Related papers: Unravelling coherences in the FMO complex
Using a formalism adapted to study transport in quantum open systems, that is the nonequilibrium Green's function formalism, we revisit the working principle of the most popular photosynthetic complex, namely the Fenna Matthews-Olson…
Decoherence effects for entangled triplet pairs in organic molecular crystals are analyzed for the case when excitons can hop between inequivalent lattice sites. The fluorescence quantum beats caused by quantum interference upon…
Recent calculations in both flat and de Sitter spacetimes have highlighted a tension between the decoupling of high-energy physics from low-energy degrees of freedom and the expectation that quantum systems decohere due to interactions with…
Floquet engineering of electronic systems is a promising way of controlling quantum material properties on an ultrafast time scale. So far, the energy structure of Floquet states in solids has been observed through time and angle-resolved…
At least two significant roles for large scale quantum coherence in living systems have been suggested: Herbert Fr\"{o}hlich's coherent excitations of nonlinearly coupled ensembles of large polarizable molecules, with frequencies in the…
The electronic excitation population and coherence dynamics in the chromophores of the photosynthetic light harvesting complex 2 (LH2) B850 ring from purple bacteria (Rhodopseudomonas acidophila) have been studied theoretically at both…
Using three-pulse four-wave-mixing optical spectroscopy, we study the ultrafast dynamics of the quantum Hall system. We observe striking differences as compared to an undoped system, where the 2D electron gas is absent. In particular, we…
The nature of excited states of open quantum systems produced by incoherent natural thermal light is analyzed based on a description of the generator of the dynamics. Natural thermal light is shown to generate long-lasting coherent dynamics…
Quantum states inevitably decay with time into a probabilistic mixture of classical states, due to their interaction with the environment and measurement instrumentation. We present the first measurement of the decoherence dynamics of…
We combine the coherent modified Redfield theory (CMRT) with the equation of motion-phase matching approach (PMA) to calculate two-dimensional photon echo spectra for photoactive molecular complexes with an intermediate strength of the…
The coupling between a two-level system and its environment leads to decoherence. Within the context of coherent manipulation of electronic or quasiparticle states in nanostructures, it is crucial to understand the sources of decoherence.…
We show that the coherence between different bacteriochlorophyll-a (BChla) sites in the Fenna-Mathews-Olson complex is an essential ingredient for excitation energy transfer between various sites. The coherence delocalizes the excitation…
There is a remarkable characteristic of photosynthesis in nature, that is, the energy transfer efficiency is close to 100%. Recently, due to the rapid progress made in the experimental techniques, quantum coherent effects have been…
We develop a quantum mechanical formalism to treat the strong coupling between an electromagnetic mode and a vibrational excitation of an ensemble of organic molecules. By employing a Bloch-Redfield-Wangsness approach, we show that the…
We investigate theoretically acoustic phonon induced decoherence in quantum dots. We calculate the dephasing of fundamental (interband or intraband) optical transitions due to real and virtual transitions with higher energy levels. Up to…
High-visibility interference of photon echoes generated in spatially separated solid-state atomic ensembles is demonstrated. The solid state ensembles were LiNbO$_3$ waveguides doped with Erbium ions absorbing at 1.53 $\mu$m. Bright…
Starting from a microscopic model, we investigate the optical spectra of molecules in strongly-coupled organic microcavities examining how they might self-consistently adapt their coupling to light. We consider both rotational and…
The dynamics of excitonic energy transfer in molecular complexes triggered by interaction with laser pulses offers a unique window into the underlying physical processes. The absorbed energy moves through the network of interlinked pigments…
Addressing the role of quantum coherence in the interplay between the different matter constituents (electrons, phonons and spin) is a critical step towards understanding transition metal oxides and design complex materials with new…
Photosynthetic light harvesting provides a natural blueprint for bioengineered and biomimetic solar energy and light detection technologies. Recent evidence suggests some individual light harvesting protein complexes (LHCs) and LHC subunits…