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Search for single-molecule magnets with large magnetic anisotropy energy (MAE) is essential for the development of molecular spintronics devices used at room temperature. Through systematic first-principles calculations, we found that an…

Mesoscale and Nanoscale Physics · Physics 2018-04-19 Jiaxing Qu , Jun Hu

In recent years, intrinsic two-dimensional (2D) magnetism aroused great interest because of its potential application in spintronic devices. However, low Curie temperature (\emph{T}$_c$) and magnetic anisotropy energy (MAE) limit its…

Materials Science · Physics 2021-10-01 Tengfei Hu , Wenhui Wan , Yingmei Li , Yanfeng Ge , Yong Liu

In the quest for two-dimensional conducting materials with high ferromagnetic ordering temperature the new family of the layered Fe$_{n}$GeTe$_{2}$ compounds, especially the near-room-temperature ferromagnet Fe$_{4}$GeTe$_{2}$, receives a…

Continuous miniaturization of magnetic units in spintronics and quantum computing devices inspires efforts to search for magnetic nanostructures with large magnetic anisotropy energy (MAE). Typical nanostructures including molecular…

Materials Science · Physics 2014-04-15 Jun Hu , Ruqian Wu

By performing systematic $ab$ $initio$ density functional calculations, here we study two relativity-induced properties of atomically thin ferromagnetic (FM) Cr$_2$Ge$_2$Te$_6$ films [monolayer (ML), bilayer (BL) and trilayer (TL) as well…

Mesoscale and Nanoscale Physics · Physics 2018-09-25 Yimei Fang , Shunqing Wu , Zi-Zhong Zhu , Guang-Yu Guo

Large magnetic anisotropy energy (MAE) is desirable and critical for nanoscale magnetic devices. Here, using ligand-field level diagrams and density functional calculations, we well explain the very recent discovery [I. G. Rau et al.,…

Materials Science · Physics 2015-12-21 Xuedong Ou , Hongbo Wang , Fengren Fan , Zhengwei Li , Hua Wu

In two-dimensional (2D) magnetic systems, large magnetic anisotropy is needed to stabilize the magnetic order according to Mermin-Wagner theorem. Based on density functional theory (DFT) calculations, we propose that the magnetic…

Materials Science · Physics 2020-11-04 Xuejuan-Dong , Jingyang-You , Zheng Zhang , Bo Gu , Gang Su

Exploring giant magnetic anisotropy in small magnetic nanostructures is of both fundamental interest and technological merit for information storage. To prevent spin flipping at room temperature due to thermal fluctuation, large magnetic…

Atomic and Molecular Clusters · Physics 2017-09-07 Xiaoqing Liang , Xue Wu , Jun Hu , Jijun Zhao , Xiao Cheng Zeng

Doped transition-metal dichalcogenides monolayers exhibit exciting magnetic properties for the benefit of two-dimensional spintronic devices. Using density functional theory (DFT) incorporating Hubbard-type of correction (DFT$+U$) to…

Materials Science · Physics 2021-05-12 Adlen Smiri , Sihem Jaziri , Samir Lounis , Iann C. Gerber

Two-dimensional (2D) materials showing room-temperature magnetism and high coercivity are desired for combining magnetism with semiconducting properties useful for spintronics. In this work, the magnetic properties of the 1T phase of…

Perpendicularly magnetized spin injector with high Curie temperature is a prerequisite for developing spin optoelectronic devices on 2D materials working at room temperature (RT) with zero applied magnetic field. Here, we report the growth…

Magnets with controllable magnetization and high critical temperature are essential for practical spintronics devices, among which the two-dimensional 1T-CrTe2 stands out because of its high experimental critical temperature up to about…

Materials Science · Physics 2025-10-14 Fengping Li , Bheema Lingam Chittari , Chao Lei , Jeil Jung

Nano-structures with giant magnetocrystalline anisotropy energies (MAE) are desired in designing miniaturized magnetic storage and quantum computing devices. Through ab initio and model calculations, we propose that special p-element dimers…

Materials Science · Physics 2016-12-28 Rui Pang , Bei Deng , Xingqiang Shi

The anisotropic superconducting properties of a Rb(x)Fe(2-y)Se(2) single crystal with transition temperature 32 K were investigated by means of SQUID and torque magnetometry, probing the effective magnetic penetration depth and the magnetic…

Superconductivity · Physics 2012-02-23 S. Bosma , R. Puzniak , A. Krzton-Maziopa , M. Bendele , E. Pomjakushina , K. Conder , H. Keller , S. Weyeneth

Large magnetic anisotropy and coercivity are key properties of functional magnetic materials and are generally associated with rare earth elements. Here we show an extreme, uniaxial magnetic anisotropy and the emergence of magnetic…

Strongly Correlated Electrons · Physics 2014-02-27 A. Jesche , R. W. McCallum , S. Thimmaiah , J. L. Jacobs , V. Taufour , A. Kreyssig , R. S. Houk , S. L. Bud'ko , P. C. Canfield

We present a comprehensive study on anisotropic magnetocaloric porperties of the van der Waals weak-itinerant ferromagnet Fe$_{3-x}$GeTe$_2$ that features gate-tunable room-temperature ferromagnetism in few-layer device. Intrinsic…

Strongly Correlated Electrons · Physics 2019-09-16 Yu Liu , Jun Li , Jing Tao , Yimei Zhu , C. Petrovic

The development of two-dimensional (2D) room temperature magnets is of great significance to the practical application of spintronic devices. However, the number of synthesized intrinsic 2D magnets is limited and the performances of them…

Materials Science · Physics 2023-10-24 Jing Wu , Ruyi Guo , Daoxiong Wu , Xiuling Li , Xiaojun Wu

Two-dimensional (2D) ferromagnetic materials with high Curie temperature ($T_{\rm c}$) and large magnetic anisotropy energy (MAE) are critical for nanoscale spintronics but remain rare. We propose, via first-principles calculations, that…

Materials Science · Physics 2026-04-07 Yiran Peng , Yanfeng Ge , Yong Liu , Wenhui Wan

We present a first-principles study of the large magneto-crystalline anisotropy in the intercalated di-chalcogenide material \ce{Fe_{0.25}TaS_2}, investigated with the DFT+U approach. We verify a uniaxial magnetocrystalline anisotropy…

Strongly Correlated Electrons · Physics 2016-05-24 Vaideesh Loganathan , Jian-Xin Zhu , Andriy H. Nevidomskyy

Inspired by recent advancements in the field of single-atom magnets, particularly those involving rare-earth (RE) elements, we present a theoretical exploration employing DFT+$U$ calculations to investigate the magnetic properties of…

Mesoscale and Nanoscale Physics · Physics 2024-06-21 Johanna P. Carbone , Gustav Bihlmayer , Stefan Blügel
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