D. Kudlacik , D. Schmidt , Y. S. Huang , M. Bayer , L. Bryja

The remarkably strong Coulomb interaction in atomically thin transition metal dichalcogenides (TMDs) results in an extraordinarily rich many-particle physics including the formation of tightly bound excitons. Besides optically accessible…

Mesoscale and Nanoscale Physics · Physics 2017-03-10 Malte Selig , Gunnar Berghäuser , Marten Richter , Rudolf Bratschitsch , Andreas Knorr , Ermin Malic

Chiral interaction between light and two-dimensional transition metal dichalcogenides (2D-TMDs) has recently drawn enormous scientific attention. The optical selection rules of these atomically thin semiconductors allow the attribution of a…

Optics · Physics 2021-06-08 Irina Komen , Sabrya E. van Heijst , Sonia Conesa-Boj , L. Kuipers

Interactions between two excitons can result in the formation of bound quasiparticles, known as biexcitons. Their properties are determined by the constituent excitons, with orbital and spin states resembling those of atoms. Monolayer…

Mesoscale and Nanoscale Physics · Physics 2015-09-23 Edbert J. Sie , Alex J. Frenzel , Yi-Hsien Lee , Jing Kong , Nuh Gedik

Atomically thin two-dimensional crystals have revolutionized materials science. In particular, monolayer transition metal dichalcogenides promise novel optoelectronic applications, due to their direct energy gaps in the optical range. Their…

Transition-metal dichalcogenides can be easily produced as atomically thin sheets, exhibiting the possibility to optically polarize and read out the valley pseudospin of extremely stable excitonic quasiparticles present in these 2D…

While valleys (energy extrema) are present in all band structures of solids, their preeminent role in determining exciton resonances and dynamics in atomically thin transition metal dichalcogenides (TMDC) is unique. Using two-dimensional…

The valley pseudospin in monolayer transition metal dichalcogenides (TMDs) has been proposed as a new way to manipulate information in various optoelectronic devices. This relies on a large valley polarization that remains stable over long…

Mesoscale and Nanoscale Physics · Physics 2017-12-22 Fahad Mahmood , Zhanybek Alpichshev , Yi-Hsien Lee , Jing Kong , Nuh Gedik

Two-dimensional excitons formed in quantum materials such as monolayer transition-metal dichalcogenides and their strong light-matter interaction have attracted unrivalled attention by the research community due to their extraordinarily…

Mesoscale and Nanoscale Physics · Physics 2018-12-31 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

We propose a scheme for the spatial exciton energy control and exciton routing in a transition metal dichalcogenide (TMD) monolayer which lies on a quantum paraelectric substrate. It relies on the ultrasensitive response of the substrate…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 V. Shahnazaryan , O. Kyriienko , H. Rostami

Monolayers of transition metal dichalcogenides, namely, molybdenum and tungsten disulfides and diselenides demonstrate unusual optical properties related to the spin-valley locking effect. Particularly, excitation of monolayers by…

Mesoscale and Nanoscale Physics · Physics 2015-11-12 M. M. Glazov , E. L. Ivchenko , G. Wang , T. Amand , X. Marie , B. Urbaszek , B. L. Liu

The strong excitonic effect in monolayer transition metal dichalcogenide (TMD) semiconductors has enabled many fascinating light-matter interaction phenomena. Examples include strongly coupled exciton-polaritons and nearly perfect atomic…

Mesoscale and Nanoscale Physics · Physics 2021-04-13 Hongchao Xie , Shengwei Jiang , Daniel A. Rhodes , James C. Hone , Jie Shan , Kin Fai Mak

Monolayers of transition metal dichalcogenides (TMDCs) feature exceptional optical properties that are dominated by excitons, tightly bound electron-hole pairs. Forming van der Waals heterostructures by deterministically stacking individual…

Single-layer transition metal dichalcogenides (TMDs) provide a promising material system to explore the electron's valley degree of freedom as a quantum information carrier. The valley degree of freedom in single-layer TMDs can be directly…

Mesoscale and Nanoscale Physics · Physics 2019-10-09 Yanhao Tang , Kin Fai Mak , Jie Shan

Transition metal dichalcogenides (TMDs) are regarded as a possible materials platform for quantum information science and related device applications. In TMD monolayers, the dephasing time and inhomogeneity are crucial parameters for any…

The dynamics of exciton formation in transition metal dichalcogenides is difficult to measure experimentally, since many momentum-indirect exciton states are not accessible to optical interband spectroscopy. Here, we combine a tuneable…

We develop a microscopic theory for excitons and cavity exciton polaritons in transition metal dichalcogenide (TMD) monolayers under a perpendicular static magnetic field. We obtain numerically exact solutions for the ground and excited…

Mesoscale and Nanoscale Physics · Physics 2025-01-27 D. de la Fuente Pico , J. Levinsen , E. Laird , M. M. Parish , F. M. Marchetti

Stacking atomic monolayers of semiconducting transition metal dichalcogenides (TMDs) has emerged as an effective way to engineer their properties. In principle, the staggered band alignment of TMD heterostructures should result in the…

Mesoscale and Nanoscale Physics · Physics 2017-09-14 M. Baranowski , A. Surrente , L. Klopotowski , J. M. Urban , N. Zhang , D. K. Maude , K. Wiwatowski , S. Mackowski , Y. C. Kung , D. Dumcenco , A. Kis , P. Plochocka