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We explore the glassy dynamics of soft colloids using microgels and charged particles interacting by steric and screened Coulomb interactions, respectively. In the supercooled regime, the structural relaxation time $\tau_\alpha$ of both…

We investigate structural and dynamical properties of moderately polydisperse emulsions across an extended range of droplet volume fractions phgr, encompassing fluid and glassy states up to jamming. Combining experiments and simulations, we…

Soft Condensed Matter · Physics 2017-10-09 Chi Zhang , Nicoletta Gnan , Thomas G. Mason , Emanuela Zaccarelli , Frank Scheffold

Much attention has been devoted to water's metastable phase behavior, including polyamorphism (multiple amorphous solid phases), and the hypothesized liquid-liquid transition and associated critical point. However, the possible relationship…

Soft Condensed Matter · Physics 2021-06-09 Thomas E. Gartner , Salvatore Torquato , Roberto Car , Pablo G. Debenedetti

By systematically varying the mobility of self-propelled particles in a two-dimensional (2D) lattice, we experimentally study the influence of particle mobility on system's collective motion. Our system is intrinsically non-equilibrium due…

Soft Condensed Matter · Physics 2016-02-19 Hongchuan Shen , Peng Tan , Lei Xu

A fresh approach to the data from experiments with hard sphere colloids yields seminal insights into the glass transition. The precise determination of the fraction of particles caged by their neighbours is unprecedented and provides…

Soft Condensed Matter · Physics 2021-10-01 W. van Megen , H. J. Schöpe

We review recent developments in structural-dynamical phase transitions in trajectory space. An open question is how the dynamic facilitation theory of the glass transition may be reconciled with thermodynamic theories that posit a…

Statistical Mechanics · Physics 2020-08-04 C. Patrick Royall , Francesco Turci , Thomas Speck

The glass transition refers to the non-equilibrium process by which an equilibrium liquid is transformed to a non-equilibrium disordered solid, or vice versa. Associated response functions, such as heat capacities, are markedly different on…

Soft Condensed Matter · Physics 2013-03-26 Aaron S. Keys , Juan P. Garrahan , David Chandler

The physics of glasses can be studied from many viewpoints, from material scientists interested in the development of new materials to statistical physicists inventing new theoretical tools to deal with disordered systems. In these lectures…

Statistical Mechanics · Physics 2007-05-23 Ludovic Berthier

The self-organization of active particles is governed by their dynamic effective interactions. Such interactions are controlled by the medium in which such active agents reside. Here, we study the interactions between active agents in a…

Soft Condensed Matter · Physics 2016-06-08 J. L. Aragones , J. P. Steimel , A. Alexander-Katz

Aspects of the dynamical glass transition are considered within a mean field spin glass model. At the dynamical transition the the system condenses in a state of lower entropy. The difference, the information entropy or complexity, is…

Condensed Matter · Physics 2007-05-23 Th. M. Nieuwenhuizen

Many properties of solids such as the glass state are commonly treated as nonequilibrium phenomena, which involve many conceptual difficulties. However, few studies have addressed the problem of understanding equilibrium itself. Equilibrium…

Statistical Mechanics · Physics 2022-01-05 Koun Shirai

We study the role of elasticity-induced facilitation on the dynamics of glass-forming liquids by a coarse-grained two-dimensional model in which local relaxation events, taking place by thermal activation, can trigger new relaxations by…

Disordered Systems and Neural Networks · Physics 2023-04-05 Misaki Ozawa , Giulio Biroli

Glasses are out-of-equilibrium systems aging under the crystallization threat. During ordinary glass formation, the atomic diffusion slows down rendering its experimental investigation impractically long, to the extent that a timescale…

Disordered Systems and Neural Networks · Physics 2015-08-28 E. A. A. Pogna , C. Rodríguez-Tinoco , G. Cerullo , C. Ferrante , J. Rodríguez-Viejo , T. Scopigno

We explore the dynamics of a simple liquid whose particles, in addition to standard potential-based interactions, are also subjected to transverse forces preserving the Boltzmann distribution. We derive the effective dynamics of one and two…

Soft Condensed Matter · Physics 2024-06-18 Federico Ghimenti , Ludovic Berthier , Grzegorz Szamel , Frédéric van Wijland

We show that the dynamics of a laser driven Rydberg gas in the limit of strong dephasing is described by a master equation with manifest kinetic constraints. The equilibrium state of the system is uncorrelated but the constraints in the…

Atomic Physics · Physics 2015-06-16 Igor Lesanovsky , Juan P. Garrahan

Dynamic facilitation theory assumes short-ranged dynamic constraints to be the essential feature of supercooled liquids and draws much of its conclusions from the study of kinetically constrained models. While deceptively simple, these…

Materials Science · Physics 2012-06-12 Thomas Speck , David Chandler

We present experimental confirmation of dynamic facilitation in monodisperse and bidisperse colloidal suspensions near the glass transition volume fraction. Correlations in particle dynamics are seen to exist not only in space (clusters and…

Soft Condensed Matter · Physics 2014-06-24 Scott V. Franklin , Eric R. Weeks

We investigate the dynamics of a driven system of dissipative hard spheres in the framework of mode-coupling theory. The dissipation is modeled by normal restitution, and driving is applied to individual particles in the bulk. In such a…

Soft Condensed Matter · Physics 2010-06-29 W. Till Kranz , Matthias Sperl , Annette Zippelius

We use computer simulations to study the glass transition of dense fluids made of polydisperse, repulsive spheres. For hard particles, we vary the volume fraction, phi, and use compressible particles to explore finite temperatures, T>0. In…

Statistical Mechanics · Physics 2009-08-25 Ludovic Berthier , Thomas A. Witten

The dramatic slowdown of dynamics in supercooled liquids approaching the glass transition remains one of the central unresolved problems in condensed matter physics. We review approaches that attribute this slowdown to growing thermodynamic…

Soft Condensed Matter · Physics 2026-03-06 Massimo Pica Ciamarra , Jeppe C. Dyre , Edan Lerner , Matthieu Wyart
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