Related papers: Quantum probe hyperpolarisation of molecular nucle…
We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is…
Optically-detected paramagnetic centers in wide-bandgap semiconductors are emerging as a promising platform for nanoscale metrology at room temperature. Of particular interest are applications where the center is used as a probe to…
At temperatures below the magnetic anisotropy energy, monodomain magnetic systems (small particles, nanomagnetic devices, etc.) must relax quantum mechanically. This quantum relaxation must be mediated by the coupling to both nuclear spins…
We recently showed that macroscopic nuclear spin ensembles prepared in coherent spin states can dramatically enhance the interaction rates of weakly interacting cosmic relics-such as dark matter and the cosmic neutrino background-through…
Nuclear Magnetic Resonance (NMR) forms a natural test-bed to perform quantum information processing (QIP) and has so far proven to be one of the most successful quantum information processors. The nuclear spins in a molecule treated as…
Van der Waals layered materials are a focus of materials research as they support strong quantum effects and can easily form heterostructures. Electron spins in van der Waals materials played crucial roles in many recent breakthroughs,…
We consider two new quantum gate mechanisms based on nuclear spins in hyperpolarized solid $^{129}Xe$ and HCl mixtures and inorganic semiconductors. We propose two schemes for implementing a controlled NOT (CNOT) gate based on nuclear…
We have theoretically analyzed coherent nuclear-spin dynamics induced by electron transport through a quantum-dot spin valve. The hyperfine interaction between electron and nuclear spins in a quantum dot allows for the transfer of angular…
We theoretically investigate dynamic nuclear spin polarization in a self-assembled quantum dot pumped optically by two laser beams. With the assumption that a noncollinear interaction between the hole spin and nuclear spins leads to nuclear…
Repeated injection of spin polarized carriers in a quantum dot leads to the polarization of nuclear spins, a process known as dynamic nuclear spin polarization (DNP). Here, we report the first observation of p-shell carrier assisted DNP in…
Nuclear-spin qubits have long coherence time and are desirably applied into quantum information processing. However, the existing methods either fail to address single nucleus (such as nuclear magnetic resonance), or severely affect nuclear…
The shaping of nuclear spin polarization profiles and the induction of nuclear resonances are demonstrated within a parabolic quantum well using an externally applied gate voltage. Voltage control of the electron and hole wave functions…
A microscopic theory of spin fluctuations of localized electrons interacting with optically cooled nuclear spin bath has been developed. Since nuclear spin temperature may stay low enough for macroscopically long time, the nuclear spin…
We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the Cross Effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate…
Nuclear quadrupolar resonance (NQR) spectroscopy reveals chemical bonding patterns in materials and molecules through the unique coupling between nuclear spins and local fields. However, traditional NQR techniques require macroscopic…
The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature…
We perform sensitive nuclear magnetic resonance (NMR) with spin ensembles which are polarized by nitrogen vacancy centers (NV centers) in diamond at room-temperature. With a near shot-noise-limited photoluminescence detection and a highly…
Most of dynamic nuclear polarization (DNP) has been requiring helium cryogenics and strong magnetic fields for a high degree of polarization. In this work, we instead demonstrate an optical hyperpolarization of naturally abundant $^{13}$C…
Precise control of the resonant frequency of a spin qubit is of fundamental importance to quantum sensing protocols. We demonstrate a control technique on a single nitrogen-vacancy (NV) centre in diamond where the applied magnetic field is…
Diamond-based quantum sensors have enabled high-resolution NMR spectroscopy at the microscale in scenarios where fast molecular motion averages out dipolar interactions among target nuclei. However, in samples with low-diffusion, ubiquitous…