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Order-disorder processes fundamentally determine the structure and properties of many important oxide systems for energy and computing applications. While these processes have been intensively studied in bulk materials, they are less…

Materials Science · Physics 2020-11-10 Steven R. Spurgeon

Herein, fundamentals of topology and symmetry breaking are used to understand crystallization and geometrical frustration in topologically close-packed structures. This frames solidification from a new perspective that is unique from…

Materials Science · Physics 2019-06-13 Carline S. Gorham , David E. Laughlin

The glass transition GT is usually thought of as a structural arrest that occurs during the cooling of a liquid, or sometimes a plastic crystal, trapping a metastable state of the system before it can recrystallize to stabler forms1. This…

Chemical Physics · Physics 2015-05-18 Shuai Wei , Isabella Gallino , Ralf Busch , C. Austen Angell

The underlying structural order that transcends the liquid, glass and crystalline states is identified using an efficient genetic algorithm (GA). GA identifies the most common energetically favorable packing motif in crystalline structures…

Orientation and microstructure are investigated in sheared Brownian suspensions of hard dicolloidal particles, with the dicolloids modeled as two fused spheres of varying radii and center to center separations. Two different particle shapes…

Soft Condensed Matter · Physics 2012-07-24 Amit Kumar , Jonathan J. L. Higdon

The following properties are in the present literature associated with the behavior of super-cooled glass-forming liquids: faster than exponential growth of the relaxation time, dynamical heterogeneities, growing point-to-set correlation…

Statistical Mechanics · Physics 2011-01-25 Florent Krzakala , Lenka Zdeborová

In a preceding paper, Mukhopadhyay and I studied the diffusive motion of a tagged molecule in a heterogeneous glass-forming liquid at temperatures just above a glass transition. Among other features of this system, we postulated a relation…

Statistical Mechanics · Physics 2009-11-13 J. S. Langer

We introduce a minimal model of solid-forming anisotropic molecules that displays, in thermal equilibrium, surface orientational order without bulk orientational order. The model reproduces the nonequilibrium behavior of recent experiments…

Statistical Mechanics · Physics 2021-10-13 Stephen Whitelam , Peter Harrowell

The random first-order transition (RFOT) theory of the structural glass transition is reviewed in a pedagogical fashion. The rigidity that emerges in crystals and glassy liquids is of the same fundamental origin. In both cases, it…

Disordered Systems and Neural Networks · Physics 2015-11-20 Vassiliy Lubchenko

An extended interference pattern close to surface may result in both a transmissive or evanescent surface fields for large area manipulation of trapped particles. The affinity of differing particle sizes to a moving standing wave light…

The thermal conductivity of some orientational glasses of protonated C2H5OH and deuterated C2D5OD ethanol, cyclic substances (cyclohexanol C6H11OH, cyanocyclohexane C6H11CN, cyclohexene C6H10), and freon 112 (CFCl2)2 have been analyzed in…

Disordered Systems and Neural Networks · Physics 2014-04-03 A. I. Krivchikov , G. A. Vdovychenko , O. A. Korolyuk , O. O. Romantsova

Understanding the physics of supercooled liquids near glassy transition remains one of the major challenges in condensed matter science. There has been long recognized that supercooled liquids have spatially dynamical heterogeneity whose…

Statistical Mechanics · Physics 2023-07-10 Viet Nguyen , Xueyu Song

Using molecular dynamics simulations, with a realistic many-body embedded-atom potential, and a novel method to characterize local order, we study the structure of pure nickel during the rapid quench of the liquid and in the resulting…

Disordered Systems and Neural Networks · Physics 2016-08-15 Oscar Rodríguez de la Fuente , José M. Soler

The mode-coupling theory of the glass transition treats the dynamics of supercooled liquids in terms of two-point density correlation functions. Here we consider a generalized, hierarchical formulation of schematic mode-coupling equations…

Statistical Mechanics · Physics 2014-11-27 Liesbeth M. C. Janssen , Peter Mayer , David R. Reichman

A novel kind of crystal order in high-density nanoconfined bilayer ice is proposed from molecular dynamics and density-functional theory simulations. A first-order transition is observed between a low-temperature proton-ordered solid and a…

Soft Condensed Matter · Physics 2016-02-29 Fabiano Corsetti , Jon Zubeltzu , Emilio Artacho

The thermodynamics of a disordered planar vortex array is studied numerically using a new polynomial algorithm which circumvents slow glassy dynamics. Close to the glass transition, the anomalous vortex displacement is found to agree well…

Disordered Systems and Neural Networks · Physics 2009-10-31 Chen Zeng , Paul L. Leath , Terence Hwa

We study slow dynamics of particles moving in a matrix of immobile obstacles using molecular dynamics simulations. The glass transition point decreases drastically as the obstacle density increases. At higher obstacle densities, the…

Soft Condensed Matter · Physics 2009-11-17 Kang Kim , Kunimasa Miyazaki , Shinji Saito

We present an event-driven molecular dynamics study of glass formation in two-dimensional binary mixtures composed of hard disks and hard ellipses, where both types of particles have the same area. We demonstrate that characteristic…

Soft Condensed Matter · Physics 2015-05-27 Wen-Sheng Xu , Xiaozheng Duan , Zhao-Yan Sun , Li-Jia An

We study concentrated colloidal suspensions, a model system which has a glass transition. Samples in the glassy state show aging, in that the motion of the colloidal particles slows as the sample ages from an initial state. We study the…

Soft Condensed Matter · Physics 2007-05-23 Gianguido C. Cianci , Rachel E. Courtland , Eric R. Weeks

In the Mott insulating phase of the transition metal oxides, the effective orbital-orbital interaction is directional both in the orbital space and in the real space. We discuss a classical realization of directional coupling in two…

Strongly Correlated Electrons · Physics 2009-11-10 Anup Mishra , Michael Ma , Fu-Chun Zhang , Siegfried Guertler , Lei-Han Tang , Shaolong Wan
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