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We show how dynamical heterogeneities in glass forming systems emerge as a consequence of the existence of dynamical constraints, and we offer an interpretation of the glass transition as an entropy crisis in trajectory space (space-time)…

Statistical Mechanics · Physics 2009-11-07 Juan P. Garrahan , David Chandler

Unraveling the structural factors influencing the dynamics of amorphous solids is crucial. While deep learning aids in navigating these complexities, transparency issues persist. Inspired by the successful application of prototype neural…

Soft Condensed Matter · Physics 2024-03-19 Xiao Jiang , Zean Tian , Kenli Li , Wangyu Hu

When a liquid freezes, a change in the local atomic structure marks the transition to the crystal. When a liquid is cooled to form a glass, however, no noticeable structural change marks the glass transition. Indeed, characteristic features…

Soft Condensed Matter · Physics 2015-11-24 Samuel S. Schoenholz , Ekin D. Cubuk , Daniel M. Sussman , Efthimios Kaxiras , Andrea J Liu

Due to the lack of long-range order, it remains challenging to characterize the structure of disordered solids and understand the nature of the glass transition. Here we propose a new structural order parameter by taking into account…

Soft Condensed Matter · Physics 2024-08-26 Ding Xu , Qinyi Liao , Ning Xu

Using video microscopy, we measure local spatial constraints in disordered binary colloidal samples, ranging from dilute fluids to jammed glasses, and probe their spatial and temporal correlations to local dynamics during the glass…

Soft Condensed Matter · Physics 2019-07-03 Xiunan Yang , Hua Tong , Wei-Hua Wang , Ke Chen

We study the thermodynamic and dynamic phase transitions in two-dimensional polydisperse hard disks using Monte Carlo methods. A conventional local Monte Carlo algorithm allows us to observe a dynamic liquid-glass transition at a density,…

Statistical Mechanics · Physics 2007-05-23 Ludger Santen , Werner Krauth

We investigate the calorimetric liquid-glass transition by performing simulations of a binary Lennard-Jones mixture in one through four dimensions. Starting at a high temperature, the systems are cooled to T=0 and heated back to the ergodic…

Disordered Systems and Neural Networks · Physics 2009-01-01 Ralf Brüning , Denis A. St-Onge , Steve Patterson , Walter Kob

When flat or on a firm mechanical substrate, the atomic composition and atomistic structure of two-dimensional crystals dictate their chemical, electronic, optical, and mechanical properties. These properties change when the two-dimensional…

Mesoscale and Nanoscale Physics · Physics 2014-02-27 Alejandro A. Pacheco Sanjuan , Mehrshad Mehboudi , Edmund O. Harriss , Humberto Terrones , Salvador Barraza-Lopez

Experimental evidence for the possible universality classes of the metal-insulator transition (MIT) in two dimensions (2D) is discussed. Sufficiently strong disorder, in particular, changes the nature of the transition. Comprehensive…

Strongly Correlated Electrons · Physics 2016-03-22 Dragana Popović

One of the central problems of the liquid-glass transition is whether there is a structural signature that can qualitatively distinguish different dynamic behaviors at different degrees of supercooling. Here, we propose a novel structural…

Soft Condensed Matter · Physics 2015-09-24 Yan-Wei Li , You-Liang Zhu , Zhao-Yan Sun

Dynamic heterogeneity in glass-formers has been related to their static structure using the concept of dynamic propensity. We re-examine this relationship by analyzing dynamical fluctuations in two atomistic glass-formers and two…

Statistical Mechanics · Physics 2009-08-25 Ludovic Berthier , Robert L. Jack

The magnetic susceptibility of the 1/1 approximants to icosahedral quasicrystals in a series of Cd85-xMgxTb15 (x = 5, 10, 15, 20) alloys was investigated in detail. The occurrence of antiferromagnetic to spin-glass-like transition was…

This is a commentary on two recent experimental papers in PNAS by Vivek et al. and Illing et al. that convincingly address an issue at the junction of two fundamental questions in glass physics: the role of the dimensionality of space on…

Statistical Mechanics · Physics 2022-06-08 Gilles Tarjus

We investigate the heterogeneity of dynamics, the breakdown of the Stokes-Einstein relation and fragility in a model glass forming liquid, a binary mixture of soft spheres with a harmonic interaction potential, for spatial dimensions from 3…

Soft Condensed Matter · Physics 2021-08-20 Monoj Adhikari , Smarajit Karmakar , Srikanth Sastry

A wide range of materials can exist in microscopically disordered solid forms, referred to as amorphous solids or glasses. Such materials -- oxide glasses and metallic glasses, to polymer glasses, and soft solids such as colloidal glasses,…

Soft Condensed Matter · Physics 2021-08-20 Anshul D. S. Parmar , Srikanth Sastry

We present a combined study of thermal expansion and resistance fluctuation spectroscopy measurements exploring the static and dynamic aspects of the charge-glass formation in the quasi-two-dimensional organic conductors…

Strongly Correlated Electrons · Physics 2022-02-03 Tatjana Thomas , Yohei Saito , Yassine Agarmani , Tim Thyzel , Kenichiro Hashimoto , Takahiko Sasaki , Michael Lang , Jens Müller

The glass transition is a long-standing problem in physics. Identifying the structural origin of the transition may lead to the ultimate solution to the problem. Here, for the first time, we discover such a structural origin by proposing a…

Soft Condensed Matter · Physics 2020-02-13 Xinzhuo Liu , Huaguang Wang , Zexin Zhang , Xinsheng Sean Ling

Using a modified Lennard-Jones model for anisotropic particles, we present results of molecular dynamics simulation in two dimensions. In one-component systems, we find crystallization, a Berezinskii-Kosterlitz-Thouless phase, and a…

Soft Condensed Matter · Physics 2011-12-23 Kyohei Takae , Akira Onuki

Glasses are ubiquitous in daily life and technology. However the microscopic mechanisms generating this state of matter remain subject to debate: Glasses are considered either as merely hyper-viscous liquids or as resulting from a genuine…

Disordered Systems and Neural Networks · Physics 2016-06-14 S. Albert , Th. Bauer , M. Michl , G. Biroli , J. -P. Bouchaud , A. Loidl , P. Lunkenheimer , R. Tourbot , C. Wiertel-Gasquet , F. Ladieu

Mechanical behaviors of bulk metallic glasses (BMGs) including heterogeneous and homogeneous deformation are interpreted by phenomenological shear transformation zones (STZs) model. Currently, information about STZs, i.e. size and density,…

Materials Science · Physics 2018-09-18 Yang Tong
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