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This paper describes a general method for manipulation of nuclear spins in zero magnetic field. In the absence of magnetic fields, the spins lose the individual information on chemical shifts and inequivalent spins can only be distinguished…

Detecting and controlling nuclear spin nano-ensembles is crucial for the further development of nuclear magnetic resonance (NMR) spectroscopy and for the emerging solid state quantum technology. Here we present the fabrication of a…

The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…

Quantum Physics · Physics 2025-12-15 Hester G. Vennema , Cristina Mier , Evert W. Stolte , Leonard Edens , Jinwon Lee , Sander Otte

We present experimental results which demonstrate that nuclear magnetic resonance spectroscopy is capable of efficiently emulating many of the capabilities of quantum computers, including unitary evolution and coherent superpositions, but…

Quantum Physics · Physics 2009-10-30 David G. Cory , Mark D. Price , Timothy F. Havel

Fifty years of developments in nuclear magnetic resonance (NMR) have resulted in an unrivaled degree of control of the dynamics of coupled two-level quantum systems. This coherent control of nuclear spin dynamics has recently been taken to…

Quantum Physics · Physics 2015-06-26 Lieven M. K. Vandersypen , Isaac L. Chuang

We propose a new approach to the measurement of a single spin state, based on nuclear magnetic resonance (NMR) techniques and inspired by the coherent control over many-body systems envisaged by Quantum Information Processing (QIP). A…

Nuclear magnetic resonance (NMR) spectroscopy is a powerful technique for analyzing the structure and function of molecules, and for performing three-dimensional imaging of the spin density. At the heart of NMR spectrometers is the…

Quantum Physics · Physics 2019-04-15 K. S. Cujia , J. M. Boss , K. Herb , J. Zopes , C. L. Degen

The ability to control and manipulate spins via electrical, magnetic and optical means has generated numerous applications in metrology and quantum information science in recent years. A promising alternative method for spin manipulation is…

Mesoscale and Nanoscale Physics · Physics 2013-04-04 Sungkun Hong , Michael S. Grinolds , Patrick Maletinsky , Ronald L. Walsworth , Mikhail D. Lukin , Amir Yacoby

Experiments in coherent spectroscopy correspond to control of quantum mechanical ensembles guiding them from initial to final target states. The control inputs (pulse sequences) that accomplish these transformations should be designed to…

Quantum Physics · Physics 2009-11-07 Navin Khaneja , Timo Reiss , Burkhard Luy , Steffen J. Glaser

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Quantum sensors have recently achieved to detect the magnetic moment of few or single nuclear spins and measure their magnetic resonance (NMR) signal. However, the spectral resolution, a key feature of NMR, has been limited by relaxation of…

Nuclear spins are highly coherent quantum objects. In large ensembles, their control and detection via magnetic resonance is widely exploited, e.g. in chemistry, medicine, materials science and mining. Nuclear spins also featured in early…

An unusual regime for liquid-state nuclear magnetic resonance (NMR) where the magnetic field strength is so low that the $J$-coupling (intramolecular spin-spin) interactions dominate the spin Hamiltonian opens a new paradigm with…

Atomic Physics · Physics 2019-10-02 Dmitry Budker

The ultimate precision limit in estimating the Larmor frequency of $N$ unentangled rotating spins is well established, and is highly important for magnetometers, gyroscopes and many other sensors. However this limit assumes perfect, single…

Quantum Physics · Physics 2020-10-06 Daniel Cohen , Tuvia Gefen , Laura Ortiz , Alex Retzker

Single-qubit gates are essential components of a universal quantum computer. Without selective addressing of individual qubits, scalable implementation of quantum algorithms is not possible. When the qubits are discrete points or regions on…

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

Nuclear Magnetic Resonance (NMR) forms a natural test-bed to perform quantum information processing (QIP) and has so far proven to be one of the most successful quantum information processors. The nuclear spins in a molecule treated as…

Quantum Physics · Physics 2012-10-30 Soumya Singha Roy

Single-molecule nuclear magnetic resonance (NMR) is a crown-jewel challenge in the field of magnetic resonance spectroscopy and has important applications in chemical analysis and in quantum computing. Recently, it becomes possible to…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Fazhan Shi , Xi Kong , Pengfei Wang , Fei Kong , Nan Zhao , Ren-Bao Liu , Jiangfeng Du

Nuclear Magnetic Ressonance (NMR) is a widely used technique, with a long history of applications in chemestry, medicine, and material science. Twenty years ago, it emerged as a reliable source for quantum computing too, since the work of…

Quantum Physics · Physics 2021-02-24 José L. Figueiredo

Nuclear Magnetic Resonance (NMR) has provided a valuable experimental testbed for quantum information processing (QIP). Here, we briefly review the use of nuclear spins as qubits, and discuss the current status of NMR-QIP. Advances in the…

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